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Research Progress on Recovery and Regeneration of Valuable Metals from Cathode Materials of Spent Ternary Lithium-ion Batteries
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Hao ZHANG1, Dongqi SONG1, Qingkang YAN1, Mingjun BAI2, Hao WAN3, Hui GUO1
Hydrometallurgy of China | 2024, 43(5) : 513 - 523
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Hydrometallurgy of China | 2024, 43(5): 513-523
• Reviews •
Research Progress on Recovery and Regeneration of Valuable Metals from Cathode Materials of Spent Ternary Lithium-ion Batteries
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Hao ZHANG1, Dongqi SONG1, Qingkang YAN1, Mingjun BAI2, Hao WAN3, Hui GUO1
Affiliations
  • 1 School of Chemical Engineering, Zhengzhou University, Zhengzhou 450001, China
  • 2 College of Materials Science and Engineering, Chongqing University of Technology, Chongqing 400054, China
  • 3 Zhongyuan Critical Metals Laboratory, Zhengzhou University, Zhengzhou 450001, China
Published: 2024-10-20 doi: 10.13355/j.cnki.sfyj.2024.05.006
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The cathode material of spent ternary lithium-ion battery is rich in valuable metals such as Li, Ni, Co and Mn, and efficient separation and recovery of these metals is crucial for environmental protection. The principles, conditions and effects of chemical precipitation, solvent extraction and electrochemical deposition for the separation of dissolved Li, Ni, Co and Mn are evaluated and analyzed. According to the failure mechanism of NCM cathode material, the development status, advantages and disadvantages of direct regeneration strategy of solid-state sintering, hydrothermal method and lithium based eutectic molten salt method, and indirect regeneration strategy of coprecipitation method, sol-gel method and electrochemical method are systematically reviewed. The challenges faced in the separation of valuable metals such as lithium, nickel, cobalt and manganese and the recycling of electrode materials are summarized, and the improvement direction is put forward to provide important guidance for the efficient recycling of valuable metals in the cathode materials of spent ternary lithium-ion batteries.

spent ternary lithium-ion batteries  /  cathode material  /  separation  /  regeneration  /  valuable metals  /  research progress
Hao ZHANG, Dongqi SONG, Qingkang YAN, Mingjun BAI, Hao WAN, Hui GUO. Research Progress on Recovery and Regeneration of Valuable Metals from Cathode Materials of Spent Ternary Lithium-ion Batteries[J]. Hydrometallurgy of China, 2024 , 43 (5) : 513 -523 . DOI: 10.13355/j.cnki.sfyj.2024.05.006
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doi: 10.13355/j.cnki.sfyj.2024.05.006
  • Receive Date：2024-07-01
  • Online Date：2025-09-10
  • Published：2024-10-20
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  • Received：2024-07-01
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Affiliations
    1 School of Chemical Engineering, Zhengzhou University, Zhengzhou 450001, China
    2 College of Materials Science and Engineering, Chongqing University of Technology, Chongqing 400054, China
    3 Zhongyuan Critical Metals Laboratory, Zhengzhou University, Zhengzhou 450001, China
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https://castjournals.cast.org.cn/joweb/sfyj/EN/10.13355/j.cnki.sfyj.2024.05.006
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表12种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
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Percentage of total
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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