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Preparation of Zeolite T Membranes for Isopropanol Dehydration Using Homogenous Liquid Precursors
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Yi LIU, Huizhi ZHANG, Jiayou ZHANG, Fei ZHANG, Tian GUI, Na HU, Xiangshu CHEN
Journal of the Chinese Ceramic Society | 2020, 48(2) : 316 - 324
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Journal of the Chinese Ceramic Society | 2020, 48(2): 316-324
Preparation of Zeolite T Membranes for Isopropanol Dehydration Using Homogenous Liquid Precursors
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Yi LIU, Huizhi ZHANG, Jiayou ZHANG, Fei ZHANG, Tian GUI, Na HU, Xiangshu CHEN
Affiliations
  • Institute of Advanced Materials (IAM), State-Province Joint Engineering Laboratory of Zeolite Membrane Materials, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, China
  • LIU Yi (1994-), female, Master candidate. E-mail:

About Author:

LIU Yi (1994-), female, Master candidate. E-mail:

Published: 2020-02-20 doi: 10.14062/j.issn.0454-5648.20190376
Outline
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Thin and dense zeolite T membranes with a thickness of 5 μm on low-cost mullite tubular supports were synthesized via two-stage varying-temperature crystallization (TSVTC) with homogeneous liquid precursors. Effect of precursors on the crystal morphology and pervaporation performance of as-synthesized membranes, and synthesis time/temperature during the two-stage hydrothermal crystallization process was investigated. The results show that zeolite T membranes synthesized under optimized conditions have an enhanced pervaporation performance (i.e., the high flux of 4.3 kg/(m2·h), and the separation factor of 2 000 in water/isopropanol (10/90, mass ratio) aqueous solution at 348 K). These membranes show a good reproducibility and a long-term hydrothermal stability as well.

zeolite membrane  /  homogeneous liquid precursor  /  two-stage varying-temperature crystallization  /  crystal growth  /  pervaporation
刘义, 张慧智, 张家友, 张飞, 桂田, 胡娜, 陈祥树. 均相溶胶体系合成用于异丙醇脱水的T型分子筛膜. 硅酸盐学报, 2020 , 48 (2) : 316 -324 . DOI: 10.14062/j.issn.0454-5648.20190376
Yi LIU, Huizhi ZHANG, Jiayou ZHANG, Fei ZHANG, Tian GUI, Na HU, Xiangshu CHEN. Preparation of Zeolite T Membranes for Isopropanol Dehydration Using Homogenous Liquid Precursors[J]. Journal of the Chinese Ceramic Society, 2020 , 48 (2) : 316 -324 . DOI: 10.14062/j.issn.0454-5648.20190376
Year 2020 volume 48 Issue 2
29
6
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Article Info
doi: 10.14062/j.issn.0454-5648.20190376
  • Receive Date:2019-07-01
  • Online Date:2026-10-29
  • Published:2020-02-20
Article Data
Affiliations
History
  • Received:2019-07-01
  • Revised:2019-08-01
Funding
Affiliations
    Institute of Advanced Materials (IAM), State-Province Joint Engineering Laboratory of Zeolite Membrane Materials, College of Chemistry and Chemical Engineering, Jiangxi Normal University, Nanchang 330022, China

Corresponding:

HU Na (1984-), female, Ph.D., Senior Experimentalist; E-mail:
CHEN Xiangshu (1966-), male, Ph.D., Professor.
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表12种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
total species (%)
属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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