Article(id=1308543990476137395, tenantId=1146029695717560320, journalId=1146120122248306696, issueId=1308543982137860950, articleNumber=null, orderNo=null, doi=10.13355/j.cnki.sfyj.2025.05.008, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1742832000000, receivedDateStr=2025-03-25, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1789910798900, onlineDateStr=2026-09-20, pubDate=1760889600000, pubDateStr=2025-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1789910798900, onlineIssueDateStr=2026-09-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1789910798900, creator=13701087609, updateTime=1789910798900, updator=13701087609, issue=Issue{id=1308543982137860950, tenantId=1146029695717560320, journalId=1146120122248306696, year='2025', volume='44', issue='5', pageStart='583', pageEnd='705', issueExtLink='null', onlineDate='null', pubDate='1760889600000', pubDateStr='2025-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1789910796911, creator='13701087609', updateTime=1789955335202, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1308730789341266049, tenantId=1146029695717560320, journalId=1146120122248306696, issueId=1308543982137860950, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1308730789341266050, tenantId=1146029695717560320, journalId=1146120122248306696, issueId=1308543982137860950, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=635, endPage=644, ext={EN=ArticleExt(id=1308543990706824116, articleId=1308543990476137395, tenantId=1146029695717560320, journalId=1146120122248306696, language=EN, title=Removal Effect and Mechanism of Phosphate-modified Nitrogen-doped Biochar for Uranium, columnId=1152626641181700664, journalTitle=Hydrometallurgy of China, columnName=Experiment Research, runingTitle=null, highlight=null, articleAbstract=

The original biochar (BC) was prepared by pyrolysis using chestnut shells as raw materials, and then the phosphate-modified nitrogen-doped biochar (NP-BC) was prepared by nitrogen doping and phosphate modification methods. The adsorption performance of BC and NP-BC for uranium in wastewater was investigated. The surface morphology and elements of BC and NP-BC were analyzed by means of SEM, EDS, BET, FT-IR and XPS, and the adsorption mechanism of BC and NP-BC for uranium was discussed. The results show that for the wastewater with an initial mass concentration of uranium of 10 mg/L and initial pH of 4, under the conditions of NP-BC dosage of 0.2 g/L and reaction temperature of 30 ℃, the adsorption removal rate of U(Ⅵ) can reach 99.32%. The influence of coexisting anions and cations on the division of U(Ⅵ) in NP-BC increases with the increase of ion concentration. The adsorption process is more suitable to be described by the pseudo-second-order kinetic model and the Langmuir isothermal adsorption model. It is concluded through FT-IR and XPS analysis that the adsorption mechanism of uranium by NP-BC is the coordination effect and reduction effect of oxygen-containing functional groups, nitrogen-containing functional groups and phosphate groups.

, authors=Zhiyu XIONG, Yuemei MAO, Shiyou LI, Jiayao LIU, Qiqi DENG, Taotao ZENG, authorsList=Zhiyu XIONG, Yuemei MAO, Shiyou LI, Jiayao LIU, Qiqi DENG, Taotao ZENG, authorCompany=null, correspAuthors=Taotao ZENG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1308543991159808949, articleId=1308543990476137395, tenantId=1146029695717560320, journalId=1146120122248306696, language=CN, title=磷酸盐改性氮掺杂生物炭除铀效果及机制研究, columnId=1152626641328501305, journalTitle=湿法冶金, columnName=试验研究, runingTitle=null, highlight=null, articleAbstract=

研究了以板栗壳为原料，先用热解法制备原始生物炭（BC），再用氮掺杂和磷酸盐改性法制备磷酸盐改性氮掺杂生物炭（NP-BC）。考察了BC和NP-BC对废水中铀的吸附性能，通过SEM、EDS、BET、FT-IR和XPS等手段分析了BC和NP-BC的表面形貌和元素，探讨了BC和NP-BC对铀的吸附机制。结果表明：针对铀初始质量浓度10 mg/L、初始pH=4的废水，在NP-BC投加量0.2 g/L、反应温度30 ℃条件下，U（Ⅵ）吸附去除率达99.32%；共存阴、阳离子对NP-BC除U（Ⅵ）的影响随离子浓度增大而增强；吸附过程更适宜用准二级动力学模型和Langmuir等温吸附模型描述；通过FT-IR和XPS分析得出，NP-BC对铀的吸附机制为含氧官能团、含氮官能团和磷酸基团的配合作用及还原作用。

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熊芷毓（1999—），女，硕士研究生，主要研究方向为铀废水处理。

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熊芷毓（1999—），女，硕士研究生，主要研究方向为铀废水处理。

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