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Acidic mine drainage (AMD) containing high concentrations of heavy metal ions such as Fe²⁺ and Mn²⁺ was treated by a freezing method utilizing the purification effect of ice crystals. The process parameters for removing Fe²⁺ and Mn²⁺ from simulated AMD via the freezing method were optimized through single-factor and orthogonal experiments, and the optimal conditions were determined (for Fe²⁺: freezing temperature of -12℃, initial concentration of 0.9mg/L, freezing radius of 4.25cm; for Mn²⁺: freezing temperature of -6℃, initial concentration of 1.2mg/L, freezing radius of 5.00cm). The optimized process was then applied to treat actual AMD. The results showed that the removal rates of Fe²⁺ and Mn²⁺ from the actual AMD reached 60% and 59%, respectively, which confirmed the effectiveness of the technology. Furthermore, barley seeds and seedlings were used as model plants to evaluate the phytotoxicity of the AMD before and after treatment. The results indicated that, compared with the untreated AMD, the treated AMD did not inhibit the germination of barley seeds or the growth of barley seedlings. This study confirmed that the freezing method can not only effectively remove heavy metal pollutants from AMD but also significantly reduce its biotoxicity.

, authors=Yue WANG¹, Rong-yu DUAN², Nan SANG^{1, 2}, Guang-ke LI^{2, *}, authorsList=Yue WANG, Rong-yu DUAN, Nan SANG, Guang-ke LI, authorCompany=null, correspAuthors=Guang-ke LI, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314923023073894832, articleId=1314923022537023918, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=煤矿矿井水中Fe²⁺、Mn²⁺在冷冻条件下的迁移规律及植物毒性, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

含有高浓度的Fe²⁺、Mn²⁺等重金属离子的酸性煤矿矿井水（AMD）利用冰晶净化效应的冷冻法来处理．AMD通过单因素与正交实验，优化了冷冻法去除模拟AMD中Fe²⁺与Mn²⁺的工艺参数，并确定了其最佳条件（Fe²⁺：冷冻温度为-12℃、初始浓度为0.9mg/L、冷冻半径为4.25cm；Mn²⁺：冷冻温度-6℃、初始浓度1.2mg/L、冷冻半径5.00cm），将优化工艺应用于实际AMD处理．结果表明，实际AMD中Fe²⁺和Mn²⁺的去除率分别达到60%和59%，证实了该技术的有效性．此外，我们使用大麦种子和幼苗作为模型植物，对处理前后AMD的植物毒性进行了评估．结果表明，与未处理的AMD相比，处理后的AMD未抑制大麦种子的发芽和大麦幼苗的生长．本研究证实，冷冻法不仅能有效去除AMD中的重金属污染物，还能显著消减其生物毒性．

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王悦（1992-），女，山西清徐人，副教授，博士，主要研究方向为环境与生态毒理学．发表论文10余篇.

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王悦（1992-），女，山西清徐人，副教授，博士，主要研究方向为环境与生态毒理学．发表论文10余篇.

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