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This study systematically investigated the adsorption mechanisms of heavy metal Tl by layered double hydroxide (LDH). For the first time, CaAl-LDH was applied to immobilize Tl in three typical Tl-contaminated soils-red soil, yellow soil, and black soil. The immobilization effectiveness was assessed based on the ecological and health risks associated with soil Tl, using the Tessier sequential extraction method and an in vitro test method. Results showed that the active sites on CaAl-LDH surface were uniformly distributed, with Tl⁺ adsorption primarily following monolayer adsorption behavior, consistent with the Langmuir model. The key adsorption mechanisms included: (1) synergistic adsorption induced by anion exchange in LDH interlayers; (2) surface adsorption of Tl⁺ on LDH lamella surfaces and edges; and (3) complexation with Tl⁺ following the release of functional groups from the LDH surface. At the relative optimal application rate (5% of soil mass), CaAl-LDH significantly reduced the mobility factor of soil Tl and the relevant ecological risk and crop uptake risk, with an average decrease of 24.1%. Also, it significantly lowered the bioaccessibility of soil Tl and the relevant human health risk, with an average decrease of 30.5% in the gastric phase and 21.3% in the small intestinal phase. These findings provide a scientific foundation and practical reference for developing immobilizing remediation agents for Tl-contaminated soils, thereby contributing to improved soil environmental quality and human health protection.

, authors=Xiao-chen CHEN¹, Qian GUAN¹, Hao-chen FANG¹, Jian-ying YU², Jian-yu ZHANG³, Xue-ping HAN⁴, Teng-fei GUO², Qi-jia ZHANG², Xu-chuan ZHANG⁵, Kai-qin XU¹, Nan WEI^{6, *}, authorsList=Xiao-chen CHEN, Qian GUAN, Hao-chen FANG, Jian-ying YU, Jian-yu ZHANG, Xue-ping HAN, Teng-fei GUO, Qi-jia ZHANG, Xu-chuan ZHANG, Kai-qin XU, Nan WEI, authorCompany=null, correspAuthors=Nan WEI, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314918578592247900, articleId=1314918578105708634, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=钙铝基层状双金属氢氧化物对土壤中铊的钝化修复及风险评估, columnId=1234106394572550190, journalTitle=中国环境科学, columnName=土壤污染与控制, runingTitle=null, highlight=null, articleAbstract=

系统探究了层状双金属氢氧化物（LDH）对铊（Tl）的吸附机理．首次应用CaAl-LDH对Tl污染的红壤、黄壤和黑土进行钝化修复，并使用Tessier连续提取法和in vitro试验法，从土壤Tl的生态风险和健康风险角度对修复成效进行评估．结果表明，CaAl-LDH表面活性位点分布均匀，对Tl⁺吸附方式以符合Langmuir模型的单分子层为主，吸附机理包括：LDH层间阴离子交换主导的协同吸附反应；LDH层板表面和边缘部分对Tl⁺的表面吸附；LDH表面官能团释放后与Tl⁺形成络合物．在土壤质量5%的相对最优施用量下，CaAl-LDH可显著降低土壤Tl的活性系数及其所反映的生态风险及作物吸收风险，平均降幅达24.1%；亦可显著降低土壤Tl在胃和小肠阶段的生物可给性及其所反映的人体健康风险，平均降幅达30.5%和21.3%．相关成果将为Tl污染土壤钝化修复剂的研发提供科学依据和有价值的参考，对土壤环境质量改善和人群健康质量保障做出贡献．

, authors=陈晓晨¹, 官倩¹, 房灏宸¹, 余健英², 张剑宇³, 韩雪平⁴, 郭腾飞², 张起佳², 张旭钏⁵, 徐开钦¹, 魏楠^{6, *}, authorsList=陈晓晨, 官倩, 房灏宸, 余健英, 张剑宇, 韩雪平, 郭腾飞, 张起佳, 张旭钏, 徐开钦, 魏楠, authorCompany=null, correspAuthors=魏楠, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=LebrQpjG8uxYZsLw2SA+sQ==, magXml=WOXpg0nDXvbV+EjYFuKUKw==, pdfUrl=null, pdf=HQ0eb8B5zkzTpHXu2M9kow==, pdfFileSize=1827615, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=wy7fF3YbKZovJdaNlk2xbQ==, mapNumber=null, fund=null)}, authors=[Author(id=1314918579372388464, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918578105708634, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=chenxiaochen@fzu.edu.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1314918579477246066, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918578105708634, authorId=1314918579372388464, language=EN, stringName=Xiao-chen CHEN, firstName=Xiao-chen, middleName=null, lastName=CHEN, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1. Innovation Center for Soil Remediation and Restoration Technologies, College of Environment and Safety Engineering, Fuzhou University, Fuzhou 350108, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314918579561132147, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918578105708634, authorId=1314918579372388464, language=CN, stringName=陈晓晨, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.福州大学环境与安全工程学院，福州大学冶金地质土壤综合修复治理工程技术研发中心，福建 福州 350108, bio={"content":"

陈晓晨（1984-），男，福建福州人，教授，博士，主要从事土壤污染风险评价及其控制技术研究．发表论文80余篇．chenxiaochen@fzu.edu.cn.

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陈晓晨（1984-），男，福建福州人，教授，博士，主要从事土壤污染风险评价及其控制技术研究．发表论文80余篇．chenxiaochen@fzu.edu.cn.

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