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To achieve efficient filtration and enhance the degradation of antibiotics in water, a CoFe₂O₄-modified flat-sheet ceramic membrane was prepared using the impregnation-sintering method. The performance of this ceramic membrane activated by peroxymonosulfate (PMS) for the removal of florfenicol (FLO) and other antibiotics was investigated under dead-end filtration mode. The results indicated that at a pH value of 6 and a PMS dosage of 0.5mmol/L, the removal efficiency of FLO (10mg/L) was achieved at 88% within 30minutes. Furthermore, the system exhibited excellent resistance to interference from coexisting species such as Cl^-, NO₃^-, HCO₃^- and humic acid. After 7 cycles of FLO degradation using the CoFe₂O₄ ceramic membrane/PMS system, the removal rate of FLO remained high at 84%. Mechanistic studies revealed that HO^·, SO₄^·-, O₂^·-, ¹O₂ were identified as the primary reactive species responsible for the catalytic degradation. Treatment results of actual aquaculture wastewater showed that the removal efficiencies for COD and turbidity were 65.4% and 99.3%, respectively. Simultaneously, the removal rates for eight typical antibiotics present in the wastewater exceeded 80%, highlighting its significant potential for practical application.

, authors=Rong-rong ZHU¹, Ji-xiao XU¹, Wei-wei RUAN², Ru-ya CHEN^{1, *}, Yi-jing XIA¹, Hua-jun FENG³, Yang-cheng DING^{3, **}, authorsList=Rong-rong ZHU, Ji-xiao XU, Wei-wei RUAN, Ru-ya CHEN, Yi-jing XIA, Hua-jun FENG, Yang-cheng DING, authorCompany=null, correspAuthors=Ru-ya CHEN, Yang-cheng DING, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314918263482577391, articleId=1314918263000232429, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=CoFe₂O₄催化陶瓷膜活化过一硫酸盐去除水中典型抗生素, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

为实现高效过滤并强化水中抗生素降解，采用浸渍烧结法制备了一种CoFe₂O₄修饰的平板陶瓷膜，并在死端过滤模式下对该陶瓷膜活化过一硫酸盐（PMS）去除氟苯尼考（FLO）等抗生素的性能进行了研究．结果表明，在pH值为6，PMS投加量为0.5mmol/L时，30min内该体系对10mg/L的FLO的去除率高达88%．此外，该体系对Cl^-、NO₃^-、HCO₃^-和腐殖酸等共存物质表现出良好的抗干扰能力．利用CoFe₂O₄陶瓷膜/PMS体系循环降解FLO 7次后，该体系对FLO的去除率仍高达84%．机理研究表明，HO^·、SO₄^·-、O₂^·-和¹O₂是催化降解过程中的主要活性物种．对实际养殖废水的处理结果显示，该体系对COD和浊度的去除率分别为65.4%和99.3%，同时对废水中8种典型抗生素的去除率均达到80%以上，展现出巨大的应用潜力．

, authors=朱荣荣¹, 徐纪晓¹, 阮薇薇², 陈儒雅^{1, *}, 夏伊静¹, 冯华军³, 丁养城^{3, **}, authorsList=朱荣荣, 徐纪晓, 阮薇薇, 陈儒雅, 夏伊静, 冯华军, 丁养城, authorCompany=null, correspAuthors=陈儒雅, 丁养城, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=wItqQppoUyKgKOIq2tZAfg==, magXml=KCDgV+1qG71Z8RDfplyxbA==, pdfUrl=null, pdf=Ig+ScSfjstaraKGF2+uAWA==, pdfFileSize=4096784, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=daFxGcPPJjMLkER8fR1Y1g==, mapNumber=null, fund=null)}, authors=[Author(id=1314918263935562234, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918263000232429, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=2644684503@qq.com, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1314918264015254012, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918263000232429, authorId=1314918263935562234, language=EN, stringName=Rong-rong ZHU, firstName=Rong-rong, middleName=null, lastName=ZHU, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.School of Environmental Science and Engineering, Zhejiang Gongshang University, Hangzhou 310018, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314918264103334397, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314918263000232429, authorId=1314918263935562234, language=CN, stringName=朱荣荣, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=¹, address=^1.浙江工商大学环境科学与工程学院，浙江 杭州 310018, bio={"content":"

朱荣荣（1996-），女，江西上饶人，浙江工商大学硕士研究生，主要从事催化陶瓷膜去除水中抗生素研究．2644684503@qq.com.

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朱荣荣（1996-），女，江西上饶人，浙江工商大学硕士研究生，主要从事催化陶瓷膜去除水中抗生素研究．2644684503@qq.com.

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