Article(id=1314917631845560416, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917567911788907, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1739116800000, receivedDateStr=2025-02-10, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1791430393419, onlineDateStr=2026-10-08, pubDate=1758297600000, pubDateStr=2025-09-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1791430393419, onlineIssueDateStr=2026-10-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1791430393419, creator=13701087609, updateTime=1791430393419, updator=13701087609, issue=Issue{id=1314917567911788907, tenantId=1146029695717560320, journalId=1234093305789726721, year='2025', volume='45', issue='9', pageStart='4737', pageEnd='5328', issueExtLink='null', onlineDate='null', pubDate='1758297600000', pubDateStr='2025-09-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1791430378177, creator='13701087609', updateTime=1791431890195, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1314923910001418489, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917567911788907, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1314923910001418490, tenantId=1146029695717560320, journalId=1234093305789726721, issueId=1314917567911788907, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=4888, endPage=4895, ext={EN=ArticleExt(id=1314917632080441441, articleId=1314917631845560416, tenantId=1146029695717560320, journalId=1234093305789726721, language=EN, title=Study on the catalytic oxidation mechanism of acetone over rod-like SBA-15supported palladium-cobalt catalyst, columnId=1234106386020365051, journalTitle=China Environmental Science, columnName=Air Pollution Control, runingTitle=null, highlight=null, articleAbstract=

Taking the well-structured rod-like SBA-15 as support, Pd₁Co_x/SBA-15 bimetallic catalysts with different palladium(Pd) and cobalt(Co) molar ratios were prepared by adjusting the Co content for acetone (C₃H₆O) catalytic oxidation. Among these, the Pd₁Co₁/SBA-15 catalyst was found to exhibit superior performance for the low-temperature oxidation of C₃H₆O, achieving 90% conversion at 220℃, along with high CO₂ selectivity and thermal stability. Characterization by SEM, XRD, FT-IR, and N₂ adsorption-desorption was conducted, and it was revealed that Pd₁Co₁/SBA-15 possessed the optimal Pd/Co ratio and a higher specific surface area, which were crucial for the stabilization and exposure of active sites. Further investigations using H₂-TPR, O₂-TPD, and XPS indicated that the primary active oxygen species in Pd₁Co_0.5/SBA-15 and Pd₁Co₃/SBA-15 were chemisorbed oxygen, while surface lattice oxygen was predominantly present in Pd₁Co₁/SBA-15. Moreover, the transformation of abundant active oxygen species in Pd₁Co₁/SBA-15 was significantly promoted. The reaction mechanism of acetone oxidation over Pd₁Co₁/SBA-15 was elucidated by in-situ infrared spectroscopy. The decomposition path of acetone molecules over Pd₁Co₁/SBA-15 catalyst was determined as C₃H₆O→CH₃CH₂OH→CH₃COO^-→COO^-→CO₂, which further indicated that enhanced surface lattice oxygen can significantly accelerate activation and cleavage during the acetone oxidation process.

, authors=Ya-ni WU, Jing-jing WANG, Ji-chen LIU, Jia-lei WAN, Fan DANG, Chun-li AI, Mu-di MA^**, Ze-yu JIANG^*, authorsList=Ya-ni WU, Jing-jing WANG, Ji-chen LIU, Jia-lei WAN, Fan DANG, Chun-li AI, Mu-di MA, Ze-yu JIANG, authorCompany=null, correspAuthors=Mu-di MA, Ze-yu JIANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314917632487288930, articleId=1314917631845560416, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=棒状SBA-15负载的钯钴催化剂对丙酮催化氧化机制研究, columnId=1234106388364981004, journalTitle=中国环境科学, columnName=大气污染与控制, runingTitle=null, highlight=null, articleAbstract=

以结构规整的棒状SBA-15分子筛为载体，通过调控过渡金属Co的含量，制备不同Pd-Co摩尔比的Pd₁Co_x/SBA-15贵金属-过渡金属耦合催化剂，用于丙酮（C₃H₆O）的催化氧化研究．结果表明，Pd₁Co₁/SBA-15催化剂展现出最佳的丙酮低温氧化活性，其在220℃时即可实现90%的丙酮转化率，并表现出优异的CO₂选择性与热稳定性．通过SEM，XRD，FT-IR和N₂吸脱附表征分析可知，Pd₁Co₁/SBA-15具有最佳的Pd-Co配比和比表面积，有利于活性位点的锚定与暴露．H₂-TPR，O₂-TPD和XPS表征结果表明，Pd1Co_0.5/SBA-15与Pd₁Co₃/SBA-15中的主要活性氧物种为化学吸附氧，而Pd₁Co₁/SBA-15中的主要活性氧物种为表面晶格氧，且Pd₁Co₁/SBA-15催化剂具有丰富的活性氧物种，在反应过程中保持了高效的晶格氧迁移与循环．通过原位红外光谱揭示了丙酮的反应机理，Pd₁Co₁/SBA-15催化剂上丙酮转化路径为：C₃H₆O→CH₃CH₂OH→CH₃COO^-→COO^-→CO₂，丰富的晶格氧是丙酮活化和裂解的关键．

, authors=武雅妮, 王晶晶, 刘基丞, 万嘉蕾, 党凡, 艾春丽, 马牧笛^**, 姜泽宇^*, authorsList=武雅妮, 王晶晶, 刘基丞, 万嘉蕾, 党凡, 艾春丽, 马牧笛, 姜泽宇, authorCompany=null, correspAuthors=马牧笛, 姜泽宇, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=eSawF+DXlJqURSNKTunJ/Q==, magXml=E6YJ+nb0axFW6LrcMdirkA==, pdfUrl=null, pdf=RpR1zWIawaLRRjQw3Ne0vw==, pdfFileSize=1326512, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=D27awfeuR93fS/XLJ9Ek9Q==, mapNumber=null, fund=null)}, authors=[Author(id=1314917906975125553, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917631845560416, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=wuyani1998@stu.xjtu.edu.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1314917907092566067, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917631845560416, authorId=1314917906975125553, language=EN, stringName=Ya-ni WU, firstName=Ya-ni, middleName=null, lastName=WU, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=Department of Environmental Science and Engineering, Xi'an Jiaotong University, Xi'an 710049, China, bio=null, bioImg=null, bioContent=null, aboutCorrespAuthor=null), CN=AuthorExt(id=1314917907155480628, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1314917631845560416, authorId=1314917906975125553, language=CN, stringName=武雅妮, firstName=null, middleName=null, lastName=null, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=西安交通大学环境科学与工程系，陕西 西安 710049, bio={"content":"

武雅妮（1998-），女，陕西延安人，西安交通大学博士研究生，主要从事挥发性有机污染物降解和贵金属-过渡金属协同催化剂研究．发表论文1篇．wuyani1998@stu.xjtu.edu.cn.

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武雅妮（1998-），女，陕西延安人，西安交通大学博士研究生，主要从事挥发性有机污染物降解和贵金属-过渡金属协同催化剂研究．发表论文1篇．wuyani1998@stu.xjtu.edu.cn.

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