Article(id=1314922173400183452, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314922077824578469, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1752508800000, receivedDateStr=2025-07-15, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791431476210, onlineDateStr=2026-10-08, pubDate=1771516800000, pubDateStr=2026-02-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791431476210, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791431476210, creator=13701087609, updateTime=1791431476210, updator=13701087609, issue=Issue{id=1314922077824578469, tenantId=1146029695717560320, journalId=1234093305789726721, year='2026', volume='46', issue='2', pageStart='593', pageEnd='1184', issueExtLink='null', onlineDate='null', pubDate='1771516800000', pubDateStr='2026-02-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791431453424, creator='13701087609', updateTime=1791431520751, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314922360277398376, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314922077824578469, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314922360277398377, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314922077824578469, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=785, endPage=796, ext={EN=ArticleExt(id=1314922173609898653, articleId=1314922173400183452, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Degradation mechanism of Azo dye ARG by VUV/Fe²⁺/Ox Fenton-like system, columnId=1234106386360103680, journalTitle=China Environmental Science, columnName=Water Pollution Control, runingTitle=null, highlight=null, articleAbstract=

A novel exogenous oxidant-free Fenton-like reaction system based on vacuum ultraviolet (VUV)/Fe²⁺/oxalic acid (Ox) was constructed and applied to the degradation of azo dye Acid Red G (ARG). Results indicated that this system enabled the dynamic release of H₂O₂, which further reacts with Fe²⁺ to trigger Fenton-like reactions, and maintained high reactivity over a wide pH range. Experimental data showed that under the conditions of initial ARG concentration of 60mg/L, Fe²⁺ concentration of 0.06mmol/L and Ox concentration of 0.7mmol/L, the ARG removal efficiency by the VUV/Fe²⁺/Ox system reached 96.2% within 5min, and the degradation process fitted well with the pseudo-first-order kinetic model. With the increase of initial solution pH, the ARG removal efficiency exhibited a decreasing trend. Even at pH=7, the first-order rate constant k still reached 0.454min^-1, which was 69.6% of that at pH=3, demonstrating that the system could retain high reactivity under neutral conditions. During the initial 5min of the reaction, the concentration of H₂O₂ in the system gradually increased to a maximum of 62.5μmol/L, then decreased slowly and remained at 51.8μmol/L at 9min. Free radical trapping experiments and the electron paramagnetic resonance (EPR) measurements collectively confirmed that hydroxyl radicals (·OH) and superoxide radicals (O₂^·-) were the dominant reactive oxygen species (ROS). In addition, common inorganic anions in aqueous environments (HCO₃^-, NO₃^-, Cl^-, SO₄^2-) all inhibited ARG degradation to varying degrees. Analysis via UV-visible absorption spectroscopy and liquid chromatography-mass spectrometry (LC-MS) revealed that ROS generated during the degradation process attacked the azo bonds and benzene ring structures in the ARG molecule, thereby achieving decolorization and removal of the dye.

, authors=Kun WANG¹, Wei CHEN¹, Yu-chao TANG¹, Kang-ping CUI², Chang-nian WU¹, Xian-sheng ZHU¹, Hai-xiang SUN¹, Xian-huai HUANG^{1, *}, authorsList=Kun WANG, Wei CHEN, Yu-chao TANG, Kang-ping CUI, Chang-nian WU, Xian-sheng ZHU, Hai-xiang SUN, Xian-huai HUANG, authorCompany=null, correspAuthors=Xian-huai HUANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314922175459586719, articleId=1314922173400183452, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=VUV/Fe²⁺/Ox类芬顿体系对偶氮染料酸性红G的降解机理研究, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

构建了一种基于真空紫外（VUV）/Fe²⁺/草酸（Ox）的新型无外源氧化剂类芬顿反应体系，并将其应用于偶氮染料酸性红G（ARG）的降解研究．结果表明，该体系可实现H₂O₂的动态释放，进而与Fe²⁺形成类芬顿反应，且在较宽pH值范围内均能保持高反应活性．结果表明：在ARG初始质量浓度为60mg/L、Fe²⁺与Ox浓度分别为0.06和0.7mmol/L的条件下，VUV/Fe²⁺/Ox体系对ARG的去除率在5min内即可达到96.2%，其降解过程符合准一级动力学模型．随着溶液初始pH值的升高，ARG去除率呈下降趋势，在pH=7时，一级速率常数k值仍可达0.454min^-1，为pH=3时的69.6%，表明该体系在中性条件下仍能维持较高反应活性．反应初始5min内，体系中H₂O₂浓度逐渐上升至最高62.5μmol/L，随后缓慢下降，至9min时仍保持在51.8μmol/L．自由基捕获实验与EPR检测结果共同证实，羟基自由基（·OH）和超氧自由基（O₂^·-）是该体系中的主要活性氧化物种．此外，水环境中常见的无机阴离子（HCO₃^-、NO₃^-、Cl^-、SO₄^2-）均会对ARG降解产生不同程度的抑制作用．通过紫外可见吸收光谱及液相色谱-质谱联用（LC-MS）分析可知，降解过程中生成的活性氧（ROS）通过攻击ARG分子中的偶氮键和苯环结构，实现了染料的脱色与去除．

, authors=王坤¹, 陈伟¹, 唐玉朝¹, 崔康平², 伍昌年¹, 朱先胜¹, 孙海翔¹, 黄显怀^{1, *}, authorsList=王坤, 陈伟, 唐玉朝, 崔康平, 伍昌年, 朱先胜, 孙海翔, 黄显怀, authorCompany=null, correspAuthors=黄显怀, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=BaSqwFJ2hU4/WvqgTX6g1A==, magXml=kcAtmqWfE29sg5GUsaAXSA==, pdfUrl=null, pdf=Mf/UZZxXTYZVqAeYZS924w==, pdfFileSize=2679001, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=YkLKErnatY/juxyrUQEjIA==, mapNumber=null, fund=null)}, authors=[Author(id=1314922175849657000, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314922173400183452, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=wangkun@ahjzu.edu.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1314922175933543082, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314922173400183452, authorId=1314922175849657000, language=EN, stringName=Kun WANG, firstName=Kun, middleName=null, lastName=WANG, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.Anhui Provincial Key Laboratory of Environmental Pollution Control and Resource Reuse, Anhui Jianzhu University, Hefei 230601, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314922176000651947, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314922173400183452, authorId=1314922175849657000, language=CN, stringName=王坤, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.安徽建筑大学，环境污染控制与资源化安徽省重点实验室，安徽 合肥 230601, bio={"content":"

王坤（1980-），男，安徽亳州人，副教授，硕士，主要从事水处理理论与技术研究．发表论文数量50余篇．wangkun@ahjzu.edu.cn.

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王坤（1980-），男，安徽亳州人，副教授，硕士，主要从事水处理理论与技术研究．发表论文数量50余篇．wangkun@ahjzu.edu.cn.

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