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Simulation and Measurement of Solid Phase Distribution in Fluidized Bed Hydrogen Reduction for Preparation of Uranium Oxide
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Haonan SHEN, Yuqing NIU, Dabing LI, Shaohui KANG, Xiuming KANG, Kaikai YE, Jiayu ZHANG
Hydrometallurgy of China | 2025, 44(6) : 759 - 765
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Hydrometallurgy of China | 2025, 44(6): 759-765
• Experiment Research •
Simulation and Measurement of Solid Phase Distribution in Fluidized Bed Hydrogen Reduction for Preparation of Uranium Oxide
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Haonan SHEN, Yuqing NIU, Dabing LI, Shaohui KANG, Xiuming KANG, Kaikai YE, Jiayu ZHANG
Affiliations
  • Beijing Research Institute of Chemical Engineering and Metallurgy, CNNC, Beijing 101149, China
Published: 2025-12-20 doi: 10.13355/j.cnki.sfyj.2025.06.007
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In order to determine the solid phase distribution law of UO2 particles during the gas-liquid-solid fluidization process, Fluidization behavior of nickel powder (simulating catalyst) and alumina (simulating UO2 product) in a cold model experiment of a magnetic field-assisted gas-liquid-solid three-phase fluidized bed, with a focus on separation characteristics under magnetic field regulation were systematically investigated. The results show that in the absence of a magnetic field, the axial solid content distribution of alumina particles varies significantly with the gas flow rates (5-40 L/min). Under low gas flow rates (5-20 L/min), a high-concentration deposition zone is formed at the bottom of the bed, and the larger the particle size, the more obvious the deposition effect. Under medium and high gas flow rates (25-40 L/min), large bubbles break to enhance axial mixing, but the solid content at the top is still lower than that at the bottom. Nickel powder shows significant differences due to its high-density characteristics. Fine particles (200-300 mesh) require a gas flow rate of ≥15 L/min to achieve quasi-uniform dispersion, while coarse particles (100-200 mesh) remain deposited at the bottom of the bed even when the gas flow rate reaches 40 L/min. After the application of a magnetic field, nickel particles gradually accumulate in the lower part of the bed as the magnetic field intensity increases, forming magnetic agglomerated "apparent large particles" that are stably deposited near the gas distribution plate, while non-magnetic alumina floats up with the liquid flow. Under the same magnetic field the solid content ratio of nickel powder to alumina to increase from top to bottom, but the ratio drops rapidly with the strengthening of the magnetic field, indicating a significant aggregation effect of magnetic particles. The research results verified the dynamic separation efficiency of magnetic field-assisted fluidized beds for magnetic catalysts and non-magnetic products, clarified the key parameters of gas flow rate, magnetic field intensity and particle matching, and provided theoretical support for the design of continuous reactors in uranium chemical industry.

magnetized fluidized bed  /  hydrogen reduction  /  preparation  /  uranium oxide  /  gas-liquid-solid three-phase  /  solids concentration distribution
申浩楠, 牛玉清, 李大炳, 康绍辉, 康修铭, 叶开凯, 张佳宇. 流化床氢还原制备铀氧化物固相分布模拟测定研究. 湿法冶金, 2025 , 44 (6) : 759 -765 . DOI: 10.13355/j.cnki.sfyj.2025.06.007
Haonan SHEN, Yuqing NIU, Dabing LI, Shaohui KANG, Xiuming KANG, Kaikai YE, Jiayu ZHANG. Simulation and Measurement of Solid Phase Distribution in Fluidized Bed Hydrogen Reduction for Preparation of Uranium Oxide[J]. Hydrometallurgy of China, 2025 , 44 (6) : 759 -765 . DOI: 10.13355/j.cnki.sfyj.2025.06.007
Year 2025 volume 44 Issue 6
156
34
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doi: 10.13355/j.cnki.sfyj.2025.06.007
  • Receive Date:2025-05-10
  • Online Date:2026-09-28
  • Published:2025-12-20
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  • Received:2025-05-10
Affiliations
    Beijing Research Institute of Chemical Engineering and Metallurgy, CNNC, Beijing 101149, China
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表12种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
total species (%)
属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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