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Green hydrogen has become an important technological option for building a diversified green energy structure and plays a key role in achieving carbon neutrality goals. This article aims to review the research and development progress of green hydrogen production technology. Based on the current development status and policy background of China’s hydrogen energy industry, this article defined green hydrogen according to the Chinese and international research and development status and focused on hydrogen production from renewable energy water splitting and biomass. The technical characteristics, advantages, and challenges of these technologies were analyzed. Additionally, technologies such as hydrogen production by nuclear energy, methane pyrolysis, green ammonia, and aqua hydrogen, which do not belong to traditional green hydrogen but may play an important role in carbon emission reduction, were explored. Finally, the article summarized the issues existing in green hydrogen production and provided suggestions for the development of green hydrogen in China from aspects such as policy incentives, technological innovation, and market application.
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绿氢已经成为构建多元绿色能源结构的重要技术选项，在实现“碳达峰与碳中和”目标进程中具有关键作用。文章旨在综述绿氢生产技术的研发进展和发展趋势。根据中国氢能产业的发展现状和政策背景，界定了适合于国内外研发现状的绿氢定义，重点介绍了可再生能源分解水制氢、生物质制氢技术，分析了各自的技术特点、优势和挑战。此外，还探讨了核能制氢、甲烷热解制氢、绿氨制氢和水氢等虽不属于传统的绿氢，但有可能对碳减排起到重要作用的技术。最后，对绿氢生产中存在的问题进行了总结，从政策激励、技术创新、市场应用等方面对中国绿氢发展给出了建议。
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 |
党成雄，副教授。主要从事生物质热化学制氢、CO2捕获与催化转化、钙基化学链的构建与应用等领域的研究。主持国家自然科学基金、广东省自然科学基金等项目5项。获2020年中国颗粒学会优秀博士论文奖等。发表论文29篇。电子信箱：cxdang@gzhu.edu.cn。 |
 |
余皓，教授，博士研究生导师。华南理工大学化学与化工学院副院长。中国颗粒学会理事，广东省化工学会副秘书长，科普与学术工作委员会主任委员。主要从事纳米碳材料、多相催化等研究。获教育部新世纪优秀人才、广东省自然科学基金杰出青年基金、广东省“千百十”省级培养对象、广州市珠江科技新星、全国石油化工青年教学名师。广东省线上线下混合本科一流课程《化学反应工程》课程负责人。获教育部自然科学奖一等奖、二等奖，中国石油和化学工业联合会科技进步奖一等奖。发表论文200余篇。电子信箱：yuhao@scut.edu.cn。 |
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党成雄，副教授。主要从事生物质热化学制氢、CO2捕获与催化转化、钙基化学链的构建与应用等领域的研究。主持国家自然科学基金、广东省自然科学基金等项目5项。获2020年中国颗粒学会优秀博士论文奖等。发表论文29篇。电子信箱：cxdang@gzhu.edu.cn。
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党成雄，副教授。主要从事生物质热化学制氢、CO2捕获与催化转化、钙基化学链的构建与应用等领域的研究。主持国家自然科学基金、广东省自然科学基金等项目5项。获2020年中国颗粒学会优秀博士论文奖等。发表论文29篇。电子信箱：cxdang@gzhu.edu.cn。
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余皓，教授，博士研究生导师。华南理工大学化学与化工学院副院长。中国颗粒学会理事，广东省化工学会副秘书长，科普与学术工作委员会主任委员。主要从事纳米碳材料、多相催化等研究。获教育部新世纪优秀人才、广东省自然科学基金杰出青年基金、广东省“千百十”省级培养对象、广州市珠江科技新星、全国石油化工青年教学名师。广东省线上线下混合本科一流课程《化学反应工程》课程负责人。获教育部自然科学奖一等奖、二等奖，中国石油和化学工业联合会科技进步奖一等奖。发表论文200余篇。电子信箱：yuhao@scut.edu.cn。
"}, bioImg=BZjA4OgjRqC39dB1FTm1bw==, bioContent=
余皓，教授，博士研究生导师。华南理工大学化学与化工学院副院长。中国颗粒学会理事，广东省化工学会副秘书长，科普与学术工作委员会主任委员。主要从事纳米碳材料、多相催化等研究。获教育部新世纪优秀人才、广东省自然科学基金杰出青年基金、广东省“千百十”省级培养对象、广州市珠江科技新星、全国石油化工青年教学名师。广东省线上线下混合本科一流课程《化学反应工程》课程负责人。获教育部自然科学奖一等奖、二等奖，中国石油和化学工业联合会科技进步奖一等奖。发表论文200余篇。电子信箱：yuhao@scut.edu.cn。
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The ammonia industry has made outstanding contributions to human food security and economic and social development, while also causing a large amount of carbon dioxide emissions in the production process. Green ammonia produced using renewable energy has the characteristic of “zero carbon” and significant carbon reduction effects throughout its lifecycle. It has become one of the hotspots for low-carbon industry development worldwide. this paper introduces the policies of the green ammonia industry, the current development status and progress of the green ammonia industry, and analyzes the market competitiveness of green ammonia in four downstream applications such as vehicle and ship fuel, hydrogen storage carriers, fuel power generation, and chemical raw materials. It is considered that the major global ship engine technology companies and ship manufacturers are developing ammonia fuel engines and ammonia powered ships which are gradually conducting operational tests. And the ammonia fuel engines for vehicles have achieved breakthroughs in related technologies in China. It is believed that ocean shipping is the first breakthrough area for green ammonia, and when the price of green electricity drops to around 0.20CNY/kWh with the advancement of new energy technology, global green ammonia vehicle and ship fuel will usher in significant development. Green ammonia will become increasingly cost competitive in the heavy-duty truck and ocean shipping industries. At the same time, ammonia has great potential for development as a hydrogen storage carrier. The cost of liquid ammonia synthesis and dehydrogenation accounts for over 85% of the total cost, and it is not sensitive to transportation distance. In the future, it will become one of the main forms of global long-distance transportation of bulk hydrogen. The sustainable development of the green ammonia industry requires support from technological innovation, industrial policies, and standard formulation.
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Nuclear hydrogen production is one of the most prospective approaches for efficient, massive and CO2-free hydrogen production, while the high temperature gas cooled reactor (HTGR) which has been intensively developed in China is considered as the most suitable reactor type for nuclear hydrogen production. Currently, the HTGR demonstration plant, HTR-PM, is under construction under the framework of the National Science and Technology Major Project. The principles and main routes for nuclear hydrogen production, including the iodine-sulfur thermochemical water-splitting process, the hybrid sulfur process, as well as the high temperature steam electrolysis, are introduced. The progress of the nuclear hydrogen production technologies both in the world and China are shortly presented and reviewed, and its safety analysis and techno-economic assessment are discussed. In addition, the potential technologies for coupling to the reactor are discussed, and the industrial application of the nuclear hydrogen production based on HTGR is prospected, taking steelmaking by hydrogen as an example. Finally, the development strategy and prospects of nuclear hydrogen production technology in China are proposed.
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10.1016/j.coelec.2023.101255., articleTitle=Electrolysis of lignin for production of chemicals and hydrogen, refAbstract=null)], funds=[Fund(id=1242114001560212443, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, awardId=22078106, language=CN, fundingSource=国家自然科学基金(22078106), fundOrder=null, country=null), Fund(id=1242114001627321308, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, awardId=2024B1515040016, language=CN, fundingSource=广东省自然科学基金(2024B1515040016), fundOrder=null, country=null)], companyList=[AuthorCompany(id=1242113997680481195, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, xref=null, ext=[AuthorCompanyExt(id=1242113997693064108, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, companyId=1242113997680481195, language=EN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=1. School of Chemistry and Chemical Engineering, Guangzhou University, Guangzhou 510006, China), AuthorCompanyExt(id=1242113997697258413, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, companyId=1242113997680481195, language=CN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=1.广州大学化学化工学院，广州 510006)]), AuthorCompany(id=1242113997764367278, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, xref=null, ext=[AuthorCompanyExt(id=1242113997768561583, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, companyId=1242113997764367278, language=EN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=2. School of Chemistry and Chemical Engineering, South China University of Technology, Guangzhou 510641, China), AuthorCompanyExt(id=1242113997776950192, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, companyId=1242113997764367278, language=CN, country=null, province=null, city=null, postcode=null, companyName=null, departmentName=null, remark=2.华南理工大学化学与化工学院，广州 510641)])], figs=[ArticleFig(id=1242113999580500949, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, language=EN, label=Fig. 1, caption=
Principles of four typical water electrolysis technologies for hydrogen production, figureFileSmall=jdOGxGNCm1vrdQYU27nUeA==, figureFileBig=L9m5xFCCUzn9ulrLv1H4QQ==, tableContent=null), ArticleFig(id=1242113999643415510, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, language=CN, label=图1, caption=
4种典型电解水制氢技术原理示意图, figureFileSmall=jdOGxGNCm1vrdQYU27nUeA==, figureFileBig=L9m5xFCCUzn9ulrLv1H4QQ==, tableContent=null), ArticleFig(id=1242114001178530775, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, language=EN, label=Fig. 2, caption=
Chemical-looping hydrogen production from partial oxidation of biomass and complete oxidation of biomass, figureFileSmall=xydu98cE8bbnU74NwBk1oA==, figureFileBig=8kY/6GqGcJSyDEl4i1TdOg==, tableContent=null), ArticleFig(id=1242114001233056728, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, language=CN, label=图2, caption=
生物质部分氧化和生物质完全氧化化学链制氢示意图 CLRB：Chemical Looping Reforming of Biomass，化学循环生物质重整。
, figureFileSmall=xydu98cE8bbnU74NwBk1oA==, figureFileBig=8kY/6GqGcJSyDEl4i1TdOg==, tableContent=null), ArticleFig(id=1242114001308554201, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, language=EN, label=Table 1, caption=
Comparison of technical parameters for hydrogen production through water electrolysis
, figureFileSmall=null, figureFileBig=null, tableContent=
| 项目 | AWE | PEMWE | AEMWE | SOWE |
| 电解质 | 氢氧化钾溶液 | PFSA膜 | 阴离子交换膜 | 钇稳定的氧化锆 |
| 阴极材料 | 镍基材料 | 铂基材料 | 镍基材料 | Ni/YSZ |
| 阳极材料 | 镍基材料 | 钌或铱基材料 | 镍、铁、钴氧化物 | YSZ |
| 操作温度/oC | 70~90 | 50~80 | 40~60 | 700~850 |
| 操作压力/MPa | 小于3 | 小于7 | 小于3.5 | 0.1 |
| 运行寿命/kh | 60~100 | 20~60 | <小于10 | — |
电流密度/
(A·cm-2) | 0.2~0.8 | 1.0~2.0 | 0.2~2.0 | 0.3~1.0 |
| 效率/% | 50~78 | 50~83 | 57~59 | 89 |
| 电压/V | 1.4~3.0 | 1.4~2.5 | 1.4~2.0 | 1.0~1.5 |
| 技术成熟度 | 成熟工业化 | 商业化过程中 | 示范装置 | 示范装置 |
| 优点 | 已成熟工业化、无贵金属电催化剂、成本相对较低、长期稳定性 | 商业化技术、高电流密度、气体纯度高、反应器紧凑、响应迅速 | 无贵金属电催化剂、低浓度（1 mol/L KOH）液体电解质 | 效率高、效率更高 |
| 缺点 | 电流密度有限、气体交叉（渗透）、高浓度碱电解质 | 电池组件成本高、贵金属电催化剂、酸性电解质 | 稳定性不够、尚在研发过程中 | 稳定性不够、尚在研发过程中 |
), ArticleFig(id=1242114001388245978, tenantId=1146029695717560320, journalId=1146032081894723586, articleId=1157002943091270418, language=CN, label=表1, caption=
电解水制氢技术参数对比
, figureFileSmall=null, figureFileBig=null, tableContent=
| 项目 | AWE | PEMWE | AEMWE | SOWE |
| 电解质 | 氢氧化钾溶液 | PFSA膜 | 阴离子交换膜 | 钇稳定的氧化锆 |
| 阴极材料 | 镍基材料 | 铂基材料 | 镍基材料 | Ni/YSZ |
| 阳极材料 | 镍基材料 | 钌或铱基材料 | 镍、铁、钴氧化物 | YSZ |
| 操作温度/oC | 70~90 | 50~80 | 40~60 | 700~850 |
| 操作压力/MPa | 小于3 | 小于7 | 小于3.5 | 0.1 |
| 运行寿命/kh | 60~100 | 20~60 | <小于10 | — |
电流密度/
(A·cm-2) | 0.2~0.8 | 1.0~2.0 | 0.2~2.0 | 0.3~1.0 |
| 效率/% | 50~78 | 50~83 | 57~59 | 89 |
| 电压/V | 1.4~3.0 | 1.4~2.5 | 1.4~2.0 | 1.0~1.5 |
| 技术成熟度 | 成熟工业化 | 商业化过程中 | 示范装置 | 示范装置 |
| 优点 | 已成熟工业化、无贵金属电催化剂、成本相对较低、长期稳定性 | 商业化技术、高电流密度、气体纯度高、反应器紧凑、响应迅速 | 无贵金属电催化剂、低浓度（1 mol/L KOH）液体电解质 | 效率高、效率更高 |
| 缺点 | 电流密度有限、气体交叉（渗透）、高浓度碱电解质 | 电池组件成本高、贵金属电催化剂、酸性电解质 | 稳定性不够、尚在研发过程中 | 稳定性不够、尚在研发过程中 |
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