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The heavy metal copper (Cu) in acid mine drainage (AMD) is an essential element for organisms but potentially toxic. To control its environmental impact, it is necessary to investigate the factors that influence Cu migration in AMD-sediment interfaces. This study investigated the isotopic composition and fractionation characteristics of Cu in AMD systems from three different mining areas in central China. By coupling these isotopic signatures with detailed physicochemical analyses, we elucidated the key factors and mechanisms controlling Cu adsorption and migration. The results revealed that the Cu isotope fractionation between solutions and sediments in the Dingjiashan gold-copper-sulfur mining area, the Guanchao lead-zinc mining area, and the Qiaolichong polymetallic mining area ranged from (0.3±0.01)‰ to (1.5±0.07)‰, (0.61±0.01)‰, and (1.03±0.02)‰, respectively. This indicates that Cu isotope fractionation in AMD systems varies across mining areas and at different locations within the same mining area. The trends in the primary Cu species in sediments are consistent with those in AMD systems, and exhibit a clear pattern: as sediment Fe-oxide content and the proportion of Fe-/Mn-oxide-bound Cu increase, the isotopic fractionation magnitude decreases; conversely, elevated sulfur/organic matters and a larger fraction of organic- sulfide-bound Cu amplify the fractionation scale, confirming that mineral adsorption and organic-sulfur complexation are the key factors governing Cu mobility and transformation in AMD systems. These results suggest that the characteristics of Cu stable isotope fractionation may serve as a potential tool to explore the key factors controlling Cu migration in AMD systems across different mining areas.

, authors=De-hong LIU¹, Kai-wen CAO^{1, 2}, Wen LIAO³, Dong-mei HOU², Song-xiong ZHONG^{1, *}, authorsList=De-hong LIU, Kai-wen CAO, Wen LIAO, Dong-mei HOU, Song-xiong ZHONG, authorCompany=null, correspAuthors=Song-xiong ZHONG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314923081840296316, articleId=1314923081324396922, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=矿区酸性矿山废水-沉积物界面铜同位素分馏与转化, columnId=1234106388268503686, journalTitle=中国环境科学, columnName=环境生态, runingTitle=null, highlight=null, articleAbstract=

本文研究了华中地区3个不同类型矿区的酸性矿山废水（AMD）体系溶液-沉积物界面Cu同位素组成及分馏特征，结合理化指标探讨影响Cu吸附和迁移的因素及机制．结果发现，丁家山金铜硫矿区、观巢铅锌矿区和桥里冲多金属矿区溶液和沉积物之间Cu同位素分馏值分别为（0.3±0.01）‰~（1.5±0.07）‰、（0.61±0.01）‰和（1.03±0.02）‰，表明不同种类矿区及同一矿区不同点位AMD体系Cu同位素分馏具有差异，且呈现沉积物铁氧化物含量升高，铁锰氧化物结合态比例增大，分馏尺度降低；硫/有机质含量升高，有机-硫化物结合态比例增大，分馏尺度放大的规律，证实矿物吸附与有机硫络合是控制Cu在AMD体系中迁移转化的关键因子．Cu稳定同位素分馏特征可为探究制约不同矿区的AMD体系中Cu迁移的关键因子提供潜在手段．

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刘德洪（1990-），男，广东紫金人，工程师，硕士，主要从事土壤污染控制与修复和农用地安全利用研究．发表论文9篇．ldehong138@163.com.

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刘德洪（1990-），男，广东紫金人，工程师，硕士，主要从事土壤污染控制与修复和农用地安全利用研究．发表论文9篇．ldehong138@163.com.

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