Article(id=1314918437030298202, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918356222829028, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1744560000000, receivedDateStr=2025-04-14, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791430585390, onlineDateStr=2026-10-08, pubDate=1763568000000, pubDateStr=2025-11-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791430585390, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791430585390, creator=13701087609, updateTime=1791430585390, updator=13701087609, issue=Issue{id=1314918356222829028, tenantId=1146029695717560320, journalId=1234093305789726721, year='2025', volume='45', issue='11', pageStart='5921', pageEnd='6512', issueExtLink='null', onlineDate='null', pubDate='1763568000000', pubDateStr='2025-11-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791430566125, creator='13701087609', updateTime=1791431596967, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314922679942078535, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918356222829028, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314922679942078536, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918356222829028, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=5980, endPage=5991, ext={EN=ArticleExt(id=1314918437256790619, articleId=1314918437030298202, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Characteristics of ozone pollution andphotochemical reactivity of VOCs in Hong Kong during autumn, columnId=1234106386020365051, journalTitle=China Environmental Science, columnName=Air Pollution Control, runingTitle=null, highlight=null, articleAbstract=

To investigate the pollution characteristics and formation mechanisms of ozone episodes in the Guangdong-Hong Kong-Macao Greater Bay Area (GBA) during autumn, ozone (O₃) concentrations and emission characteristics of volatile organic compounds (VOCs) were analyzed during three ozone episodesin Hong Kong.Observational data combined withobservation-based model(OBM) and the empirical kinetics modeling approach (EKMA) wasemployed to assess the impact of VOCs on O₃ formation sensitivity mechanisms and contribution to O₃ formation. The peak O₃ values recorded during the three episodes were 382.65, 302.67, and 301.76μg/m³, with corresponding concentrations of VOCs measuring 23.6×10^-9, 25.4×10^-9, and 32.1×10^-9, respectively. Oxygenated volatile organic compounds (OVOCs)were the most dominant of the observed species, with methanol, formaldehyde, and acetone being the three most prevalent by volume fraction. EKMA curves confirmedthat the nonlinear relationship among O₃-nitrogen oxides (NO_x)-VOCs depends ontheir instantaneous concentrations. The morning hours were characterized as VOC-limited regimes, while the afternoon hourswerethe transitional regime. The photochemical initial concentration (PIC) was 8.2×10^-9 higher than measured concentration, indicating that neglecting photochemically VOCs consumption may lead to an underestimation of the contribution of local VOCs photochemical reactions to O₃ formation. Furthermore, differences in the types and concentrations of O₃ precursors and radicals resulted in varying O₃ formation and loss rates, confirming the promoting effect of VOCs as precursors on net O₃ formation. Based on O₃ formation potential (OFP) and OH loss rate (L_OH) calculations, the VOCs with the highest contribution to the OFP were OVOCs (68.9%), alkenes (17.5%), and aromatics (13.6%). Formaldehyde and isoprene were the dominant species driving O₃ formation and hydroxyl radical (OH) consumption in the autumn in Hong Kong, respectively. The OFP of formaldehyde ranged from 42.1 to 73.1μg/m³, and the L_OH of isoprene varied from 1.35 to 2.12s^-1. Backward trajectory cluster analysis revealed that Hong Kong’s background site was primarily influenced by three air mass types driven by northeasterly winds: long-range transport (52%), short-range transport (28%), and local sources (20%). Results reveal that the photochemical reactions of VOCs, the response characteristics of different VOCs to the sensitivity of O₃ formation, and the synergistic effect of regional transport and local emissions have a significant impact on the O₃ pollution in Hong Kong during autumn.

, authors=Yan TAN¹, Yu-jia ZHANG¹, Yi-yang RONG¹, Yi-fan WANG¹, Shun-cheng LEE^{2, *}, Zi-zhen MA¹, Ting LIU¹, Hua-wei ZHANG¹, Zhi-fei ZHAO³, Yong-tao ZHANG³, authorsList=Yan TAN, Yu-jia ZHANG, Yi-yang RONG, Yi-fan WANG, Shun-cheng LEE, Zi-zhen MA, Ting LIU, Hua-wei ZHANG, Zhi-fei ZHAO, Yong-tao ZHANG, authorCompany=null, correspAuthors=Shun-cheng LEE, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314918437558780509, articleId=1314918437030298202, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=香港地区秋季臭氧污染特征及VOCs光化学反应的研究, columnId=1234106388364981004, journalTitle=中国环境科学, columnName=大气污染与控制, runingTitle=null, highlight=null, articleAbstract=

为探究粤港澳大湾区秋季高浓度臭氧（O₃）事件的污染特征及形成机制,本研究综合观测数据,利用基于观测的模型（OBM）和经验动力学方法（EKMA）,以香港为例,分析该地区3次高浓度O₃污染事件中O₃浓度及前体物挥发性有机物（VOCs）的排放特征,评估VOCs对O₃生成敏感性机制的影响和对O₃生成的贡献.结果表明:在3次事件中,O₃峰值分别为382.65、302.67和301.76μg/m³,对应的VOCs浓度均值分别为23.6×10^-9、25.4×10^-9和32.1×10^-9.含氧挥发性有机物（OVOCs）在观测物种中占据主导地位,其中甲醇、甲醛和丙酮是体积分数前三的VOCs.EKMA曲线证实O₃-氮氧化物（NO_x）-VOCs之间的非线性关系取决于NO_x与VOCs的即时浓度,观测期间上午时段为VOCs控制区,下午时段为NO_x-VOCs协同控制区.光化学初始浓度（PIC）较实测值高8.2×10^-9,表明忽视实际消耗的VOCs会低估本地VOCs光化学反应对O₃生成的贡献.此外,由于O₃前体物和自由基的种类及浓度的差异,导致了O₃生成和损耗速率的不同,证实VOCs作为前体物对O₃净生成过程的促进效应.通过对臭氧生成潜势（OFP）与羟基消耗速率（L_OH）的计算可知,对OFP贡献率最高的VOCs组分依次为OVOCs（68.9%）,烯烃（17.5%）和芳香烃（13.6%）.甲醛和异戊二烯分别是香港秋季驱动O₃生成以及羟基（OH）消耗的优势物种,其中甲醛的OFP为42.1~73.1μg/m³,异戊二烯的L_OH为1.35~2.12s^-1.基于后向轨迹聚类分析,香港背景点主要受东北风驱动的三类气团影响:长距离输送（52%）、短距离输送（28%）和本地源（20%）.研究结果揭示本地VOCs光化学反应、不同VOCs对O₃生成敏感性的响应特征以及区域传输与本地排放的协同作用对香港秋季O₃污染具有重要影响.

, authors=谈琰¹, 张玉佳¹, 荣毅阳¹, 王一帆¹, 李顺诚^{2, *}, 马子轸¹, 刘亭¹, 张华伟¹, 赵志飞³, 张永涛³, authorsList=谈琰, 张玉佳, 荣毅阳, 王一帆, 李顺诚, 马子轸, 刘亭, 张华伟, 赵志飞, 张永涛, authorCompany=null, correspAuthors=李顺诚, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=kKt6X5RveUlwQ+noFtEOgg==, magXml=usqKRkn83+0i0J9rGa2c0A==, pdfUrl=null, pdf=8wZeIReUa/cHW79j89gn6w==, pdfFileSize=2627848, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=TwI3BKlMSyi3pIBJCygVTg==, mapNumber=null, fund=null)}, authors=[Author(id=1314918439681098345, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918437030298202, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=tanyan@qut.edu.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1314918439773373035, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918437030298202, authorId=1314918439681098345, language=EN, stringName=Yan TAN, firstName=Yan, middleName=null, lastName=TAN, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.School of Environmental and Municipal Engineering, Qingdao University of Technology, Qingdao 266520, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314918439886619244, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918437030298202, authorId=1314918439681098345, language=CN, stringName=谈琰, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.青岛理工大学环境与市政工程学院，山东 青岛 266520, bio={"content":"

谈琰（1992-），女，副教授，博士，主要研究方向为大气中挥发性有机物特征的研究．发表论文30余篇．tanyan@qut.edu.cn.

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谈琰（1992-），女，副教授，博士，主要研究方向为大气中挥发性有机物特征的研究．发表论文30余篇．tanyan@qut.edu.cn.

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