Article(id=1242135244682375841, tenantId=1146029695717560320, journalId=1146031591421210625, issueId=1242135205469823510, articleNumber=null, orderNo=15, doi=10.3981/j.issn.1000-7857.2016.18.009, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1433347200000, receivedDateStr=2015-06-04, revisedDate=1450281600000, revisedDateStr=2015-12-17, acceptedDate=null, acceptedDateStr=null, onlineDate=1477015793510, onlineDateStr=2016-10-21, pubDate=1474992000000, pubDateStr=2016-09-28, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1477015793510, onlineIssueDateStr=2016-10-21, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1774077720083, creator=sys-migrate, updateTime=1774077720083, updator=sys-migrate, issue=Issue{id=1242135205469823510, tenantId=1146029695717560320, journalId=1146031591421210625, year='2016', volume='34', issue='18', pageStart='1', pageEnd='320', issueExtLink='null', onlineDate='null', pubDate='1474992000000', pubDateStr='2016-09-28', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=3, issueType=-1, specialIssue=null, createTime=1774077710737, creator='sys-migrate', updateTime=1774077710737, updator='sys-migrate', preIssue=null, nextIssue=null, articleTotal=null, ext=null, issueFiles=null, downloadFileDto=null}, startPage=84, endPage=88, ext={EN=ArticleExt(id=1242135248784401050, articleId=1242135244682375841, tenantId=1146029695717560320, journalId=1146031591421210625, language=EN, title=Effects of femtosecond laser parameters on state populations of three-level ladder molecule, columnId=1242116080374710456, journalTitle=Science & Technology Review, columnName=Articles, runingTitle=null, highlight=null, articleAbstract=The effects of the pump intensity, the wavelength and the pulse width on the state populations of the three-level ladder K2 molecule driven by intense femtosecond pump-probe pulses are investigated by employing the time-dependent wave packet approach and are thus quantified. The Rabi oscillation is affected by the pump intensity, the wavelength and the pulse width, and its variation results in a periodical change of the populations in the ground state and the excited state. Quantifying their effects on the population of the excited state verifies the periodical nature and shows that the frequency varies with the increasing pump intensity and pulse width. The results illustrate that the needed population in the electronic state of interest can be obtained by controlling these parameters, which provides some important basis for light manipulation of molecular processes., authors=GUO Wei1,2 , FENG Xiaojing1 , authorsList=GUO Wei, FENG Xiaojing, authorCompany=1. School of Electrical Engineering, University of South China, Hengyang 421001, China;
2. State Key Laboratory of Molecular Reaction Dynamics;Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China, correspAuthors=null, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=unw8XQZ6bTpxcx8ctrb89g==, pdfFileSize=2288292, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1242135247651943087, articleId=1242135244682375841, tenantId=1146029695717560320, journalId=1146031591421210625, language=CN, title=飞秒激光参数对三态梯度型分子态布居数的影响, columnId=1146540929516700224, journalTitle=科技导报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=利用含时波包法研究并且首次量化了强飞秒泵浦-探测激光场中泵浦场强、泵浦波长和脉宽对三态梯度型K2 分子态布居数的影响。泵浦场强、泵浦波长和脉宽影响Rabi振荡,而Rabi振荡的变化又导致了基态和激发态布居数周期性变化。量化这3个激光场参数对激发态布居数的影响验证了此周期性变化规律,表明变化频率随着泵浦场强和脉宽的增大而变化。研究表明调节激光场参数可实现对态布居数的选择性分布,可以为实验上实现分子的光控制提供重要参考。, authors=郭玮1,2 , 冯小静1 , authorsList=郭玮, 冯小静, authorCompany=1. 南华大学电气工程学院, 衡阳 421001;
2. 中国科学院大连化学物理研究所;分子反应动力学国家重点实验室, 大连 116023, correspAuthors=null, authorNote=郭玮,副教授,研究方向为物理电子学,电子信箱:vella99@163.com;冯小静(共同第一作者),硕士研究生,研究方向为物理电子学,电子信箱:1012277640@qq.com, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=TXUP4F5y+F6gWwmJ489SOg==, pdfFileSize=2288292, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=国家自然科学基金项目(11447020);湖南省自然科学基金项目(2015JJ3104))}, authors=null, keywords=[Keyword(id=1242135247136043690, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=CN, orderNo=1, keyword=含时波包法), Keyword(id=1242135247228318379, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=CN, orderNo=1, keyword=三态梯度型K2 分子), Keyword(id=1242135247337370285, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=CN, orderNo=1, keyword=态布居数), Keyword(id=1242135247425450669, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=CN, orderNo=1, keyword=Rabi振荡), Keyword(id=1242135248419500730, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=EN, orderNo=1, keyword=time-dependent wave packet approach), Keyword(id=1242135248494998203, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=EN, orderNo=1, keyword=three-level K2 molecule), Keyword(id=1242135248570495677, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=EN, orderNo=1, keyword=state populations), Keyword(id=1242135248650187454, tenantId=1146029695717560320, journalId=1146031591421210625, articleId=1242135244682375841, language=EN, orderNo=1, keyword=Rabi oscillation)], refs=null, funds=null, companyList=null, figs=null, attaches=null, journal=Journal(id=1125356956822126595, delFlag=0, nameCn=科技导报, nameEn=Science & Technology Review, nameHistory1=null, nameHistory2=null, issn=1000-7857, eissn=, cn=11-1421/N, coden=null, periodic=3, language=CN, oaType=0, ccby=null, superviseOffice=null, ownerOffice=null, pubOffice=null, editorOffice=null, officeType=null, aims=null, clcCode=null, officeProv=null, officeCity=null, officeAddr=null, officeZip=null, officeEmail=null, officePhone=null, editDirector=null, officeDirector=null, officeDirectorPhone=null, officeStaffNum=null, officeEmpNum=null, coverPicUrl=wfghvu3bhh/dKxuZ+ucVHA==, journalPrice=null, startedYear=null, abbrevIsoEn=Sci Technol Rev, journalRemark=null, publicationField=null, createdTime=null, updatedTime=1774230116083, createdBy=null, updatedBy=13041195026, firstLetterCn=S, firstLetterEn=S, subjectCode=Natural Sciences, subjectName=自然科学, subjectCodeEn=Natural Sciences, subjectNameEn=null, picCn=wfghvu3bhh/dKxuZ+ucVHA==, picEn=yjSfclmpNm7ihn9NbTZ69g==, jcr=null, cjcr=null, exts=[JournalExt(id=1242774439910290156, language=CN, name=科技导报, nameHistory1=null, nameHistory2=null, managedBy=中国科学技术协会, sponsoredBy=中国科学技术协会, publishedBy=科技导报社, editorOffice=, officeProv=null, officeCity=null, officeAddr=, officeZip=, editDirector=, officeDirector=null, officePhone=null, coverPicUrl=null, journalRemark=, submitArticleUrl=null, websiteUrl=http://www.kjdb.org/CN/home, createdTime=1774230116107, updatedTime=1774230116107, createdBy=13041195026, updatedBy=13041195026, submissionGuidelinesUrl=http://www.kjdb.org/CN/column/column7.shtml, submissionAuthorUrl=https://kjdbauthor.cast.org.cn/webm, submissionEditorUrl=https://kjdbeditor.cast.org.cn/webm/, submissionReviewUrl=https://kjdbauthor.cast.org.cn/webm, submissionCeEditorUrl=https://kjdbeditor.cast.org.cn/webm/, submissionAeEditorUrl=https://kjdbeditor.cast.org.cn/webm/, option={"copyright":""}), JournalExt(id=1242774439960621805, language=EN, name=Science & Technology Review, nameHistory1=null, nameHistory2=null, managedBy=, sponsoredBy=, publishedBy=, editorOffice=, officeProv=null, officeCity=null, officeAddr=, officeZip=, editDirector=, officeDirector=null, officePhone=null, coverPicUrl=null, journalRemark=, submitArticleUrl=null, websiteUrl=http://www.kjdb.org/EN/home, createdTime=1774230116119, updatedTime=1774230116119, createdBy=13041195026, updatedBy=13041195026, submissionGuidelinesUrl=http://www.kjdb.org/EN/column/column7.shtml, submissionAuthorUrl=https://kjdbauthor.manuscriptcloud.com/login, submissionEditorUrl=https://kjdbeditor.manuscriptcloud.com/login, submissionReviewUrl=https://kjdbauthor.manuscriptcloud.com/login, submissionCeEditorUrl=https://kjdbeditor.manuscriptcloud.com/login, submissionAeEditorUrl=https://kjdbeditor.manuscriptcloud.com/login, option={"copyright":""})], databaseList=null, tenantJournalId=1146031591421210625, websiteList=[Website(id=1146104741081231361, webName=null, webTitle=null, webDomain=null, webCopyrigh=null, webIpcNo=null, seoTitle=null, seoKeywords=null, seoDescription=null, tenantJournalId=null, journalId=1146031591421210625, journalNameCn=null, journalNameEn=null, grayFlag=null, tenantId=1146029695717560320, platformId=null, journalGroupId=null, journalGroupNameCn=null, journalGroupNameEn=null, type=1, domain=https://castjournals.cast.org.cn/joweb/kjdb/CN, language=CN, createTime=1751182263881, createBy=18614031015, updateTime=1751778001962, updateBy=18614031015, name=科技导报, tplId=1146099689490845704, title=科技导报, delFlag=0, indexPage=/home, props=[WebsiteProps(id=1148021146403992296, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146104741081231361, code=articleTextType, value=kx, createTime=1751639170504, updateTime=1751639170504, creator=18614031015, updator=18614031015), WebsiteProps(id=1148021146378826469, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146104741081231361, code=banner, value=null, createTime=1751639170498, updateTime=1751639170498, creator=18614031015, updator=18614031015), WebsiteProps(id=1148021146366243556, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146104741081231361, code=logo, value=https://castjournals.cast.org.cn/joweb/kjdb/CN/file/pic?fileId=9GHSf7eGlIPH0Tv/OOdstA==, createTime=1751639170495, updateTime=1751639170495, creator=18614031015, updator=18614031015), WebsiteProps(id=1148021146395603687, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146104741081231361, code=picServerUrl, value=https://castjournals.cast.org.cn/joweb/kjdb/CN/file/pic, createTime=1751639170502, updateTime=1751639170502, creator=18614031015, updator=18614031015), WebsiteProps(id=1148021146387215078, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146104741081231361, code=staticResourcePath, value=https://castjournals.cast.org.cn/joweb/cast_kjdb_cn_619/, createTime=1751639170500, updateTime=1751639170500, creator=18614031015, updator=18614031015)]), Website(id=1146105254833139715, webName=null, webTitle=null, webDomain=null, webCopyrigh=null, webIpcNo=null, seoTitle=null, seoKeywords=null, seoDescription=null, tenantJournalId=null, journalId=1146031591421210625, journalNameCn=null, journalNameEn=null, grayFlag=null, tenantId=1146029695717560320, platformId=null, journalGroupId=null, journalGroupNameCn=null, journalGroupNameEn=null, type=1, domain=https://castjournals.cast.org.cn/joweb/kjdb/EN, language=EN, createTime=1751182386363, createBy=18614031015, updateTime=1753500121937, updateBy=18614031015, name=科技导报, tplId=1146101810881728533, title=Science & Technology Review, delFlag=0, indexPage=/home, props=[WebsiteProps(id=1155838567709528217, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146105254833139715, code=articleTextType, value=kx, createTime=1753502988984, updateTime=1753502988984, creator=18614031015, updator=18614031015), WebsiteProps(id=1155838567692750998, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146105254833139715, code=banner, value=null, createTime=1753502988980, updateTime=1753502988980, creator=18614031015, updator=18614031015), WebsiteProps(id=1155838567688556693, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146105254833139715, code=logo, value=https://castjournals.cast.org.cn/joweb/kjdb/EN/file/pic?fileId=9GHSf7eGlIPH0Tv/OOdstA==, createTime=1753502988979, updateTime=1753502988979, creator=18614031015, updator=18614031015), WebsiteProps(id=1155838567705333912, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146105254833139715, code=picServerUrl, value=https://castjournals.cast.org.cn/joweb/kjdb/EN/file/pic, createTime=1753502988983, updateTime=1753502988983, creator=18614031015, updator=18614031015), WebsiteProps(id=1155838567701139607, tenantId=1146029695717560320, journalId=null, journalGroupId=null, siteId=1146105254833139715, code=staticResourcePath, value=https://castjournals.cast.org.cn/joweb/cast_kjdb_en_623/, createTime=1753502988982, updateTime=1753502988982, creator=18614031015, updator=18614031015)])], journalTitle=科技导报, weixinUrl=null, journalUrl=null, iacademicId=null, status=1, seqNo=null, journalTitleEn=Science & Technology Review, journalPhotoCn=wfghvu3bhh/dKxuZ+ucVHA==, journalPhotoEn=yjSfclmpNm7ihn9NbTZ69g==, journalFirstLetter=S, journalRecommend=null, journalNew=null, journalCollection=1, jcrJf=null, cjcrJf=0.91, jcrJfStr=null, cjcrJfStr=null, submissionFirstDecision=null, sciSubjectClassification=null, casSubjectClassification=null, citeScore=null, totalCitationFrequency=null, icpCode=null, psCode=null, advertisingLicenseCode=null, copyrightInformation=null, country=null, option=, provinceCode=null, provinceName=null, collectFlag=false, interPubPlatform=null, interPubPlatformUrl=null), detailUrlCn=https://castjournals.cast.org.cn/joweb/kjdb/CN/10.3981/j.issn.1000-7857.2016.18.009, detailUrlEn=https://castjournals.cast.org.cn/joweb/kjdb/EN/10.3981/j.issn.1000-7857.2016.18.009, pdfUrlCn=https://castjournals.cast.org.cn/joweb/kjdb/CN/PDF/10.3981/j.issn.1000-7857.2016.18.009, pdfUrlEn=https://castjournals.cast.org.cn/joweb/kjdb/EN/PDF/10.3981/j.issn.1000-7857.2016.18.009, aliStartDate=null, aliEndDate=null, collectionFlag=false, citedCount=null, citedUrl=null, previewStatus=0, delFlag=0, hasFullText=0, orderTime=1474992000000, fullTextJson=null, articleText=null, reference=null)
科技导报
| 研究论文 2016, 34(18): 84-88
飞秒激光参数对三态梯度型分子态布居数的影响
全屏
郭玮1,2 , 冯小静1
作者信息
1. 南华大学电气工程学院, 衡阳 421001;
2. 中国科学院大连化学物理研究所;分子反应动力学国家重点实验室, 大连 116023
Effects of femtosecond laser parameters on state populations of three-level ladder molecule
Affiliations
出版时间: 2016-09-28
doi: 10.3981/j.issn.1000-7857.2016.18.009
文章导航
利用含时波包法研究并且首次量化了强飞秒泵浦-探测激光场中泵浦场强、泵浦波长和脉宽对三态梯度型K2 分子态布居数的影响。泵浦场强、泵浦波长和脉宽影响Rabi振荡,而Rabi振荡的变化又导致了基态和激发态布居数周期性变化。量化这3个激光场参数对激发态布居数的影响验证了此周期性变化规律,表明变化频率随着泵浦场强和脉宽的增大而变化。研究表明调节激光场参数可实现对态布居数的选择性分布,可以为实验上实现分子的光控制提供重要参考。
含时波包法
/
三态梯度型K2 分子
/
态布居数
/
Rabi振荡
The effects of the pump intensity, the wavelength and the pulse width on the state populations of the three-level ladder K2 molecule driven by intense femtosecond pump-probe pulses are investigated by employing the time-dependent wave packet approach and are thus quantified. The Rabi oscillation is affected by the pump intensity, the wavelength and the pulse width, and its variation results in a periodical change of the populations in the ground state and the excited state. Quantifying their effects on the population of the excited state verifies the periodical nature and shows that the frequency varies with the increasing pump intensity and pulse width. The results illustrate that the needed population in the electronic state of interest can be obtained by controlling these parameters, which provides some important basis for light manipulation of molecular processes.
time-dependent wave packet approach
/
three-level K2 molecule
/
state populations
/
Rabi oscillation
郭玮, 冯小静.
飞秒激光参数对三态梯度型分子态布居数的影响.
科技导报,
2016
, 34
(18)
: 84
-88
.
DOI: 10.3981/j.issn.1000-7857.2016.18.009
GUO Wei, FENG Xiaojing.
Effects of femtosecond laser parameters on state populations of three-level ladder molecule[J].
Science & Technology Review ,
2016
, 34
(18)
: 84
-88
.
DOI: 10.3981/j.issn.1000-7857.2016.18.009
2016年第34卷第18期
PDF下载
190
19
引用本文
BibTeX
文章信息
doi: 10.3981/j.issn.1000-7857.2016.18.009
接收时间:2015-06-04
首发时间:2016-10-21
出版时间:2016-09-28
收稿日期:2015-06-04
修回日期:2015-12-17
https://castjournals.cast.org.cn/joweb/kjdb/CN/10.3981/j.issn.1000-7857.2016.18.009
复制链接
引用本文
BibTeX
2种不同金属材料的力学参数
科 Family 属数 Number of genus 种数 Number of species 占总种数比例 Percentage of total species (%) 属 Genus 种数 Number of species 占总种数比例 Percentage of total species (%) 鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78 小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39 多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39 红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87 小菇属 Mycena 11 5.26 光柄菇属 Pluteus 5 2.39 红菇属 Russula 17 8.13 栓菌属 Trametes 5 2.39
关闭全屏
BibTeX
EndNote
RefWorks
TxT