Article(id=1314918401835885382, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918356222829028, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1745424000000, receivedDateStr=2025-04-24, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791430577000, onlineDateStr=2026-10-08, pubDate=1763568000000, pubDateStr=2025-11-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791430577000, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791430577000, creator=13701087609, updateTime=1791430577000, updator=13701087609, issue=Issue{id=1314918356222829028, tenantId=1146029695717560320, journalId=1234093305789726721, year='2025', volume='45', issue='11', pageStart='5921', pageEnd='6512', issueExtLink='null', onlineDate='null', pubDate='1763568000000', pubDateStr='2025-11-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791430566125, creator='13701087609', updateTime=1791431596967, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314922679942078535, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918356222829028, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314922679942078536, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918356222829028, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=6091, endPage=6100, ext={EN=ArticleExt(id=1314918403446498119, articleId=1314918401835885382, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Efficient adsorption behavior and mechanism of C7HFPO-TA in water by fluorinated defective covalent triazine frameworks, columnId=1234106386360103680, journalTitle=China Environmental Science, columnName=Water Pollution Control, runingTitle=null, highlight=null, articleAbstract=

In this study, fluorine-defective covalent triazine frameworks (CTFs) were designed and synthesized to improve adsorption performance for per-and polyfluoroalkyl substances (PFAS). Compared with pristine CTFs, the fluorine-defective CTFs exhibited a 55% increase in adsorption capacity. A systematic evaluation of different particle sizes revealed that CTF-F10 (246.421mg/g) achieved a 59% higher capacity than CTF-F595 (154.403mg/g). These results demonstrate that reducing the adsorbent particle size not only substantially increases the equilibrium adsorption capacity, but also accelerates the adsorption rate. At pH 2, CTF-F10 achieved a C7HFPO-TA removal efficiency of 89.55%, significantly higher than that at pH 6 (50.15%) and pH 10 (26.35%). The presence of NaCl or fulvic acid (FA) reduced removal efficiency by about 20%. DFT calculations indicated that the adsorption of C7HFPO-TA onto fluorine-defective CTFs is primarily governed by electrostatic and fluorophilic interactions. Regeneration experiments also excellent recyclability and reusability of powdered CTFs. This work establishes a novel design strategy for fluorine-defective CTFs for PFAS removal from water and provides a first comparative evaluation of the particle size effects on C7HFPO-TA adsorption, providing scientific and technical guidance for mitigating PFAS contamination in aquatic environments.

, authors=Zhi-cheng ZHANG^{1, 2}, Rui LI², Guo-tao XIAO^{1, 2}, De-yan LI¹, Ming-chao ZHANG¹, Dong-hai ZHU¹, Wei WANG^{1, 2, *}, authorsList=Zhi-cheng ZHANG, Rui LI, Guo-tao XIAO, De-yan LI, Ming-chao ZHANG, Dong-hai ZHU, Wei WANG, authorCompany=null, correspAuthors=Wei WANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314918403807208264, articleId=1314918401835885382, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=含氟缺陷共价三嗪框架高效吸附水中全氟-2,5-二甲基-3,6-二氧杂庚酸的特性和机理, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

本研究设计并成功制备了含氟缺陷共价三嗪框架（CTFs）,相较于原始CTFs,含氟缺陷CTFs吸附量提升了55%,并比较了不同粒径CTFs的吸附效果,相较于CTF-F595（154.403mg/g）, CTF-F10（246.421mg/g）提升了59%.结果表明,吸附剂粒径的减小不仅能显著提升吸附剂对于吸附质的饱和吸附量,而且可以极快地提升吸附剂对于吸附质的吸附速率.研究发现,在pH=2时, CTF-F10对C7HFPO-TA的去除率（89.55%）显著高于pH=6（50.15%）和pH=10（26.35%）.而NaCl和FA对CTF-F10吸附C7HFPO-TA效果的影响大致相同,两者的存在使去除率下降了约20%.DFT计算结果表明,含氟缺陷CTFs对C7HFPO-TA的吸附以静电作用和亲氟作用为主.吸附再生实验证明粉末态CTFs具有良好的再生性能和循环使用性能.本研究为设计含氟缺陷CTFs吸附水中PFAS提供了新的思路,并创新性比较CTFs不同粒径对C7HFPO-TA吸附性能的影响,为水环境中PFAS的削减和去除提供了科学技术指导.

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张芝诚（2001-），男，陕西宝鸡人，青海大学硕士研究生，主要研究方向为水中污染物环境生态修复研究．发表论文2篇．ys240713000066@qhu.edu.cn.

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张芝诚（2001-），男，陕西宝鸡人，青海大学硕士研究生，主要研究方向为水中污染物环境生态修复研究．发表论文2篇．ys240713000066@qhu.edu.cn.

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