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In order to improve the leaching efficiency of chalcopyrite, on the basis of the conventional heating leaching system, the pulse microbubble method is introduced to reduce the influence of the sulfide layer by improving the mass transfer efficiency in the leaching process. The kinetics is discussed, the morphology of the leaching residue is analyzed, and the mechanism of pulse microbubble-enhanced leaching is revealed. The results show that the pulsed microbubbles can significantly improve the leaching rate of chalcopyrite, and the increase rate rises with the decrease in microbubble size. Under the optimum conditions of conventional leaching, the copper leaching rate is only 53.6%, while under the same conditions, the copper leaching rate can increase to 62.48% and 80.40% when the pore size of the orifice plate is 94 and 75 μm, respectively. The SEM test results show that the pulsed microbubbles can effectively improve the aggregation degree and coverage area of the sulfide layer on the surface of chalcopyrite. The mechanism may be that the pulsed microbubbles have higher mass transfer efficiency and can accelerate the reaction rate. At the same time, the local high temperature and high pressure released during the burst can weaken the passivation of the sulfide layer during the leaching process, thereby improving the leaching effect of chalcopyrite.

, authors=Mengheng LUO^{1, 2}, Siyuan YANG¹, Xinghai CHEN^{1, 3}, Lingyun HUANG², Cheng LIU^{1, 2}, authorsList=Mengheng LUO, Siyuan YANG, Xinghai CHEN, Lingyun HUANG, Cheng LIU, authorCompany=null, correspAuthors=Siyuan YANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1305178374482191260, articleId=1305178374029206426, tenantId=1146029695717560320, journalId=1146120122248306696, language=CN, title=脉冲微泡强化黄铜矿浸出机制研究, columnId=1152626641328501305, journalTitle=湿法冶金, columnName=试验研究, runingTitle=null, highlight=null, articleAbstract=

为提高黄铜矿浸出效率，研究了在常规加热浸出体系的基础上，引入脉冲微泡手段，通过提高浸出过程中传质效率，降低硫化层的影响。探讨了动力学，分析了浸出渣形貌，揭示了脉冲微泡强化浸出的作用机制。研究结果表明：脉冲微泡体可显著提高黄铜矿浸出率，且提升幅度随微泡尺寸减小而增加；常规浸出最佳条件下铜浸出率仅为53.6%，而在相同条件下，孔板孔径尺寸分别为94、75μm时的铜浸出率可提高至62.48%和80.40%。SEM检测结果表明，脉冲微泡可有效改善硫化层在黄铜矿表面的聚集程度与覆盖面积，其作用机制可能是由于脉冲微泡具有较高的传质效率，能使反应速率加快，同时其破灭时释放的局部高温高压能削弱浸出过程的硫化层钝化作用，从而提高黄铜矿浸出效果。

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罗梦恒（2001—），男，硕士，主要研究方向为湿法冶金。

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罗梦恒（2001—），男，硕士，主要研究方向为湿法冶金。

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