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Solid-State Synthesis of Spherical-like Silicalite-1 Zeolite
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Mingquan LI, Jiayuan WANG, Yajie FU, Xu SUN, Ruiqin YANG, Chuang XING
Journal of the Chinese Ceramic Society | 2021, 49(10) : 2089 - 2097
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Journal of the Chinese Ceramic Society | 2021, 49(10): 2089-2097
Solid-State Synthesis of Spherical-like Silicalite-1 Zeolite
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Mingquan LI, Jiayuan WANG, Yajie FU, Xu SUN, Ruiqin YANG, Chuang XING
Affiliations
  • School of Biological and Chemical Engineering, Zhejiang University of Science and Technology, Hangzhou 310023, China
  • LI Mingquan (1997-), male, Master candidate. E-mail:

About Author:

LI Mingquan (1997-), male, Master candidate. E-mail:

Published: 2021-10-20 doi: 10.14062/j.issn.0454-5648.20200912
Outline
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Clustered crystals of Silicalite-1 forming spherical-like structures were synthesized by a solvent-free solid-state method using activated carbon as a hard template. The influence of activated carbon dosage on the Silicalite-1 zeolite was explored by X-ray diffraction, specific surface area analysis, scanning electron microscopy, transmission electron microscopy, infrared spectroscopy, and X-ray photoelectric spectroscopy. The results show that the C—O—Si bond is formed between hydroxyl groups on the surface of activated carbon and silicic acid, growing and aggregating along the activated carbon and formed spherical-like Silicalite-1 zeolites after calcination. The spherical-like Silicalite-1 prepared with 10% (in mass fraction) activated carbon has a greater crystallinity with great specific surface area and pore volume as well as uniform particle size.

activated carbon  /  hard template  /  solid-state synthesis  /  spherical-like  /  zeolite
李明权, 王佳元, 傅亚杰, 孙旭, 杨瑞芹, 邢闯. 固相合成法制备类球形Silicalite-1分子筛. 硅酸盐学报, 2021 , 49 (10) : 2089 -2097 . DOI: 10.14062/j.issn.0454-5648.20200912
Mingquan LI, Jiayuan WANG, Yajie FU, Xu SUN, Ruiqin YANG, Chuang XING. Solid-State Synthesis of Spherical-like Silicalite-1 Zeolite[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (10) : 2089 -2097 . DOI: 10.14062/j.issn.0454-5648.20200912
Year 2021 volume 49 Issue 10
22
5
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Article Info
doi: 10.14062/j.issn.0454-5648.20200912
  • Receive Date:2020-12-11
  • Online Date:2026-10-30
  • Published:2021-10-20
Article Data
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History
  • Received:2020-12-11
  • Revised:2021-04-17
Funding
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    School of Biological and Chemical Engineering, Zhejiang University of Science and Technology, Hangzhou 310023, China

Corresponding:

XING Chuang (1986-), male, Ph.D., Associate Professor. E-mail:
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表12种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
total species (%)
属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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