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Microstructural engineering of two-dimensional clay-based materials for advanced electrochemical energy conversion
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Ruiqian Zhanga, Binbin Qianb, Ke Xub, Amir Saida, Kunfeng Chenc, Chunlei Yanga, Sridhar Komarnenid, Dongfeng Xueb, *
Review of Materials Research | 2025, 1(1) : 100016
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Review of Materials Research | 2025, 1(1): 100016
• CONCISE REVIEW •
Microstructural engineering of two-dimensional clay-based materials for advanced electrochemical energy conversion
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Ruiqian Zhanga, Binbin Qianb, Ke Xub, Amir Saida, Kunfeng Chenc, Chunlei Yanga, Sridhar Komarnenid, Dongfeng Xueb, *
Affiliations
  • aCenter for Photonics Information and Energy Materials, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen, 518055, China
  • bShenzhen Institute for Advanced Study, University of Electronic Science and Technology of China, Shenzhen, 518110, China
  • cState Key Laboratory of Crystal Materials, Institute of Novel Semiconductors, Shandong University, Jinan, 250100, China
  • dMaterials Research Institute and Department of Ecosystem Science and Management, 204 Energy and the Environment Laboratory, The Pennsylvania State University, University Park, PA, 16802, USA
Published: 2025-04-08 doi: 10.1016/j.revmat.2025.100016
Outline
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Two-dimensional clay-based materials have shown significant potential in key electrochemical processes, including hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and oxygen reduction reaction (ORR). Two-dimensional clay-based materials possess intrinsic properties such as porous structures, tunable specific surface areas, excellent thermal and mechanical stability, abundant reserves, and cost-effectiveness. However, limited electrocatalytic activity of two-dimensional clay-based materials remains a major challenge. The issue is closely tied to microscopic structures, including spin states, orbital hybridization, energy band alignment, and lattice stability of two-dimensional clay-based materials. The review delves into the relationship between modified two-dimensional clay-based materials and catalytic performance, summarizing strategies such as defect engineering and heteroatom doping to enhance orbital overlap, thereby improving HER, OER, and ORR activities. Finally, this review discusses the development prospects of clay-based materials, emphasizing the critical role of combining advanced computational and experimental techniques in driving innovations in energy conversion materials.

Two-dimensional clay-based materials  /  Energy conversion  /  Non-noble metal electrocatalysts
Ruiqian Zhang, Binbin Qian, Ke Xu, Amir Said, Kunfeng Chen, Chunlei Yang, Sridhar Komarneni, Dongfeng Xue. Microstructural engineering of two-dimensional clay-based materials for advanced electrochemical energy conversion[J]. Review of Materials Research, 2025 , 1 (1) : 100016 - . DOI: 10.1016/j.revmat.2025.100016
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  • National Natural Science Foundation of China(52220105010; 52203343; M-0755)
  • Guangdong Basic and Applied Basic Research Foundation(2023A1515010052)
  • Key Technologies R&D Program of Guangdong Province(2024B0101070003)
  • Shenzhen Science and Technology Program(SGDX20230116092051001; RCBS20221008093303001)
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Year 2025 volume 1 Issue 1
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6
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Article Info
doi: 10.1016/j.revmat.2025.100016
  • Receive Date：2025-03-21
  • Online Date：2026-06-10
  • Published：2025-04-08
Article Data
Affiliations
History
  • Received：2025-03-21
  • Revised：2025-04-07
  • Accepted：2025-04-07
Funding
National Natural Science Foundation of China(52220105010; 52203343; M-0755)
Guangdong Basic and Applied Basic Research Foundation(2023A1515010052)
Key Technologies R&D Program of Guangdong Province(2024B0101070003)
Shenzhen Science and Technology Program(SGDX20230116092051001; RCBS20221008093303001)
Affiliations
    aCenter for Photonics Information and Energy Materials, Shenzhen Institute of Advanced Technology, Chinese Academy of Sciences, Shenzhen, 518055, China
    bShenzhen Institute for Advanced Study, University of Electronic Science and Technology of China, Shenzhen, 518110, China
    cState Key Laboratory of Crystal Materials, Institute of Novel Semiconductors, Shandong University, Jinan, 250100, China
    dMaterials Research Institute and Department of Ecosystem Science and Management, 204 Energy and the Environment Laboratory, The Pennsylvania State University, University Park, PA, 16802, USA

Corresponding:

* E-mail address: (D. Xue).
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表12种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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