Article(id=1314917781284422494, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917704910340427, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1737475200000, receivedDateStr=2025-01-22, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791430429049, onlineDateStr=2026-10-08, pubDate=1755619200000, pubDateStr=2025-08-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791430429049, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791430429049, creator=13701087609, updateTime=1791430429049, updator=13701087609, issue=Issue{id=1314917704910340427, tenantId=1146029695717560320, journalId=1234093305789726721, year='2025', volume='45', issue='8', pageStart='4145', pageEnd='4736', issueExtLink='null', onlineDate='null', pubDate='1755619200000', pubDateStr='2025-08-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791430410840, creator='13701087609', updateTime=1791431909627, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314923991341555972, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917704910340427, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314923991345750277, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917704910340427, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=4341, endPage=4353, ext={EN=ArticleExt(id=1314917781498331999, articleId=1314917781284422494, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Degradation of azo dyes in sio₂coated nzvi@Fe₃O₄ Fenton-like system, columnId=1234106386360103680, journalTitle=China Environmental Science, columnName=Water Pollution Control, runingTitle=null, highlight=null, articleAbstract=

SiO₂@nZVI@Fe₃O₄ composites were successfully synthesized by liquid-phase reduction and stőber hydrolysis. The microstructures and physical phase compositions of SiO₂@nZVI@Fe₃O₄ were analyzed by SEM-EDS, TEM, XRD, FTIR, VSM, and XPS. The degradation performance of azo dyes was investigated by using SiO₂@nZVI@Fe₃O₄ as a non-homogeneous catalyst combined with H₂O₂to construct a Fenton-like system. The results showed that the SiO₂ coating improved the dispersion and oxidation resistance of nZVI@Fe₃O₄, and it was able to enhance the generation of Fe²⁺ and HO· in the Fenton-like reaction system. Under the conditions of 25℃, pH 3, H₂O₂ concentration of 15mmol/L, and material dosage of 0.6g/L, the removal efficiency of Congo red, Orange II and Acid Black 210 reached 99.68 %、98.14 % and 99.35 %. The composite material could still remove more than 79% of the three pollutants after recycling for three times, which has good stable catalytic performance. The removal of azo dyes by SiO₂@nZVI@Fe₃O₄ combined with Fenton-like system was mainly through the reduction of nZVI and the oxidation of HO·, as demonstrated by reactive oxygen species quenching experiment and UV-visible spectral analysis.

, authors=Jin-kui ZHONG^{1, 2, *}, Jia-wen HE¹, Xin-hao WANG¹, Yin ZHANG¹, Yuan-hu GAO¹, Cai-ya ZHU¹, Xin-yue ZHOU¹, Si-qian WANG¹, authorsList=Jin-kui ZHONG, Jia-wen HE, Xin-hao WANG, Yin ZHANG, Yuan-hu GAO, Cai-ya ZHU, Xin-yue ZHOU, Si-qian WANG, authorCompany=null, correspAuthors=Jin-kui ZHONG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314917783373185890, articleId=1314917781284422494, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=SiO₂包覆nZVI@Fe₃O₄类Fenton体系对偶氮染料的降解, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

通过液相还原法和stőber水解法合成了SiO₂@nZVI@Fe₃O₄复合材料，并采用SEM-EDS、TEM、XRD、FTIR、VSM和XPS对其微观结构和物相组成进行了分析和表征．以SiO₂@nZVI@Fe₃O₄为非均相催化剂与H₂O₂耦合构建类Fenton体系，考察该体系对偶氮类染料的降解性能．结果表明，SiO₂包覆后nZVI@Fe₃O₄复合材料的分散性和抗氧化性得到提高，由其构建的类Fenton反应体系能促进Fe²⁺和HO·的生成．在25℃，pH3，H₂O₂浓度为15mmol/L，材料投加量为0.6g/L的条件下，刚果红、橙黄Ⅱ和酸性黑210的去除率分别为99.68%、98.14%和99.35%．复合材料在循环利用3次后对3种污染物的去除率仍保持在79%以上，表明SiO₂@nZVI@Fe₃O₄材料具有良好的稳定催化性能．活性氧物种淬灭实验和紫外-可见光谱分析表明，SiO₂@nZVI@Fe₃O₄类Fenton体系对偶氮染料的去除机理主要是通过nZVI的还原作用和HO·的氧化作用．

, authors=钟金魁^{1, 2, *}, 何嘉文¹, 王新昊¹, 张尹¹, 高原虎¹, 朱彩亚¹, 周鑫悦¹, 王思倩¹, authorsList=钟金魁, 何嘉文, 王新昊, 张尹, 高原虎, 朱彩亚, 周鑫悦, 王思倩, authorCompany=null, correspAuthors=钟金魁, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=tYaU/fgONfyQhzJd2VtGfQ==, magXml=pj7kXsAfpMztIzJN2TILQw==, pdfUrl=null, pdf=Djc1+4+Ord0qi0g95j7WqQ==, pdfFileSize=2738025, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=RdqXnXmID0ZfiwGIk/NX7w==, mapNumber=null, fund=null)}, authors=[Author(id=1314917783918445418, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917781284422494, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=zhongjk@mail.lzjtu.cn, emailSecond=null, emailThird=null, correspondingAuthor=1, authorType=1, ext={EN=AuthorExt(id=1314917784006525805, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917781284422494, authorId=1314917783918445418, language=EN, stringName=Jin-kui ZHONG, firstName=Jin-kui, middleName=null, lastName=ZHONG, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=^{1, 2, *}, address=^1.School of Environmental and Municipal Engineering, Lanzhou Jiaotong University, Lanzhou 730070, China
^2.Ministry of Education Engineering Research Center of Water Resource Comprehensive Utilization in Cold and Arid Regions, Lanzhou 730070, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314917784107189102, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917781284422494, authorId=1314917783918445418, language=CN, stringName=钟金魁, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=^{1, 2, *}, address=^1.兰州交通大学环境与市政工程学院，甘肃 兰州 730070
^2.寒旱地区水资源综合利用教育部工程研究中心，甘肃 兰州 730070, bio={"content":"

钟金魁（1968-），男，甘肃古浪人，教授，硕士，主要从事土壤污染修复和污水处理研究．发表论文44篇．zhongjk@mail.lzjtu.cn.

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钟金魁（1968-），男，甘肃古浪人，教授，硕士，主要从事土壤污染修复和污水处理研究．发表论文44篇．zhongjk@mail.lzjtu.cn.

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