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Based on the second level sounding data and routine environmental meteorological monitoring data from four regions(Chengdu, Yibin, Dazhou, and Chongqing) of the Sichuan Basin, during the winter of 2014~2017, combined with Mie scattering liDAR detection data in Chengdu during the same period, the boundary layer structure was identified by atmospheric extinction coefficient profile, and the evolution characteristics and pollution effects of atmospheric boundary layer inversion during haze weather were investigated. The results indicated that: Surface Layer Inversion (SLI), Mixed Layer Inversion (MLI), and Aerosol Boundary Layer Inversion (ABI) represented the three fundamental forms of boundary layer inversion. They showed a gradually weakened trend from bottom up and mark spatial variation among different regions. With the evolution of haze events from the formation phase to the persistence phase, the frequency of the three-layer inversions significantly increased. In the process, the intensity and thickness of SLI gradually decreased. However, the intensity and thickness of MLI exhibited quite opposite trend. In the meantime, the base height of MLI also decreased. The intensity and thickness of ABI fluctuated all the time. The coexistence and co-evolution of SLI and MLI not only strongly inhibited the vertical dispersion of ground pollutants, but also contributed to the increased near-surface humidity, which in turn induced the accumulation of particulate matter at the surface and enhanced aerosol hygroscopic properties, thereby reducing ground-level visibility. The above results revealed complex evolutionary patterns of boundary layer inversion during haze episodes in the Sichuan Basin from a new perspective and lay the foundation for integrated studies on the tropospheric lower-level inversion.
, correspAuthors=Liu YANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, authorCompany=null, fund=null, authors=null, authorsList=Li-yuan HE, Liu YANG, Yao ZHU, Chang-jian NI), CN=ArticleExt(id=1241049967641555886, articleId=1241049964210615177, tenantId=1146029695717560320, journalId=1234093305789726721, language=CN, title=四川盆地霾过程边界层逆温的演化特征及其污染效应, columnId=1234106388364981004, journalTitle=中国环境科学, columnName=大气污染与控制, runingTitle=null, highlight=null, articleAbstract=
利用四川盆地2014~2017年冬季4个地区(成都、宜宾、达州和重庆)的秒级探空资料和常规环境气象监测数据,结合同期成都的Mie散射激光雷达探测资料,通过大气消光系数廓线识别边界层结构,探究了霾天气过程中大气边界层逆温演化特征及其污染效应.结果表明:贴地逆温(SLI)、混合层顶逆温(MLI)以及气溶胶分界层逆温(ABI)是边界层逆温的3种基本形态.三层逆温一致表现为自下而上逐渐减弱的形态特征,但在地区之间呈现出明显的空间分异性.随着霾从形成期向发展期和持续期的渐进演化,三层逆温的发生频率显著上升,SLI的强度和厚度逐渐减小,MLI的强度和厚度则不断增加,底高也随之降低,ABI的强度和厚度呈波动变化.SLI和MLI的共存及其协同演变不仅强烈地抑制了地面污染物的垂直扩散,而且有利于近地面湿度的增加,进而诱发地面颗粒物的积聚以及吸湿性的增强,从而导致地面能见度降低.上述成果从新的视角揭示了四川盆地霾过程边界层逆温的复杂演化形态及其影响,也为后续针对对流层低层逆温的一体化研究奠定了基础.
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44(7):76-83., articleTitle=Research on the relationship between mixed layer height and aerosol layer height in Chengdu, refAbstract=null)], funds=[Fund(id=1241049984171307582, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, awardId=2023YFC3709301, language=CN, fundingSource=国家重点研发计划(2023YFC3709301), fundOrder=null, country=null), Fund(id=1241049984355856970, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, awardId=2024NSFSC1983, language=CN, fundingSource=四川省科技教育联合基金项目(2024NSFSC1983), fundOrder=null, country=null)], companyList=[AuthorCompany(id=1241049967935157174, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, xref=1., ext=[AuthorCompanyExt(id=1241049967943545783, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, companyId=1241049967935157174, language=EN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=
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Location of the four radiosonde stations in the Sichuan Basin, figureFileSmall=bHshKY+XwnYIlwwm+WtIWg==, figureFileBig=NlimfNceLgULLISE4wvkjg==, tableContent=null), ArticleFig(id=1241049976218906860, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=图1, caption=
四川盆地4个探空站点地理位置, figureFileSmall=bHshKY+XwnYIlwwm+WtIWg==, figureFileBig=NlimfNceLgULLISE4wvkjg==, tableContent=null), ArticleFig(id=1241049976680280337, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Fig.2, caption=
Conceptual model of the spatial relationship between boundary layer inversion and atmospheric extinction coefficient, figureFileSmall=6LzueR8A/l0K3DX5CXJjRQ==, figureFileBig=wLuVbExjcSQWl5efZGtPjQ==, tableContent=null), ArticleFig(id=1241049976860635424, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=图2, caption=
边界层逆温与大气消光系数配置关系的概念模型, figureFileSmall=6LzueR8A/l0K3DX5CXJjRQ==, figureFileBig=wLuVbExjcSQWl5efZGtPjQ==, tableContent=null), ArticleFig(id=1241049978521579831, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Fig.3, caption=
Statistical characteristics of inversions during winter haze events in different regions in the Sichuan Basin from 2014 to 2017, figureFileSmall=hZdYzGvUROJVWPjnr6iA+Q==, figureFileBig=jJbdHAYxsZw1uM8jKO1Q8Q==, tableContent=null), ArticleFig(id=1241049978647408957, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=图3, caption=
2014~2017年四川盆地冬季霾过程不同地区的逆温统计特征, figureFileSmall=hZdYzGvUROJVWPjnr6iA+Q==, figureFileBig=jJbdHAYxsZw1uM8jKO1Q8Q==, tableContent=null), ArticleFig(id=1241049978794209611, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Fig.4, caption=
The correlation coefficients between indices of three-layer inversions and visibility, figureFileSmall=fuVuBtk2pw++Vhqy2jLb+g==, figureFileBig=yN+B+C8HsfDM27W9Ju/AcA==, tableContent=null), ArticleFig(id=1241049979217834335, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=图4, caption=
三层逆温指标与能见度之间的相关系数, figureFileSmall=fuVuBtk2pw++Vhqy2jLb+g==, figureFileBig=yN+B+C8HsfDM27W9Ju/AcA==, tableContent=null), ArticleFig(id=1241049979565961587, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Fig.5, caption=
Variations of PM2.5 mass concentration and relative humidity during haze events, figureFileSmall=0f7L/AekVrs18UcCsUSuEA==, figureFileBig=/v7J8XsNOCgy/7zPONQ+SA==, tableContent=null), ArticleFig(id=1241049980111221116, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=图5, caption=
霾过程PM2.5质量浓度和相对湿度的变化, figureFileSmall=0f7L/AekVrs18UcCsUSuEA==, figureFileBig=/v7J8XsNOCgy/7zPONQ+SA==, tableContent=null), ArticleFig(id=1241049980467736968, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Table 1, caption=
Statistical characteristics of boundary layer inversion during winter haze events in the Sichuan Basin from 2014 to 2017
, figureFileSmall=null, figureFileBig=null, tableContent=
| 逆温类型 | 强度(℃/100m) | 厚度(m) | 频率(%) |
|---|
| SLI | 1.31 | 104 | 47.0 |
| MLI | 0.54 | 89 | 26.7 |
| ABI | 0.49 | 86 | 22.9 |
), ArticleFig(id=1241049980601954710, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=表1, caption=
四川盆地2014~2017年冬季霾过程边界层逆温统计特征
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| 逆温类型 | 强度(℃/100m) | 厚度(m) | 频率(%) |
|---|
| SLI | 1.31 | 104 | 47.0 |
| MLI | 0.54 | 89 | 26.7 |
| ABI | 0.49 | 86 | 22.9 |
), ArticleFig(id=1241049980715200930, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Table 2, caption=
The boundary layer inversion characteristics during winter haze events in the Sichuan Basin at different time from 2014 to 2017
, figureFileSmall=null, figureFileBig=null, tableContent=
| 逆温类型 | 08:00 | 20:00 |
|---|
| 强度(℃/100m) | 厚度(m) | 频率(%) | 强度(℃/100m) | 厚度(m) | 频率(%) |
|---|
| SLI | 1.28 | 131 | 51.8 | 1.34 | 77 | 42.3 |
| MLI | 0.62 | 102 | 37.2 | 0.46 | 75 | 16.1 |
| ABI | 0.53 | 84 | 21.6 | 0.45 | 89 | 23.9 |
), ArticleFig(id=1241049980874584495, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=表2, caption=
四川盆地2014~2017年冬季霾过程不同时次边界层逆温特征
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| 逆温类型 | 08:00 | 20:00 |
|---|
| 强度(℃/100m) | 厚度(m) | 频率(%) | 强度(℃/100m) | 厚度(m) | 频率(%) |
|---|
| SLI | 1.28 | 131 | 51.8 | 1.34 | 77 | 42.3 |
| MLI | 0.62 | 102 | 37.2 | 0.46 | 75 | 16.1 |
| ABI | 0.53 | 84 | 21.6 | 0.45 | 89 | 23.9 |
), ArticleFig(id=1241049981025579452, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Table 3, caption=
The temporal evolution characteristics of the frequency of inversion of the boundary layer during haze events (%)
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| 霾过程 | SLI | MLI | ABI |
|---|
| 形成期 | 21.2 | 15.5 | 22.6 |
| 发展期 | 31.0 | 23.0 | 25.6 |
| 持续期 | 38.4 | 46.0 | 34.3 |
| 消亡期 | 9.4 | 15.5 | 17.5 |
), ArticleFig(id=1241049981273043399, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=表3, caption=
霾过程边界层逆温发生频率的时间演变特征(%)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | SLI | MLI | ABI |
|---|
| 形成期 | 21.2 | 15.5 | 22.6 |
| 发展期 | 31.0 | 23.0 | 25.6 |
| 持续期 | 38.4 | 46.0 | 34.3 |
| 消亡期 | 9.4 | 15.5 | 17.5 |
), ArticleFig(id=1241049981398872534, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Table 4, caption=
The temporal evolution characteristics of boundary layer Inversion mean strength during haze events (℃/100m)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | SLI | MLI | ABI |
|---|
| 形成期 | 1.44 | 0.52 | 0.63 |
| 发展期 | 1.40 | 0.57 | 0.41 |
| 持续期 | 1.26 | 0.61 | 0.47 |
| 消亡期 | 1.04 | 0.48 | 0.41 |
), ArticleFig(id=1241049983026262500, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=表4, caption=
霾过程边界层逆温平均强度的时间演变特征(℃/100m)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | SLI | MLI | ABI |
|---|
| 形成期 | 1.44 | 0.52 | 0.63 |
| 发展期 | 1.40 | 0.57 | 0.41 |
| 持续期 | 1.26 | 0.61 | 0.47 |
| 消亡期 | 1.04 | 0.48 | 0.41 |
), ArticleFig(id=1241049983227589102, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Table 5, caption=
The temporal evolution characteristics of boundary layer Inversion mean thickness during haze events (m)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | SLI | MLI | ABI |
|---|
| 形成期 | 115 | 77 | 99 |
| 发展期 | 110 | 85 | 68 |
| 持续期 | 103 | 98 | 91 |
| 消亡期 | 79 | 92 | 79 |
), ArticleFig(id=1241049983546356224, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=表5, caption=
霾过程边界层逆温平均厚度的时间演变特征(m)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | SLI | MLI | ABI |
|---|
| 形成期 | 115 | 77 | 99 |
| 发展期 | 110 | 85 | 68 |
| 持续期 | 103 | 98 | 91 |
| 消亡期 | 79 | 92 | 79 |
), ArticleFig(id=1241049983793820182, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=EN, label=Table 6, caption=
The temporal evolution characteristics of boundary layer Inversion mean height during haze events (m)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | MLI底高 | ABI底高 | MLI顶高 | ABI顶高 |
|---|
| 形成期 | 284 | 918 | 361 | 1017 |
| 发展期 | 258 | 978 | 343 | 1046 |
| 持续期 | 240 | 999 | 338 | 1090 |
| 消亡期 | 245 | 937 | 337 | 1016 |
), ArticleFig(id=1241049984020312618, tenantId=1146029695717560320, journalId=1234093305789726721, articleId=1241049964210615177, language=CN, label=表6, caption=
霾过程边界层逆温平均高度的时间演变特征(m)
, figureFileSmall=null, figureFileBig=null, tableContent=
| 霾过程 | MLI底高 | ABI底高 | MLI顶高 | ABI顶高 |
|---|
| 形成期 | 284 | 918 | 361 | 1017 |
| 发展期 | 258 | 978 | 343 | 1046 |
| 持续期 | 240 | 999 | 338 | 1090 |
| 消亡期 | 245 | 937 | 337 | 1016 |
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