Article(id=1297161271888077697, tenantId=1146029695717560320, journalId=1296125381406982186, issueId=1297161216049308076, articleNumber=null, orderNo=null, doi=10.13550/j.jxhg.20250390, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1749225600000, receivedDateStr=2025-06-07, revisedDate=null, revisedDateStr=null, acceptedDate=1752681600000, acceptedDateStr=2025-07-17, onlineDate=1787196947309, onlineDateStr=2026-08-20, pubDate=1778774400000, pubDateStr=2026-05-15, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1787196947309, onlineIssueDateStr=2026-08-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1787196947309, creator=13701087609, updateTime=1787196947309, updator=13701087609, issue=Issue{id=1297161216049308076, tenantId=1146029695717560320, journalId=1296125381406982186, year='2026', volume='43', issue='5', pageStart='929', pageEnd='1184', issueExtLink='null', onlineDate='null', pubDate='1778774400000', pubDateStr='2026-05-15', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=1, specialIssue=null, createTime=1787196933996, creator='13701087609', updateTime=1787202244949, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1297183491922354645, tenantId=1146029695717560320, journalId=1296125381406982186, issueId=1297161216049308076, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1297183491922354646, tenantId=1146029695717560320, journalId=1296125381406982186, issueId=1297161216049308076, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1153, endPage=1159, ext={EN=ArticleExt(id=1297161272047461250, articleId=1297161271888077697, tenantId=1146029695717560320, journalId=1296125381406982186, language=EN, title=Preparation of nitrogen-doped carbon-coated lithium manganese iron phosphate cathode material and its performance improvement mechanism, columnId=null, journalTitle=Fine Chemicals, columnName=null, runingTitle=null, highlight=null, articleAbstract=

A nitrogen-doped carbon-coated lithium iron manganese phosphate (LMFP) composite (N-C@LMFP) was synthesized from ball-milling glucose, as carbon source, and urea, as nitrogen source, with LMFP precursor, and characterized by XRD, Raman spectroscopy, XPS, and TEM. The effect of nitrogen doping content (that is, the percentage of the amount of substance of nitrogen in urea accounting for that of carbon in glucose, the same below) on the electrochemical performance of N-C@LMFP electrode was evaluated by cyclic voltammetry and electrochemical impedance spectroscopy, while the mechanism through which the nitrogen-doped carbon layer enhanced the rate capability of LMFP cathode material was also investigated. The results indicated that the 5% N-C@LMFP electrode with 5% nitrogen doping content exhibited the best electrochemical performance, achieving a discharge specific capacity of 133.6 mA·h/g. Even under a high discharge rate of 5 C, the specific capacity remained at 98.7 mA·h/g, significantly outperforming that of the undoped C@LMFP. Furthermore, after 300 cycles at 1 C, the 5% N-C@LMFP electrode exhibited a capacity retention rate of 95.3%, surpassing that of C@LMFP (93.9%), demonstrating enhanced cycling stability. The improved performance was attributed to the strong interaction between the nitrogen-doped carbon layer and the LMFP matrix. Specifically, chemical bonds such as N—Mn and N—Fe formed at the interface effectively reduced the charge transfer resistance and enhanced the lithium ion diffusion coefficient, thereby improving both structural stability and ion transport kinetics.

, authors=Yongpeng CUI¹, Shuxin ZHENG², Yajun WANG¹, Wei XING², authorsList=Yongpeng CUI, Shuxin ZHENG, Yajun WANG, Wei XING, authorCompany=null, correspAuthors=null, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1297161272450114435, articleId=1297161271888077697, tenantId=1146029695717560320, journalId=1296125381406982186, language=CN, title=氮掺杂碳层包覆磷酸锰铁锂正极材料的制备及其性能提升机制, columnId=1297161248622273210, journalTitle=精细化工, columnName=有机电化学与工业, runingTitle=null, highlight=null, articleAbstract=

以葡萄糖为碳源、尿素为氮源，将其与磷酸锰铁锂（LMFP）前驱体进行球磨，制备了氮掺杂碳包覆的LMFP复合材料（N-C@LMFP）。采用XRD、Raman、XPS、TEM对N-C@LMFP进行了表征。通过循环伏安和电化学阻抗测试，考察了氮掺杂量（即尿素中氮元素物质的量与葡萄糖中碳元素物质的量的百分数，下同）对N-C@LMFP电极电化学性能的影响。探究了氮掺杂碳层对LMFP正极材料倍率性能的提升机制。结果表明，氮掺杂量为5%的5% N-C@LMFP表现出最好的电化学性能，放电比容量高达133.6 mA·h/g，在5 C下快速放电，比容量仍可达98.7 mA·h/g，明显高于未氮掺杂改性的C@LMFP。5% N-C@LMFP在1 C下循环300圈后容量保留率为95.3%，优于C@LMFP（93.9%），表现出良好的循环稳定性。氮掺杂碳层与LMFP基体间的相互作用是增强电极材料结构稳定性和提高锂离子传输动力学的关键，原因在于碳掺杂碳层与LMFP基体间形成的N—Mn、N—Fe等化学键可有效降低电极中的电荷转移电阻，提升锂离子扩散系数。

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崔永朋（1992—），男，博士，副教授，博士生导师，E-mail: yongpengcui@cup.edu.cn。

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崔永朋（1992—），男，博士，副教授，博士生导师，E-mail: yongpengcui@cup.edu.cn。

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