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Article(id=1314918264396939456, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918247384834796, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1741017600000, receivedDateStr=2025-03-04, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791430544231, onlineDateStr=2026-10-08, pubDate=1760889600000, pubDateStr=2025-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791430544231, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791430544231, creator=13701087609, updateTime=1791430544231, updator=13701087609, issue=Issue{id=1314918247384834796, tenantId=1146029695717560320, journalId=1234093305789726721, year='2025', volume='45', issue='10', pageStart='5329', pageEnd='5920', issueExtLink='null', onlineDate='null', pubDate='1760889600000', pubDateStr='2025-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791430540175, creator='13701087609', updateTime=1791431660009, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314922944367784036, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918247384834796, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314922944367784037, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314918247384834796, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=5435, endPage=5447, ext={EN=ArticleExt(id=1314918264602460353, articleId=1314918264396939456, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Research progress of SCR denitrification catalysts for copper-based LDHs derivatives, columnId=1234106386020365051, journalTitle=China Environmental Science, columnName=Air Pollution Control, runingTitle=null, highlight=null, articleAbstract=

Copper-based layered double hydroxides (Cu-LDHs) are layered compounds composed of positively charged lamels and interlayer negative anions. With their excellent ion exchange properties, adjustable interlayer structure, unique memory effect, excellent catalytic activity and good thermal stability, they show great application potential in the field of denitrification. In this paper, the application progress of Cu-LDHs derivative catalysts in denitrification technology was reviewed. The types of SCR catalysts for Cu-LDHs derivatives were systematically classified from the perspectives of metal doping, carrier loading and anion regulation. The reaction mechanism of NH3, CO and C3H6 as reducing agents in SCR system of Cu-LDHs derivatives was investigated. In addition, the strengthening strategy of the Cu-LDHs derivative catalyst in the aspects of sulfur resistance, hydrothermal aging resistance and alkali metal poisoning resistance was described in detail, aiming to enhance the stability and durability of the catalyst by comprehensive means. Finally, the future research direction of Cu-LDHs derivatives is prospectively prospected.

, authors=Wei ZHANG1, 2, *, Kai-kai ZHANG1, 2, Quan-bin SONG1, 2, Yan-shan YIN1, 2, Shan CHENG1, 2, Yan-ni XUAN1, 2, Min RUAN1, 2, Tao LIU1, 2, Zhao-yi ZHOU1, 2, Zhi-hao YAO1, 2, Dan-cong LI1, 2, authorsList=Wei ZHANG, Kai-kai ZHANG, Quan-bin SONG, Yan-shan YIN, Shan CHENG, Yan-ni XUAN, Min RUAN, Tao LIU, Zhao-yi ZHOU, Zhi-hao YAO, Dan-cong LI, authorCompany=null, correspAuthors=Wei ZHANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314918265151914178, articleId=1314918264396939456, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=铜基LDHs衍生物SCR脱硝催化剂的研究进展, columnId=1234106388364981004, journalTitle=中国环境科学, columnName=大气污染与控制, runingTitle=null, highlight=null, articleAbstract=

铜基层状双氢氧化物（Cu-LDHs）是一种由正电荷层板和层间负电荷阴离子构成的层状化合物，以其卓越的离子交换性、可调节的层间结构、独特的记忆效应、优异的催化活性和良好的热稳定性，在脱硝领域展现出巨大的应用潜力．因此，本文综述了Cu-LDHs衍生物催化剂在脱硝技术中的应用进展，从金属掺杂、载体负载和阴离子调控等多个角度，对Cu-LDHs衍生物SCR催化剂的类型进行了系统分类．探讨了Cu-LDHs衍生物在SCR系统中NH3、CO和C3H6作为还原剂的反应机制．此外，详细阐述了Cu-LDHs衍生物催化剂在抗硫性能、抗水热老化性能和抗碱金属中毒性能方面的强化策略，旨在通过综合手段增强催化剂的稳定性和耐用性．最后，对Cu-LDHs衍生物的未来研究方向进行了前瞻性展望．

, authors=张巍1, 2, *, 张凯凯1, 2, 宋权斌1, 2, 尹艳山1, 2, 成珊1, 2, 宣艳妮1, 2, 阮敏1, 2, 刘涛1, 2, 周昭仪1, 2, 姚志豪1, 2, 李丹聪1, 2, authorsList=张巍, 张凯凯, 宋权斌, 尹艳山, 成珊, 宣艳妮, 阮敏, 刘涛, 周昭仪, 姚志豪, 李丹聪, authorCompany=null, correspAuthors=张巍, authorNote=

张巍（1974-），男，湖南常德人，副教授，博士，主要从事绿色能源开发利用及大气污染控制过程中环境催化新方法和新技术的研究．发表论文30余篇．.

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* 责任作者，副教授，
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张巍（1974-），男，湖南常德人，副教授，博士，主要从事绿色能源开发利用及大气污染控制过程中环境催化新方法和新技术的研究．发表论文30余篇．.

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张巍（1974-），男，湖南常德人，副教授，博士，主要从事绿色能源开发利用及大气污染控制过程中环境催化新方法和新技术的研究．发表论文30余篇．.

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铜基LDHs衍生物SCR脱硝催化剂的研究进展
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张巍 1, 2, * , 张凯凯 1, 2 , 宋权斌 1, 2 , 尹艳山 1, 2 , 成珊 1, 2 , 宣艳妮 1, 2 , 阮敏 1, 2 , 刘涛 1, 2 , 周昭仪 1, 2 , 姚志豪 1, 2 , 李丹聪 1, 2
中国环境科学 | 大气污染与控制 2025,45(10): 5435-5447
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中国环境科学 |大气污染与控制 2025 , 45 (10) : 5435 -5447
铜基LDHs衍生物SCR脱硝催化剂的研究进展
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张巍（1974-），男，湖南常德人，副教授，博士，主要从事绿色能源开发利用及大气污染控制过程中环境催化新方法和新技术的研究．发表论文30余篇．.

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张巍（1974-），男，湖南常德人，副教授，博士，主要从事绿色能源开发利用及大气污染控制过程中环境催化新方法和新技术的研究．发表论文30余篇．.

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张巍1, 2, * , 张凯凯1, 2, 宋权斌1, 2, 尹艳山1, 2, 成珊1, 2, 宣艳妮1, 2, 阮敏1, 2, 刘涛1, 2, 周昭仪1, 2, 姚志豪1, 2, 李丹聪1, 2
作者信息
  • 1.长沙理工大学能源与动力工程学院，湖南 长沙 410114
  • 2.可再生能源电力技术湖南省重点实验室，湖南 长沙 410114
通讯作者:
* 责任作者，副教授，
作者简介:

张巍（1974-），男，湖南常德人，副教授，博士，主要从事绿色能源开发利用及大气污染控制过程中环境催化新方法和新技术的研究．发表论文30余篇．.

Research progress of SCR denitrification catalysts for copper-based LDHs derivatives
Wei ZHANG1, 2, * , Kai-kai ZHANG1, 2, Quan-bin SONG1, 2, Yan-shan YIN1, 2, Shan CHENG1, 2, Yan-ni XUAN1, 2, Min RUAN1, 2, Tao LIU1, 2, Zhao-yi ZHOU1, 2, Zhi-hao YAO1, 2, Dan-cong LI1, 2
Affiliations
  • 1.School of Energy and Power Engineering, Changsha University of Science and Technology, Changsha 410114, China
  • 2.Renewable Energy Power Technology Key Laboratory of Hunan Province, Changsha 410114, China
出版时间: 2025-10-20
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铜基层状双氢氧化物（Cu-LDHs）是一种由正电荷层板和层间负电荷阴离子构成的层状化合物，以其卓越的离子交换性、可调节的层间结构、独特的记忆效应、优异的催化活性和良好的热稳定性，在脱硝领域展现出巨大的应用潜力．因此，本文综述了Cu-LDHs衍生物催化剂在脱硝技术中的应用进展，从金属掺杂、载体负载和阴离子调控等多个角度，对Cu-LDHs衍生物SCR催化剂的类型进行了系统分类．探讨了Cu-LDHs衍生物在SCR系统中NH3、CO和C3H6作为还原剂的反应机制．此外，详细阐述了Cu-LDHs衍生物催化剂在抗硫性能、抗水热老化性能和抗碱金属中毒性能方面的强化策略，旨在通过综合手段增强催化剂的稳定性和耐用性．最后，对Cu-LDHs衍生物的未来研究方向进行了前瞻性展望．

层状双氢氧化物（LDHs）  /  选择性催化还原（SCR）  /  铜基  /  反应机理  /  抗硫性

Copper-based layered double hydroxides (Cu-LDHs) are layered compounds composed of positively charged lamels and interlayer negative anions. With their excellent ion exchange properties, adjustable interlayer structure, unique memory effect, excellent catalytic activity and good thermal stability, they show great application potential in the field of denitrification. In this paper, the application progress of Cu-LDHs derivative catalysts in denitrification technology was reviewed. The types of SCR catalysts for Cu-LDHs derivatives were systematically classified from the perspectives of metal doping, carrier loading and anion regulation. The reaction mechanism of NH3, CO and C3H6 as reducing agents in SCR system of Cu-LDHs derivatives was investigated. In addition, the strengthening strategy of the Cu-LDHs derivative catalyst in the aspects of sulfur resistance, hydrothermal aging resistance and alkali metal poisoning resistance was described in detail, aiming to enhance the stability and durability of the catalyst by comprehensive means. Finally, the future research direction of Cu-LDHs derivatives is prospectively prospected.

layered double hydroxides (LDHs)  /  selective catalytic reduction (SCR)  /  copper based  /  reaction mechanism  /  sulfur resistance
张巍, 张凯凯, 宋权斌, 尹艳山, 成珊, 宣艳妮, 阮敏, 刘涛, 周昭仪, 姚志豪, 李丹聪. 铜基LDHs衍生物SCR脱硝催化剂的研究进展. 中国环境科学, 2025 , 45 (10) : 5435 -5447 .
Wei ZHANG, Kai-kai ZHANG, Quan-bin SONG, Yan-shan YIN, Shan CHENG, Yan-ni XUAN, Min RUAN, Tao LIU, Zhao-yi ZHOU, Zhi-hao YAO, Dan-cong LI. Research progress of SCR denitrification catalysts for copper-based LDHs derivatives[J]. China Environmental Science, 2025 , 45 (10) : 5435 -5447 .
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  • 国家自然科学基金资助项目(52006016)
  • 湖南省自然科学基金资助项目(2023JJ30047; 2021JJ40573; 2020JJ4098; 2025JJ60890)
  • 湖南省教育厅科学研究重点项目(21A0216)
  • 湖南省教育厅优秀青年项目(202B041; 22B0291)
  • 长沙市自然科学基金资助项目(kq2014104)
  • 长沙理工大学青年教师成长计划项目(2019QJCZ044)
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  • 接收时间：2025-03-04
  • 首发时间：2026-10-08
  • 出版时间：2025-10-20
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  • 收稿日期：2025-03-04
基金
国家自然科学基金资助项目(52006016)
湖南省自然科学基金资助项目(2023JJ30047; 2021JJ40573; 2020JJ4098; 2025JJ60890)
湖南省教育厅科学研究重点项目(21A0216)
湖南省教育厅优秀青年项目(202B041; 22B0291)
长沙市自然科学基金资助项目(kq2014104)
长沙理工大学青年教师成长计划项目(2019QJCZ044)
作者信息
    1.长沙理工大学能源与动力工程学院，湖南 长沙 410114
    2.可再生能源电力技术湖南省重点实验室，湖南 长沙 410114

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2种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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