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This paper reviewed the occurrence characteristics and abundance of microplastics (MPs) in disinfection processes of water treatment plants both inside and outside China, and analyzed the MPs removal effectiveness of chlorine, ozone and ultraviolet disinfection, followed by an in-depth discussion of the effects of MPs presence on disinfection and its secondary pollution. The results showed significant differences in the abundance of MPs across different water treatment plants, primarily existing in the forms of fibers and fragments, predominantly composed of polyethylene terephthalate (PET), polyethylene (PE), and polypropylene (PP), with most sizes less than 1.0mm and colors mostly black, white, or transparent. The removal rate of the chlorine disinfection unit ranged from 0% to 71.38%; but part of the water treatment plants had seen a rise in MPs abundance after the ozone and ultraviolet disinfection. The removal mechanisms of MPs by disinfection processes remained required further research. Additionally, the trihalomethane formation potential (THMFP) of microplastic-derived dissolved organic matter (MP-DOM) in the chlorine disinfection process could reach as high as 453.3µg/mg, higher than the formation potential of typical aquatic natural organic matter and algae organic matter, pointing to greater health risks.

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本文综述了国内外水厂消毒工艺中微塑料(MPs)的赋存特征和丰度情况，分析了氯、臭氧和紫外线消毒对MPs的去除效果，并深入探讨了MPs的存在对消毒的影响及其二次污染.结果发现，不同水厂消毒中MPs丰度具有较大差异，主要以纤维、碎片形状存在，以聚对苯二甲酸乙二醇酯(PET)、聚乙烯(PE)和聚丙烯(PP)为主，粒径大部分小于1.0mm，颜色多呈黑白和透明.氯消毒单元去除率在0~71.38%，但在部分水厂的臭氧消毒和紫外线消毒后，MPs丰度反而上升.消毒工艺对MPs的去除机制仍有待研究.此外，其释放的溶解性有机物(MP-DOM)在氯消毒过程中生成三氯甲烷的潜能(THMFP)最高可达453.3µg/mg，高于典型水生天然有机物和藻类有机物的生成潜力，显示出更大的健康风险.

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赵思凯(1999-)，男，四川乐山人，重庆交通大学硕士研究生，主要研究方向为水污染控制技术及原理.发表论文1篇.

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赵思凯(1999-)，男，四川乐山人，重庆交通大学硕士研究生，主要研究方向为水污染控制技术及原理.发表论文1篇.

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Journal of Environmental Sciences，2023，43(10):108-115., articleTitle=Effect of pre-ozonation on disinfection byproduct formation from microplastics upon subsequent chlorination, refAbstract=null)], funds=[Fund(id=1241408725257343731, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, awardId=KJQN202404306, language=CN, fundingSource=重庆市教委科学技术研究项目(KJQN202404306), fundOrder=null, country=null), Fund(id=1241408725504807683, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, awardId=JDLHPYJD2022005, language=CN, fundingSource=重庆市研究生联合培养基地建设项目(JDLHPYJD2022005), fundOrder=null, country=null), Fund(id=1241408725605470989, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, awardId=51608079, language=CN, fundingSource=国家自然科学基金资助项目(51608079), fundOrder=null, country=null)], companyList=[AuthorCompany(id=1241408717317526528, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, xref=1., ext=[AuthorCompanyExt(id=1241408717325914112, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, companyId=1241408717317526528, language=EN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=^1.Key Laboratory of Water Conservancy and Water Transport Engineering, Ministry of Education, Hehai College, Chongqing Jiaotong University, Chongqing 400074, China), AuthorCompanyExt(id=1241408717342691329, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, companyId=1241408717317526528, language=CN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=^1.重庆交通大学河海学院，水利水运工程教育部重点实验室，重庆 400074)]), AuthorCompany(id=1241408717506269196, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, xref=2., ext=[AuthorCompanyExt(id=1241408717510463501, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, companyId=1241408717506269196, language=EN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=^2.Southwest Technical Engineering Research Institute, Chongqing 400039, China), AuthorCompanyExt(id=1241408717523046414, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, companyId=1241408717506269196, language=CN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=^2.西南技术工程研究所，重庆 400039)]), AuthorCompany(id=1241408717690818585, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, xref=3., ext=[AuthorCompanyExt(id=1241408717699207194, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, companyId=1241408717690818585, language=EN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=^3.Engineering Design Group Co. 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Characteristics of MPs in the disinfection process of domestic and foreign water treatment plants

, figureFileSmall=null, figureFileBig=null, tableContent=

水厂类型	国家	处理工艺	工艺进水丰度(个/L)	工艺出水丰度(个/L)	颜色	成分	形状	粒径(µm)	文献
污水处理厂	中国	氯消毒	34.1±9.4	28.4±7.0	透明(57.6)棕色(18)黑色(10)	PA (54.8)PP (9.6)PE (9.0)	纤维(56.5)碎片(30.4)	20~300 (63.9)300~1000 (29)1000~2000 (5.5)	[22]
		氯消毒	30.1±8.2	22.9±7.2	黑色(52.5)红色(23.9)透明(22)	PP (33)PE (23)PS (18)	纤维(47.9)碎片(21.8)薄膜(17.3)颗粒(13)	0~100 (81.5)100~500 (13.4)500~1000 (3.8)	[32]
		紫外线消毒	19.67±0.94	17.33±1.25	透明(54.3)黑色(35.5)	PE (38)PS (32)PP (20)	纤维(96.6)	<500 (69.5)500~1000 (17)1000~2000 (6.8)	[33]
		紫外线消毒	0.01	0.13±0.01	—	PET (47)PS (20)PE (18)PP (15)	纤维(100)	125~250 (100)	[19]
		紫外线消毒	37.9±8.5	30.6±7.8	透明(47.3)灰色(35.9)	PES (29.5)PA (20.5)PET (14.3)PE (11.6)	纤维(54.3)碎片(34.3)	20~100 (42.7)100~500 (48.5)500~1000 (4.0)	[34]
		紫外线消毒	1.85	2.9	黑色(36)红色(23)蓝色(17)	PE (31.03)PP (24.14)PA (20.69)PET (17.24)	纤维(84)碎片(16)	80~550 (43.3)550~1700 (40.5)1700~5000 (16.2)	[35]
		反硝化-超滤-臭氧-紫外线消毒	2.21±1.43	0.59±0.22	黑色(36.6)透明(33.84)蓝色(11.88)	PET (42.3)PES (19.1)PP (13.1)	纤维(85.9)	<1000 (64.2)1000~2000 (28.7)	[36]
污水处理厂	韩国	快速砂滤-紫外线消毒	1	0.5	—	丙烯酸(25.2)PP (24.3)PU (19.9)PES/PET (18.9)	碎片(55.7)纤维(44.3)	20~50 (36.0)50~200 (33.8)200~500 (22)>500 (18.2)	[37]
		臭氧	164	33	—	—	颗粒(78.9)纤维(12)	—	[38]
	印度	纤维转盘过滤-氯消毒	328	278	黑色(76)透明(10.7)其他(13.3)	PEPPPS	碎片(87.1)纤维(12.9)	<240 (75)240~2090 (25)	[39]
饮用水厂	中国	紫外线消毒	386±211	377±23	—	PP (24.4)PET (19.0)PU (14.9)PE (13.2)	碎片(81.5)纤维(18.5)	1~5 (84.0)5~10 (12.2)10~50 (3.8)	[40]
		臭氧	2230±104	2348±109	—	PET (30.2)PE (23.3)PP (14.5)PAM (10.8)	纤维(52.2)碎片(29.8)	1~5 (85.0)5~10 (14.0)10~50 (1.0)	[23]
		氯消毒	963±57	936±51	—	PET (53.8)PE (12.9)PP (12.7)PAM (12.6)	纤维(67.1)碎片(26.2)	1~5 (87.0)5~10 (13.5)
饮用水厂	捷克共和国	臭氧	243±17	224±3	—	醋酸纤维素(27.8)PET (20.5)PP (18.5)PE (15.6)	碎片(77.5)纤维(12.5)	1~5 (48.9)5~10 (33.1)10~50 (12.0)>50 (6.0)	[41]
		紫外线-氯消毒	149±1	151±4	—	醋酸纤维素(25.1)PET (21.9)PE (17.7)PP (17.0)	碎片(78.7)纤维(11.3)	1~5 (50.2)5~10 (33.0)10~50 (8.2)>50 (8.6)
	西班牙	氯消毒	0.06±0.04	0.06±0.04	—	PES (41.6)PP (37.7)PS (6.5)	纤维(54.6)碎片(45.4)	20~200 (14.0)200~500 (42.3)500~1000 (30.2)1000~2000 (13.5)	[42]
		电渗析-氯消毒	0.032±0.013	0.075±0.019	—	人造纤维素(53)PES (21)PE (16)PP (5)	碎片(53)纤维(37)薄膜(11)	50~100 (33.0)100~500 (67.0)	[43]
	柬埔寨	氯消毒	578	521±61	—	PET (28.8)PE (27.1)PP (8.5)PES/PA (6.8)	碎片(60.8)纤维(39.2)	6.5~20 (36.5)20~53 (32.4)53~500 (19.8)>500 (11.3)	[44]
		氯消毒	693	617±147	—	PET (26)PE (20.8)PA (10.4)PES (9.1)	碎片(53.4)纤维(46.6)	6.5~20 (42.0)20~53 (29.0)53~500 (19.9)>500 (9.1)	[44]
	印度	预氯化消毒	17.88	17.53	—	PET (56)PE (33)	纤维(55)碎片/薄膜(45)	<25 (29.9)25~50 (16.9)50~100 (50.3)>100 (2.8)	[45]
饮用水厂	印度尼西亚	氯消毒	13.8	12.3	黑色(50.4)黄色(18.7)红色(16.3)蓝色(14.6)	PESPEPP	纤维(92.8)碎片(7.2)	1~100 (14.5)101~350 (25.4)351~1000 (39.9)1001~5000 (20.3)	[46]
		氯消毒	29.7	8.5	黑色(38.8)蓝色(27.1)红色(12.2)黄色(15.3)	PESPEPP	纤维(96)碎片(4)	1~100 (10.4)101~350 (20.2)351~1000 (38.4)1001~5000 (31.0)	[46]

), ArticleFig(id=1241408724703695544, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, language=CN, label=表1, caption=

国内外水厂消毒工艺中MPs的特征

, figureFileSmall=null, figureFileBig=null, tableContent=

水厂类型	国家	处理工艺	工艺进水丰度(个/L)	工艺出水丰度(个/L)	颜色	成分	形状	粒径(µm)	文献
污水处理厂	中国	氯消毒	34.1±9.4	28.4±7.0	透明(57.6)棕色(18)黑色(10)	PA (54.8)PP (9.6)PE (9.0)	纤维(56.5)碎片(30.4)	20~300 (63.9)300~1000 (29)1000~2000 (5.5)	[22]
		氯消毒	30.1±8.2	22.9±7.2	黑色(52.5)红色(23.9)透明(22)	PP (33)PE (23)PS (18)	纤维(47.9)碎片(21.8)薄膜(17.3)颗粒(13)	0~100 (81.5)100~500 (13.4)500~1000 (3.8)	[32]
		紫外线消毒	19.67±0.94	17.33±1.25	透明(54.3)黑色(35.5)	PE (38)PS (32)PP (20)	纤维(96.6)	<500 (69.5)500~1000 (17)1000~2000 (6.8)	[33]
		紫外线消毒	0.01	0.13±0.01	—	PET (47)PS (20)PE (18)PP (15)	纤维(100)	125~250 (100)	[19]
		紫外线消毒	37.9±8.5	30.6±7.8	透明(47.3)灰色(35.9)	PES (29.5)PA (20.5)PET (14.3)PE (11.6)	纤维(54.3)碎片(34.3)	20~100 (42.7)100~500 (48.5)500~1000 (4.0)	[34]
		紫外线消毒	1.85	2.9	黑色(36)红色(23)蓝色(17)	PE (31.03)PP (24.14)PA (20.69)PET (17.24)	纤维(84)碎片(16)	80~550 (43.3)550~1700 (40.5)1700~5000 (16.2)	[35]
		反硝化-超滤-臭氧-紫外线消毒	2.21±1.43	0.59±0.22	黑色(36.6)透明(33.84)蓝色(11.88)	PET (42.3)PES (19.1)PP (13.1)	纤维(85.9)	<1000 (64.2)1000~2000 (28.7)	[36]
污水处理厂	韩国	快速砂滤-紫外线消毒	1	0.5	—	丙烯酸(25.2)PP (24.3)PU (19.9)PES/PET (18.9)	碎片(55.7)纤维(44.3)	20~50 (36.0)50~200 (33.8)200~500 (22)>500 (18.2)	[37]
		臭氧	164	33	—	—	颗粒(78.9)纤维(12)	—	[38]
	印度	纤维转盘过滤-氯消毒	328	278	黑色(76)透明(10.7)其他(13.3)	PEPPPS	碎片(87.1)纤维(12.9)	<240 (75)240~2090 (25)	[39]
饮用水厂	中国	紫外线消毒	386±211	377±23	—	PP (24.4)PET (19.0)PU (14.9)PE (13.2)	碎片(81.5)纤维(18.5)	1~5 (84.0)5~10 (12.2)10~50 (3.8)	[40]
		臭氧	2230±104	2348±109	—	PET (30.2)PE (23.3)PP (14.5)PAM (10.8)	纤维(52.2)碎片(29.8)	1~5 (85.0)5~10 (14.0)10~50 (1.0)	[23]
		氯消毒	963±57	936±51	—	PET (53.8)PE (12.9)PP (12.7)PAM (12.6)	纤维(67.1)碎片(26.2)	1~5 (87.0)5~10 (13.5)
饮用水厂	捷克共和国	臭氧	243±17	224±3	—	醋酸纤维素(27.8)PET (20.5)PP (18.5)PE (15.6)	碎片(77.5)纤维(12.5)	1~5 (48.9)5~10 (33.1)10~50 (12.0)>50 (6.0)	[41]
		紫外线-氯消毒	149±1	151±4	—	醋酸纤维素(25.1)PET (21.9)PE (17.7)PP (17.0)	碎片(78.7)纤维(11.3)	1~5 (50.2)5~10 (33.0)10~50 (8.2)>50 (8.6)
	西班牙	氯消毒	0.06±0.04	0.06±0.04	—	PES (41.6)PP (37.7)PS (6.5)	纤维(54.6)碎片(45.4)	20~200 (14.0)200~500 (42.3)500~1000 (30.2)1000~2000 (13.5)	[42]
		电渗析-氯消毒	0.032±0.013	0.075±0.019	—	人造纤维素(53)PES (21)PE (16)PP (5)	碎片(53)纤维(37)薄膜(11)	50~100 (33.0)100~500 (67.0)	[43]
	柬埔寨	氯消毒	578	521±61	—	PET (28.8)PE (27.1)PP (8.5)PES/PA (6.8)	碎片(60.8)纤维(39.2)	6.5~20 (36.5)20~53 (32.4)53~500 (19.8)>500 (11.3)	[44]
		氯消毒	693	617±147	—	PET (26)PE (20.8)PA (10.4)PES (9.1)	碎片(53.4)纤维(46.6)	6.5~20 (42.0)20~53 (29.0)53~500 (19.9)>500 (9.1)	[44]
	印度	预氯化消毒	17.88	17.53	—	PET (56)PE (33)	纤维(55)碎片/薄膜(45)	<25 (29.9)25~50 (16.9)50~100 (50.3)>100 (2.8)	[45]
饮用水厂	印度尼西亚	氯消毒	13.8	12.3	黑色(50.4)黄色(18.7)红色(16.3)蓝色(14.6)	PESPEPP	纤维(92.8)碎片(7.2)	1~100 (14.5)101~350 (25.4)351~1000 (39.9)1001~5000 (20.3)	[46]
		氯消毒	29.7	8.5	黑色(38.8)蓝色(27.1)红色(12.2)黄色(15.3)	PESPEPP	纤维(96)碎片(4)	1~100 (10.4)101~350 (20.2)351~1000 (38.4)1001~5000 (31.0)	[46]

), ArticleFig(id=1241408724854690497, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, language=EN, label=Table 2, caption=

Comparison of THMFP values generated by chlorination of MP-DOM with typical aquatic NOM and AOM

, figureFileSmall=null, figureFileBig=null, tableContent=

有机物种类	来源	反应时间(d)	温度(℃)	THMFP(µg-THM/mg-C)	文献
MP-DOM	PP	7	25	81.1–82.1	[96]
	PS	7	25	76.8–82.3	[96]
	PE	4	25	80.48±4.53	[91]
	PS	4	25	125.48±8.90	[91]
	EPS和PVC(原始)	3	25	110.05±9.05	[97]
	EPS和PVC(老化)	3	25	135.6±13.4	[97]
	PE和PP(黑暗)	3	25	1.9–109.6	[90]
	PE和PP(光照)	3	25	29.2–453.3	[90]
NOM	地下水	1	25	47.1	[98]
	湖岸滤液	7	25±2	54.2±16.0	[99]
AOM	小球藻	7	25	10.1–12.1	[100]
	微囊藻	7	20	42.6±3.3	[101]

), ArticleFig(id=1241408725022462675, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241408714704475058, language=CN, label=表2, caption=

MP-DOM与典型水生NOM、AOM氯化生成的THMFP值比较

, figureFileSmall=null, figureFileBig=null, tableContent=

有机物种类	来源	反应时间(d)	温度(℃)	THMFP(µg-THM/mg-C)	文献
MP-DOM	PP	7	25	81.1–82.1	[96]
	PS	7	25	76.8–82.3	[96]
	PE	4	25	80.48±4.53	[91]
	PS	4	25	125.48±8.90	[91]
	EPS和PVC(原始)	3	25	110.05±9.05	[97]
	EPS和PVC(老化)	3	25	135.6±13.4	[97]
	PE和PP(黑暗)	3	25	1.9–109.6	[90]
	PE和PP(光照)	3	25	29.2–453.3	[90]
NOM	地下水	1	25	47.1	[98]
	湖岸滤液	7	25±2	54.2±16.0	[99]
AOM	小球藻	7	25	10.1–12.1	[100]
	微囊藻	7	20	42.6±3.3	[101]

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