Article(id=1314917810506137654, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917704910340427, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1737302400000, receivedDateStr=2025-01-20, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791430436015, onlineDateStr=2026-10-08, pubDate=1755619200000, pubDateStr=2025-08-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791430436015, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791430436015, creator=13701087609, updateTime=1791430436015, updator=13701087609, issue=Issue{id=1314917704910340427, tenantId=1146029695717560320, journalId=1234093305789726721, year='2025', volume='45', issue='8', pageStart='4145', pageEnd='4736', issueExtLink='null', onlineDate='null', pubDate='1755619200000', pubDateStr='2025-08-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791430410840, creator='13701087609', updateTime=1791431909627, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314923991341555972, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917704910340427, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314923991345750277, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917704910340427, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=4656, endPage=4666, ext={EN=ArticleExt(id=1314917810980094007, articleId=1314917810506137654, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Distribution, flux, microbial consumption and dark production of carbon monoxide in the East China Sea in autumn, columnId=1234106390126588740, journalTitle=China Environmental Science, columnName=Carbon Emission Control, runingTitle=null, highlight=null, articleAbstract=

A field survey was conducted in the East China Sea in autumn 2023 to study the distributions of carbon monoxide (CO) concentration, estimate the sea-to-air fluxes, and measure the microbial consumption and dark production rates of CO in the surface seawater. The results showed that atmospheric CO mixing ratios of the East China Sea ranged from 61.15 to 234.26 ppbv, with an average of (98.47 ± 49.64) ppbv. A headspace analysis system was used to determine CO. The concentrations of CO in the surface seawater ranged from 0.20 to 1.63 nmol/L, with an average of (0.63 ± 0.71) nmol/L. The CO concentrations exhibited noticeable daily variations across different water layers, with a maximum at noon and a minimum around dawn. The results of vertical distributions showed that the CO concentrations decreased gradually with the increase of depth. The sea-to-air fluxes of CO ranged from 0.45 to 5.66μmol/(m2·d), with an average of (2.11 ± 2.89) μmol/(m2·d). The results of sea-to-air fluxes estimation showed that the East China Sea was a source of atmospheric CO. The microbial consumption rate constants of CO in the surface seawater ranged from 0.16 to 0.33/h, with an average of (0.22 ± 0.07)/h. The consumption process showed the characteristics of first-order reaction. Dark production rates varied from 0.023 to 0.20nmol/(L·h), with an average of (0.12 ± 0.14) nmol/(L·h). The concentrations of CO increased linearly with the increase of time. This survey complements the source-sink processes of CO in the East China Sea, and contributes to a further understanding of the CO biogeochemical processes and its climatic effect in the continental shelf sea area.

, authors=Jiao-jiao PANG1, Li-xuan CHU1, Wen-yu HOU1, Jing ZHANG1, 2, Zhen HE1, 2, Gui-peng YANG1, 2, *, authorsList=Jiao-jiao PANG, Li-xuan CHU, Wen-yu HOU, Jing ZHANG, Zhen HE, Gui-peng YANG, authorCompany=null, correspAuthors=Gui-peng YANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314917812154499128, articleId=1314917810506137654, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=秋季东海一氧化碳的分布、通量、微生物消耗和暗反应生成研究, columnId=1234106391661704058, journalTitle=中国环境科学, columnName=碳排放控制, runingTitle=null, highlight=null, articleAbstract=

基于2023年秋季在中国东海的现场调查,研究该海域一氧化碳(CO)的浓度分布特征,估算CO海—气通量,测定表层海水CO微生物消耗和暗反应生成速率.结果表明,东海大气CO的混合比为61.15 ~ 234.26ppbv,平均值为(98.47 ± 49.64)ppbv.用顶空分析法测定的表层海水中CO的浓度为0.20 ~1.63nmol/L,平均值为(0.63 ± 0.71)nmol/L.各水层CO浓度日变化显著,表现为午后浓度最高,凌晨前后浓度最低.垂直剖面显示,CO浓度随深度的增加而减小.CO的海—气通量为0.45 ~ 5.66 μmol/(m2·d),平均值为(2.11 ± 2.89)μmol/(m2·d),表明东海是大气CO的源.表层海水CO微生物消耗速率常数为0.16~ 0.33/h,平均值为(0.22 ± 0.07)/h.CO浓度消耗过程表现出一级反应动力学特征.CO暗反应生成速率为0.023 ~ 0.20nmol/(L·h),平均值为(0.12 ± 0.14)nmol/(L·h),CO浓度随时间增长线性增加.本次调查对中国东海CO的源—汇过程进行了补充,有助于深入理解陆架海域CO生物地球化学过程及其气候效应.

, authors=庞娇娇1, 褚礼轩1, 侯雯彧1, 张婧1, 2, 何真1, 2, 杨桂朋1, 2, *, authorsList=庞娇娇, 褚礼轩, 侯雯彧, 张婧, 何真, 杨桂朋, authorCompany=null, correspAuthors=杨桂朋, authorNote=

庞娇娇(1999-),女,山东烟台人,中国海洋大学化学化工学院硕士研究生,主要从事海洋生源活性气体CO研究.发表论文1篇..

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庞娇娇(1999-),女,山东烟台人,中国海洋大学化学化工学院硕士研究生,主要从事海洋生源活性气体CO研究.发表论文1篇..

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庞娇娇(1999-),女,山东烟台人,中国海洋大学化学化工学院硕士研究生,主要从事海洋生源活性气体CO研究.发表论文1篇..

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秋季东海一氧化碳的分布、通量、微生物消耗和暗反应生成研究
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庞娇娇 1 , 褚礼轩 1 , 侯雯彧 1 , 张婧 1, 2 , 何真 1, 2 , 杨桂朋 1, 2, *
中国环境科学 | 碳排放控制 2025,45(8): 4656-4666
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中国环境科学 |碳排放控制 2025 , 45 (8) : 4656 -4666
秋季东海一氧化碳的分布、通量、微生物消耗和暗反应生成研究
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庞娇娇(1999-),女,山东烟台人,中国海洋大学化学化工学院硕士研究生,主要从事海洋生源活性气体CO研究.发表论文1篇..

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庞娇娇(1999-),女,山东烟台人,中国海洋大学化学化工学院硕士研究生,主要从事海洋生源活性气体CO研究.发表论文1篇..

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庞娇娇1 , 褚礼轩1, 侯雯彧1, 张婧1, 2, 何真1, 2, 杨桂朋1, 2, *
作者信息
  • 1.中国海洋大学化学化工学院,海洋化学理论与工程技术教育部重点实验室,山东 青岛 266100
  • 2.青岛海洋科技中心海洋生态与环境科学功能实验室,山东 青岛 266237
通讯作者:
* 责任作者,教授,
作者简介:

庞娇娇(1999-),女,山东烟台人,中国海洋大学化学化工学院硕士研究生,主要从事海洋生源活性气体CO研究.发表论文1篇..

Distribution, flux, microbial consumption and dark production of carbon monoxide in the East China Sea in autumn
Jiao-jiao PANG1 , Li-xuan CHU1, Wen-yu HOU1, Jing ZHANG1, 2, Zhen HE1, 2, Gui-peng YANG1, 2, *
Affiliations
  • 1.College of Chemistry Engineering, Ocean University of China, Key Laboratory of Ministry of Education for Marine Chemistry Theory and Technology, Qingdao 266100, China
  • 2.Laboratory for Marine Ecology and Environmental Science, Qingdao National Laboratory for Marine Science and Technology, Qingdao 266237, China
出版时间: 2025-08-20
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基于2023年秋季在中国东海的现场调查,研究该海域一氧化碳(CO)的浓度分布特征,估算CO海—气通量,测定表层海水CO微生物消耗和暗反应生成速率.结果表明,东海大气CO的混合比为61.15 ~ 234.26ppbv,平均值为(98.47 ± 49.64)ppbv.用顶空分析法测定的表层海水中CO的浓度为0.20 ~1.63nmol/L,平均值为(0.63 ± 0.71)nmol/L.各水层CO浓度日变化显著,表现为午后浓度最高,凌晨前后浓度最低.垂直剖面显示,CO浓度随深度的增加而减小.CO的海—气通量为0.45 ~ 5.66 μmol/(m2·d),平均值为(2.11 ± 2.89)μmol/(m2·d),表明东海是大气CO的源.表层海水CO微生物消耗速率常数为0.16~ 0.33/h,平均值为(0.22 ± 0.07)/h.CO浓度消耗过程表现出一级反应动力学特征.CO暗反应生成速率为0.023 ~ 0.20nmol/(L·h),平均值为(0.12 ± 0.14)nmol/(L·h),CO浓度随时间增长线性增加.本次调查对中国东海CO的源—汇过程进行了补充,有助于深入理解陆架海域CO生物地球化学过程及其气候效应.

一氧化碳  /  浓度分布  /  海—气通量  /  微生物消耗  /  暗反应  /  中国东海

A field survey was conducted in the East China Sea in autumn 2023 to study the distributions of carbon monoxide (CO) concentration, estimate the sea-to-air fluxes, and measure the microbial consumption and dark production rates of CO in the surface seawater. The results showed that atmospheric CO mixing ratios of the East China Sea ranged from 61.15 to 234.26 ppbv, with an average of (98.47 ± 49.64) ppbv. A headspace analysis system was used to determine CO. The concentrations of CO in the surface seawater ranged from 0.20 to 1.63 nmol/L, with an average of (0.63 ± 0.71) nmol/L. The CO concentrations exhibited noticeable daily variations across different water layers, with a maximum at noon and a minimum around dawn. The results of vertical distributions showed that the CO concentrations decreased gradually with the increase of depth. The sea-to-air fluxes of CO ranged from 0.45 to 5.66μmol/(m2·d), with an average of (2.11 ± 2.89) μmol/(m2·d). The results of sea-to-air fluxes estimation showed that the East China Sea was a source of atmospheric CO. The microbial consumption rate constants of CO in the surface seawater ranged from 0.16 to 0.33/h, with an average of (0.22 ± 0.07)/h. The consumption process showed the characteristics of first-order reaction. Dark production rates varied from 0.023 to 0.20nmol/(L·h), with an average of (0.12 ± 0.14) nmol/(L·h). The concentrations of CO increased linearly with the increase of time. This survey complements the source-sink processes of CO in the East China Sea, and contributes to a further understanding of the CO biogeochemical processes and its climatic effect in the continental shelf sea area.

carbon monoxide  /  distribution  /  sea-to-air flux  /  microbial consumption  /  dark production  /  East China Sea
庞娇娇, 褚礼轩, 侯雯彧, 张婧, 何真, 杨桂朋. 秋季东海一氧化碳的分布、通量、微生物消耗和暗反应生成研究. 中国环境科学, 2025 , 45 (8) : 4656 -4666 .
Jiao-jiao PANG, Li-xuan CHU, Wen-yu HOU, Jing ZHANG, Zhen HE, Gui-peng YANG. Distribution, flux, microbial consumption and dark production of carbon monoxide in the East China Sea in autumn[J]. China Environmental Science, 2025 , 45 (8) : 4656 -4666 .
  • 国家自然科学基金重点项目(42330402)
  • 泰山学者攀登专家项目(tspd20240805)
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  • 接收时间:2025-01-20
  • 首发时间:2026-10-08
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  • 收稿日期:2025-01-20
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国家自然科学基金重点项目(42330402)
泰山学者攀登专家项目(tspd20240805)
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    1.中国海洋大学化学化工学院,海洋化学理论与工程技术教育部重点实验室,山东 青岛 266100
    2.青岛海洋科技中心海洋生态与环境科学功能实验室,山东 青岛 266237

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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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