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This study addresses challenges in conventional advanced oxidation processes (AOPs), including mass transfer limitations of endogenous mediators, and reliance on energy-intensive/sacrificial agents' consumption to maintain the catalytic activity, by proposing an innovative strategy that employs trace H₂O₂ to micro-regulate dual-reaction center (DRC) catalysts for enhanced water self-purification. DRC catalyst (FZSO) with surface electron-polarized distribution can effectively enhance interactions between naturally dissolved oxygen and pollutants, thereby overcomes mass transfer limitations and obviously enhances water self-purification. This process radically changes the role of H₂O₂—innovatively repurposed from the sacrificial agent in AOPs to the precision micro-regulator in DRC system, largely reducing consumption in water treatment. Experimental results demonstrate that under micro-regulation with only 1mmol/L H₂O₂, the FZSO-DRC system achieved complete ciprofloxacin removal within 15min, with less than 10% H₂O₂ consumption. FZSO system also exhibits strong adaptability and stability for complex water matrices (pH or salinity ions). This study proposes a breakthrough in energy-efficient water purification by amplifying natural water self-purification capacity through the FZSO-DRC system, providing new technical perspective for developing high-efficiency, low-consumption water treatment processes.

, authors=Dong-xuan YANG, Qiu-yu LUO, Qian FANG, Ying-tao SUN, Chun HU, Lai LYU^*, authorsList=Dong-xuan YANG, Qiu-yu LUO, Qian FANG, Ying-tao SUN, Chun HU, Lai LYU, authorCompany=null, correspAuthors=Lai LYU, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314917705082298823, articleId=1314917704209883589, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=微量H₂O₂微调控铁锌共掺杂硒氧化物双反应中心体系强化水自净力, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

针对传统净水氧化体系存在的内源性介质传质受限、依赖高能耗或牺牲剂维持催化活性等瓶颈问题，提出利用微量H₂O₂微调控双反应中心（DRC）催化剂表面增强水自净化的创新策略．研究发现，通过制备表面具有电子极化分布结构的DRC催化剂（FZSO）能有效用于增强水中自然溶解氧与污染物的相互作用，打破二者间传质限制从而强化水体自净．这一过程，使H₂O₂角色发生根本性的转变—从传统高级氧化过程中的牺牲剂创新性作为微调控剂，极大降低水处理过程能耗．结果表明，在仅1mmol/L H₂O₂微调控下，FZSO自净增强体系在15min实现对环丙沙星的完全去除，其H₂O₂的消耗不到10%，且不受水中复杂介质（pH值或盐分离子等）的干扰，具有良好的适应性和稳定性．该策略通过强化水体自净力实现节能增效的突破，为开发应用高效的低能耗净水工艺提供新的思路和技术参考．

, authors=杨东旋, 罗秋雨, 方谦, 孙英涛, 胡春, 吕来^*, authorsList=杨东旋, 罗秋雨, 方谦, 孙英涛, 胡春, 吕来, authorCompany=null, correspAuthors=吕来, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=PuxeAvxPcgoSM1c06Xz1Og==, magXml=+dcb84iMfj6CPucLSYvqpA==, pdfUrl=null, pdf=8wAubokYaVZ9UOCPrPXJyw==, pdfFileSize=3358014, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=rd+lWVaZvG84BidW60NImw==, mapNumber=null, fund=null)}, authors=[Author(id=1314917834505945284, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917704209883589, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=yangdongxuannic@163.com, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1314917834614997190, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917704209883589, authorId=1314917834505945284, language=EN, stringName=Dong-xuan YANG, firstName=Dong-xuan, middleName=null, lastName=YANG, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=Key Laboratory of the Ministry of Education for Water Quality Safety and Protection in the Pearl River Delta, Greater Bay Area Environmental Research Institute, Guangzhou University, Guangzhou 510006, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314917834845683911, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917704209883589, authorId=1314917834505945284, language=CN, stringName=杨东旋, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=广州大学，大湾区环境研究院珠江三角洲水质安全与保护教育部重点实验室，广东 广州 510006, bio={"content":"

杨东旋（1998-），男，广东梅州人，博士研究生，主要从事水污染控制研究．发表论文3篇．yangdongxuannic@163.com.

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杨东旋（1998-），男，广东梅州人，博士研究生，主要从事水污染控制研究．发表论文3篇．yangdongxuannic@163.com.

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