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Electrolyte modulation strategies towards cathode-electrolyte interphase engineering in subzero-temperature lithium-ion batteries
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Zihan Xiong, Fanbo Meng, Jiahe Chen, Zhenzhong Yang, Renzong Hu*, Min Zhu
Review of Materials Research | 2025, 1(1) : 100012
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Review of Materials Research | 2025, 1(1): 100012
• COMPREHENSIVE SURVEY •
Electrolyte modulation strategies towards cathode-electrolyte interphase engineering in subzero-temperature lithium-ion batteries
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Zihan Xiong, Fanbo Meng, Jiahe Chen, Zhenzhong Yang, Renzong Hu*, Min Zhu
Affiliations
  • School of Materials Science and Engineering, Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510640, China
Published: 2025-04-07 doi: 10.1016/j.revmat.2025.100012
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Failure of lithium-ion batteries (LIBs) under subfreezing conditions limits their further development in aerospace and military applications, including severe capacity degradation, poor charge ability, and safety issue. Sluggish electrochemical reaction kinetics in the cathode-electrolyte interphases (CEI) would restrict the diffusion transfer of electric charge and Li+ ions, which is regarded as the main factor contributing to the low-temperature electrochemical failure issue. This review introduces and discusses the latest important interfacial CEI engineering on the layered oxide cathode in enhancing the low-temperature performance of LIBs based on the electrolyte modulation strategies. Firstly, the interfacial issues of layered oxide cathodes and the formation mechanism of CEI film under subzero temperatures are introduced. Secondly, recent progress about the interfacial engineering on inducing CEI construction under low temperature is summarized in terms of the components mainly involved in anions of Li salt, solvent molecule and additive. Thirdly, considering the unique composition and structure of CEI films, advanced interfacial characterization techniques and analysis are summarized. Finally, a perspective of electrolyte design matched with layered cathode materials in low-temperature LIBs is further presented, which may supply a new sight into designs and manufacture of LIBs and other devices for subzero-temperature applications.

Low-temperature performance  /  Cathode-electrolyte interface  /  Electrolyte modulation  /  Layered oxide cathode  /  Electrochemical kinetics reaction
Zihan Xiong, Fanbo Meng, Jiahe Chen, Zhenzhong Yang, Renzong Hu, Min Zhu. Electrolyte modulation strategies towards cathode-electrolyte interphase engineering in subzero-temperature lithium-ion batteries[J]. Review of Materials Research, 2025 , 1 (1) : 100012 - . DOI: 10.1016/j.revmat.2025.100012
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  • National Natural Science Foundation of China(52471227; 52231009; 52404322)
  • Guangdong Basic and Applied Basic Research Foundation(2023B1515040011)
  • Fundamental Research Funds for the Central Universities(2023ZYGXZR105)
  • Open Research Fund Program of Hunan Mine Carbon Sequestration and Sink Enhancement Engineering Technology Research Center(2024KSGTZH01)
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Year 2025 volume 1 Issue 1
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Article Info
doi: 10.1016/j.revmat.2025.100012
  • Receive Date：2025-03-21
  • Online Date：2026-06-10
  • Published：2025-04-07
Article Data
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History
  • Received：2025-03-21
  • Revised：2025-04-05
  • Accepted：2025-04-05
Funding
National Natural Science Foundation of China(52471227; 52231009; 52404322)
Guangdong Basic and Applied Basic Research Foundation(2023B1515040011)
Fundamental Research Funds for the Central Universities(2023ZYGXZR105)
Open Research Fund Program of Hunan Mine Carbon Sequestration and Sink Enhancement Engineering Technology Research Center(2024KSGTZH01)
Affiliations
    School of Materials Science and Engineering, Guangdong Provincial Key Laboratory of Advanced Energy Storage Materials, South China University of Technology, Guangzhou, 510640, China

Corresponding:

* E-mail address: (R. Hu).
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小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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