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A₂B₇-type La_xY_3-xNi_9.7Mn_0.5Al_0.3 (x=0.2, 0.4, 0.6, 0.8, 1.0) hydrogen storage alloys with different La/Y ratios were prepared by vacuum melting. The effect of partial substitution of La by Y element on the structure and properties of the alloy was systematically investigated by using XRD, SEM, gas-phase PCT curves and electrochemical charge-discharge cycle curves. The experiment results show that the prepared alloy has Ce₂Ni₇ as its main phase and contains a small amount of Gd₂Co₇, PuNi₃ and LaNi₅ phases. The abundance of main Ce₂Ni₇ phase increases gradually with the increase of La/Y ratio. When the La/Y ratio is 1∶2, the LaY₂Ni_9.7Mn_0.5Al_0.3 alloy has the maximum hydrogen absorption capacity of 1.317%. After 150 charge-discharge cycles, the alloy can have its highest capacity retention rate at 54.2%.

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采用真空熔炼法制备了不同La/Y比的A₂B₇型La_xY_3-xNi_9.7Mn_0.5Al_0.3（x=0.2，0.4，0.6，0.8，1.0）储氢合金。通过XRD、SEM、气相PCT曲线和电化学充放电循环曲线测试等方法，系统研究了A侧Y元素部分替代La元素对合金相结构和合金性能的影响。结果表明，制备的合金主相为Ce₂Ni₇相，同时还含有少量Gd₂Co₇相、PuNi₃相和LaNi₅相。主相Ce₂Ni₇相丰度随着La/Y比增加而逐渐增大，当La/Y比为1∶2时，LaY₂Ni_9.7Mn_0.5Al_0.3合金吸氢量最大，为1.317%。经过150次充放电循环，LaY₂Ni_9.7Mn_0.5Al_0.3合金容量保持率最高，为54.2%。

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刘雯雯（1989—），女，江西赣州人，硕士，工程师，主要研究方向为储氢新能源、二次资源回收利用。

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刘雯雯（1989—），女，江西赣州人，硕士，工程师，主要研究方向为储氢新能源、二次资源回收利用。

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