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Thermally Enhanced High-sensitivity Temperature Probe ScF3: Nd3+/Yb3+/Er3+ Based on Negative Thermal Expansion
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Minkun JIN, Jinmeng XIANG, Changheng CHEN, Yuexin LI, Jingjing TANG, Chongfeng GUO
Journal of the Chinese Ceramic Society | 2022, 50(12) : 3116 - 3125
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Journal of the Chinese Ceramic Society | 2022, 50(12): 3116-3125
• Research Articles •
Thermally Enhanced High-sensitivity Temperature Probe ScF3: Nd3+/Yb3+/Er3+ Based on Negative Thermal Expansion
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Minkun JIN, Jinmeng XIANG, Changheng CHEN, Yuexin LI, Jingjing TANG, Chongfeng GUO
Affiliations
  • State Key Laboratory of Photon-Technology in Western China Energy, Institute of Photonics & Photon-Technology, Northwest University, Xi'an 710069, China

    • JIN Minkun (1997-), male, Doctoral candidate. E-mail:

About Author:

JIN Minkun (1997-), male, Doctoral candidate. E-mail:

Published: 2022-12-20 doi: 10.14062/j.issn.0454-5648.20220469
Outline
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Rapid and non-invasive temperature detection inside biological tissues can be realized through a fluorescence intensity ratio thermometry technology, but it is still restricted due to the thermal quenching of fluorescence and the large absorption and scattering coefficients of tissues in practical applications. In this paper, cubic phase ScF3:Yb3+/Er3+ nanocrystals with negative thermal expansion characteristics were synthesized by a one-step hydrothermal method, in which the thermal enhancement of up-conversion (UC) luminescence was achieved due to the thermally improved energy transfer efficiency from a shortened distance between the activator and sensitizer. For further realizing its application in biology, Nd3+ was introduced in ScF3:Yb3+/Er3+ to construct a high-sensitivity temperature probe with near-infrared (NIR) excitation and NIR emission. Furthermore, calibrating the temperature measurement curve and designing the ex vivo experiment rationally can give a potential temperature detection of the present sample inside the tissue. The results indicate a strategy for solving the UC luminescence thermal quenching and developing NIR emission temperature probes for organisms.

negative thermal expansion  /  energy transfer  /  fluorescence intensity ratio  /  thermometer
金旻坤, 向进猛, 陈长恒, 李玥欣, 唐晶晶, 郭崇峰. 基于负热膨胀的热增强型ScF3：Nd3+/Yb3+/Er3+高灵敏度温度探针. 硅酸盐学报, 2022 , 50 (12) : 3116 -3125 . DOI: 10.14062/j.issn.0454-5648.20220469
Minkun JIN, Jinmeng XIANG, Changheng CHEN, Yuexin LI, Jingjing TANG, Chongfeng GUO. Thermally Enhanced High-sensitivity Temperature Probe ScF3: Nd3+/Yb3+/Er3+ Based on Negative Thermal Expansion[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (12) : 3116 -3125 . DOI: 10.14062/j.issn.0454-5648.20220469
Appendix
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Year 2022 volume 50 Issue 12
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Article Info
doi: 10.14062/j.issn.0454-5648.20220469
  • Receive Date：2022-06-10
  • Online Date：2026-10-20
  • Published：2022-12-20
Article Data
Affiliations
History
  • Received：2022-06-10
  • Revised：2022-08-26
Funding
Affiliations
    State Key Laboratory of Photon-Technology in Western China Energy, Institute of Photonics & Photon-Technology, Northwest University, Xi'an 710069, China

Corresponding:

GUO Chongfeng (1975-), male, Ph.D., Professor. E-mail:
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表12种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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