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Polyethylene terephthalate (PET) and humic acid (HA), commonly present in water, were selected to represent microfibers and organic foulants, respectively. The interaction forces of each type of foulant with the membrane surface were measured, which combined with the results of the fouling layer structure and the dynamic adsorption behavior of HA on the PET and membrane surface, to unravel the influence mechanism of microfibers on the organic fouling behavior of membranes. The results revealed that the interaction force between PET microfibers and the ultrafiltration membrane surface was more than ten times stronger than that of HA. However, the micrometer-scale size of PET induced a steric hindrance effect, leading to a disordered distribution of microfibers on the membrane surface, which had only a limited impact on the flux of the ultrafiltration membrane. In the PET-HA co-existing systems, strong interactions of PET-HA enabled microfibers to preferentially adsorb HA, effectively decreasing initial-stage membrane fouling rate by reducing the concentration of free HA. However, the dissolved HA could penetrate microfiber interstices under hydrodynamic forces and form a "membrane-HA-PET" gradient fouling layer, making the membrane fouling behavior of the mixed system comparable to that of the single HA system during the stable operation stage.

, authors=Zhuo-wen MA¹, Li FAN¹, Wen-juan ZHANG¹, Jia-lin WAN¹, Rui MIAO^{1, 2, *}, Lei WANG^{1, 2}, authorsList=Zhuo-wen MA, Li FAN, Wen-juan ZHANG, Jia-lin WAN, Rui MIAO, Lei WANG, authorCompany=null, correspAuthors=Rui MIAO, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314918396488155376, articleId=1314918395879981294, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=微纤维对天然有机物超滤膜污染行为影响机制, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

选用水体中普遍存在的聚对苯二甲酸乙二醇酯（PET）和天然有机物（HA）,通过污染物在膜面作用力、污染层结构及HA在膜和微纤维表面的吸附行为分析,解析微纤维对有机物膜污染行为的影响机制.结果发现,PET微纤维与超滤膜面的作用力强度是HA的10倍以上,但其微米级尺寸引发的空间位阻效应导致微纤维无序分散于膜面,对超滤膜通量的影响有限.在PET-HA混合体系中,二者之间较强作用力导致微纤维优先吸附HA,通过降低游离HA浓度而有效减缓运行初期的膜污染速率.但是,溶解态的HA能穿透微纤维间隙,随着运行时间在膜面形成"膜-HA-PET"梯度污染层,使混合体系与单一HA体系在稳定运行阶段的膜污染行为相当.

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马焯文（2000-），男，广西南宁人，西安建筑科技大学硕士研究生，主要研究方向为膜应用及膜污染控制．842586986@qq.com.

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马焯文（2000-），男，广西南宁人，西安建筑科技大学硕士研究生，主要研究方向为膜应用及膜污染控制．842586986@qq.com.

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