Article(id=1325116777109266639, tenantId=1146029695717560320, journalId=1255847867265597444, issueId=1325115579346059524, articleNumber=null, orderNo=null, doi=null, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1328371200000, receivedDateStr=2012-02-05, revisedDate=1330876800000, revisedDateStr=2012-03-05, acceptedDate=null, acceptedDateStr=null, onlineDate=1793862059142, onlineDateStr=2026-11-05, pubDate=1376496000000, pubDateStr=2013-08-15, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793862059142, onlineIssueDateStr=2026-11-05, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793862059142, creator=13701087609, updateTime=1793862059142, updator=13701087609, issue=Issue{id=1325115579346059524, tenantId=1146029695717560320, journalId=1255847867265597444, year='2013', volume='27', issue='4', pageStart='473', pageEnd='632', issueExtLink='null', onlineDate='null', pubDate='1376496000000', pubDateStr='2013-08-15', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793861773573, creator='13701087609', updateTime=1793861773573, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext=null, issueFiles=null, downloadFileDto=null}, startPage=490, endPage=494, ext={EN=ArticleExt(id=1325116777495142608, articleId=1325116777109266639, tenantId=1146029695717560320, journalId=1255847867265597444, language=EN, title=Liquid-Liquid Phase Transition of Water at High Pressure and Ambient Temperature, columnId=null, journalTitle=Chinese Journal of High Pressure Physics, columnName=null, runingTitle=null, highlight=null, articleAbstract=

In-situ Raman measurement of water has been conducted at the temperature of 300 K and the pressure of 0.1-1 400 MPa using a SiC anvil cell. The experimental results show that the frequency of liquid water ν₁ decreases with increase of pressure (p), and two discontinuities are observed at about 200 and 620 MPa. Therefore three states of water are recognized. From state Ⅰ to state Ⅱ then to state III, the value of |dν₁/dp| reduces, indicating that the compressibility is related to the pressure, and it is becoming more difficult to compress as the pressure is increasing. The connection mode of a water molecule with its neighboring water molecules changes as the pressure increases. The discontinuous property of water suggests a possible liquid to liquid phase transition and structural change at 200 and 620 MPa.

, authors=Hui-Yuan WANG, Hai-Fei ZHENG, authorsList=Hui-Yuan WANG, Hai-Fei ZHENG, authorCompany=null, correspAuthors=Hai-Fei ZHENG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1325116777918767313, articleId=1325116777109266639, tenantId=1146029695717560320, journalId=1255847867265597444, language=CN, title=常温高压下水的液-液相变, columnId=0, journalTitle=高压物理学报, columnName=, runingTitle=null, highlight=null, articleAbstract=

在300 K、0.1~1 400 MPa条件下，利用碳化硅压腔，进行了液态水的拉曼光谱测量和研究。实验结果表明：随着压力的增大，水的对称伸缩振动峰（ν₁）整体向低频方向移动，但在约200和620 MPa处存在不连续，可明显分为3个区间（Ⅰ、Ⅱ、Ⅲ）；水从状态Ⅰ到状态Ⅱ再到状态Ⅲ，其拉曼位移对压力p的变化率（|dν₁/dp|）减小，表明水变得越来越难以压缩；随着压力的改变，相邻的五水分子聚合体之间的连接方式发生了变化。这些性质表明，液态水在约200和620 MPa处可能存在着液-液相转变。

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王慧媛（1986-），女，博士研究生，主要从事实验地球化学研究. E-mail：wanghuiyuan1986@126.com

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王慧媛（1986-），女，博士研究生，主要从事实验地球化学研究. E-mail：wanghuiyuan1986@126.com

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