Article(id=1236334632279535942, tenantId=1146029695717560320, journalId=1235980550691926019, issueId=1236334630450819368, articleNumber=null, orderNo=null, doi=10.3969/j.issn.0253-6099.2023.06.032, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1687881600000, receivedDateStr=2023-06-28, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1772694746321, onlineDateStr=2026-03-05, pubDate=1701360000000, pubDateStr=2023-12-01, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1772694746321, onlineIssueDateStr=2026-03-05, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1772694746321, creator=13701087609, updateTime=1772694746321, updator=13701087609, issue=Issue{id=1236334630450819368, tenantId=1146029695717560320, journalId=1235980550691926019, year='2023', volume='43', issue='6', pageStart='1', pageEnd='183', issueExtLink='null', onlineDate='null', pubDate='null', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1772694745886, creator=13701087609, updateTime=1772694896382, updator=13701087609, preIssue=null, nextIssue=null, ext={EN=IssueExt(id=1236335261735506524, tenantId=1146029695717560320, journalId=1235980550691926019, issueId=1236334630450819368, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1236335261735506525, tenantId=1146029695717560320, journalId=1235980550691926019, issueId=1236334630450819368, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null}, startPage=148, endPage=152, ext={EN=ArticleExt(id=1236334632615080278, articleId=1236334632279535942, tenantId=1146029695717560320, journalId=1235980550691926019, language=EN, title=Electrochemical Performance of Dual-Layer Carbon-Coated SiO_x Anode Materials, columnId=1236276108207902848, journalTitle=Mining and Metallurgical Engineering, columnName=MATERIALS, runingTitle=null, highlight=null, articleAbstract=

To address the problems of low conductivity and poor cycling performance of silicon oxide as negative electrode material, polyacrylamide (PAM) was adopted as a carbon source for the first carbon coating, and the methane-acetylene mixture was used as a gas-phase carbon source for the second coating by chemical vapor deposition to prepare nitrogen-containing double-layer carbon-coated silicon oxide anode materials (SiO_x@ DC-N). Compared with pure gas-phase coated (SiO_x@ GC) and pure liquid-phase coated (SiO_x@ LC) silicon oxide anode material, SiO_x@ DC-N exhibits excellent rate performance and cycling stability, showing that the specific capacity is 850.1 mAh/g at a current density of 4C (1C=1 500 mA/g). The 18650 cylindrical batteries prepared by using a mixed graphite in a ratio of 5∶95 can have a capacity retention rate of 92.70% after 700 cycles of charging and discharging at a current density of 1C.

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为了解决氧化亚硅负极材料导电率低及循环性能差的问题，以聚丙烯酰胺（PAM）为液相碳源进行一次碳包覆，再通过化学气相沉积以甲烷混乙炔为气相碳源进行二次包覆，制备了具有含氮碳层的双层包覆氧化亚硅负极材料（SiO_x@ DC-N）。与纯气相包覆（SiO_x@ GC）以及纯液相包覆（SiO_x@ LC）的氧化亚硅负极材料相比，SiO_x@ DC-N展现出优异的倍率性能与循环性能，在4C（1C=1 500 mA/g）的电流密度下比容量达850.1 mAh/g，以5∶95混合石墨后制成18650圆柱电池，其在电流密度1C充放电700圈循环后容量保持率仍有92.70%。

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梁帆（1994—），男，湖南长沙人，硕士研究生，主要研究方向为高倍率性能锂离子硅基负极材料。

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梁帆（1994—），男，湖南长沙人，硕士研究生，主要研究方向为高倍率性能锂离子硅基负极材料。

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