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To solve the problems of high synthesis cost and lack of specific adsorption sites on traditional zeolites surface, polydopamine-modified coal gangue based zeolite was successfully synthesized by combining alkali melting hydrothermal method and impregnation coating method using coal gangue as raw material and dopamine as the polymerization monomer and applied for efficient adsorption of Cd(Ⅱ) from aqueous solution. The adsorption performance was investigated by batch adsorption experiments, and adsorption mechanism was revealed by SEM-EDS and XPS method. The results showed that polydopamine coating significantly improved the adsorption capacity of coal gangue-derived zeolite. The adsorption process conformed to the Langmuir adsorption isotherm model and pseudo-second-order model, suggesting that Cd(Ⅱ) adsorption by Zeolite@PDA was monolayer and chemical adsorption, and the theoretical maximum adsorption capacity could reach 130.89mg/g, which was two times as high as that of Zeolite (q_max=66.49mg/g). Thermodynamic studies indicated that Cd(Ⅱ) adsorption by Zeolite@PDA was a spontaneous, endothermic process with increased disorder at the solid-liquid interface. SEM-EDS and XPS analysis showed that cation exchange between Na⁺and Cd(Ⅱ) as well as surface complexation between surface functional groups and Cd(Ⅱ) played a primary role for Cd(Ⅱ) removal.

, authors=Yu-zhi ZHOU^{1, 2}, Lin-li LONG¹, Pian HU¹, Jing-yu SUN¹, Jing-wei NIU¹, Min CHEN³, Wen-shuo WANG¹, Xiao-yang CHEN^{1, 2, *}, authorsList=Yu-zhi ZHOU, Lin-li LONG, Pian HU, Jing-yu SUN, Jing-wei NIU, Min CHEN, Wen-shuo WANG, Xiao-yang CHEN, authorCompany=null, correspAuthors=Xiao-yang CHEN, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1314917515592032560, articleId=1314917514941915438, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=聚多巴胺修饰矸石基沸石净化含镉污水性能与机制, columnId=1234106386565624579, journalTitle=中国环境科学, columnName=水污染与控制, runingTitle=null, highlight=null, articleAbstract=

针对传统沸石合成成本高且表面缺乏特异性吸附位点的问题，以煤矸石为研究对象，多巴胺为聚合单体，采用水热法-表面自聚合反应制备了聚多巴胺改性矸石基沸石（Zeolite@PDA）用于水中镉的高效吸附去除，通过静态吸附实验研究了改性前后沸石的吸附性能，运用SEM-EDS和XPS表征手段揭示了其对水中Cd（Ⅱ）的吸附机制．结果表明，聚多巴胺涂层显著提高了煤矸石基沸石对Cd（Ⅱ）的吸附能力．Zeolite@PDA吸附Cd（Ⅱ）的过程更符合Langmuir吸附等温模型和准二级动力学模型，说明吸附过程是单层的化学吸附，且理论上最大吸附量可达130.89mg/g，约为矸石基沸石的2倍（q_max=66.49mg/g）．热力学研究表明Zeolite@PDA吸附Cd（Ⅱ）是自发，吸热且固液界面紊乱度增加的过程．SEM-EDS和XPS表征显示，Zeolite@PDA对Cd（Ⅱ）的去除机理包括沸石中Na⁺与Cd（Ⅱ）的离子交换反应和聚多巴胺涂层官能团与Cd（Ⅱ）的表面络合作用．

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周育智（1990-），男，安徽淮南人，讲师，博士，主要从事固体废物资源化利用、环境功能材料与水污染控制研究．发表论文20余篇．Zhouyuzhi1218@126.com.

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周育智（1990-），男，安徽淮南人，讲师，博士，主要从事固体废物资源化利用、环境功能材料与水污染控制研究．发表论文20余篇．Zhouyuzhi1218@126.com.

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