Article(id=1147999698855649662, tenantId=1146029695717560320, journalId=1146123346816638986, issueId=1147999683156370319, articleNumber=1000-8063(2025)01-0144-07, orderNo=null, doi=10.13426/j.cnki.yky.2024.04.16, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1714147200000, receivedDateStr=2024-04-27, revisedDate=null, revisedDateStr=null, acceptedDate=null, acceptedDateStr=null, onlineDate=1751634057009, onlineDateStr=2025-07-04, pubDate=1739980800000, pubDateStr=2025-02-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1751634057009, onlineIssueDateStr=2025-07-04, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1751634057009, creator=13701087609, updateTime=1751634057009, updator=13701087609, issue=Issue{id=1147999683156370319, tenantId=1146029695717560320, journalId=1146123346816638986, year='2025', volume='44', issue='1', pageStart='1', pageEnd='150', issueExtLink='null', onlineDate='null', pubDate='null', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1751634053267, creator=13701087609, updateTime=1759123824852, updator=13701087609, preIssue=null, nextIssue=null, ext={EN=IssueExt(id=1179414062141158321, tenantId=1146029695717560320, journalId=1146123346816638986, issueId=1147999683156370319, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1179414062141158322, tenantId=1146029695717560320, journalId=1146123346816638986, issueId=1147999683156370319, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null}, startPage=144, endPage=150, ext={EN=ArticleExt(id=1147999699094725011, articleId=1147999698855649662, tenantId=1146029695717560320, journalId=1146123346816638986, language=EN, title=Research and Application of Pretreatment Technology for Uranium Containing Waste Liquid, columnId=1175805042197152439, journalTitle=Uranium Mining and Metallurgy, columnName=SAFETY AND ENVIRONMENT PROTECTION, runingTitle=null, highlight=null, articleAbstract=

A pretreatment process for uranium containing waste liquid was proposed to address the issues of nanofiltration membrane blockage and ion exchange resin poisoning in the treatment of uranium containing waste liquid. On the basis of determining the optimal process parameters for chemical precipitation and organic matter decomposition in the laboratory, engineering design and verification were carried out. The results show that after pretreatment, the turbidity of the waste liquid can be reduced to 16.25 NTU (removal rate of 98.74%), and COD can be reduced to 110.25 mg/L (removal rate of 87.13%). The waste liquid after pretreatment meets the water quality requirements of nanofiltration and ion exchange resin, and the pretreatment process effectively solves the problems in the treatment of uranium containing wastewater during uranium conversion.

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侯彦龙(1989—),男,陕西西安人,硕士,高级工程师,主要从事核化工研究。

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侯彦龙(1989—),男,陕西西安人,硕士,高级工程师,主要从事核化工研究。

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侯彦龙(1989—),男,陕西西安人,硕士,高级工程师,主要从事核化工研究。

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Statistics for each system of pretreatment process

, figureFileSmall=null, figureFileBig=null, tableContent=
系统 浊度/NTU COD/(mg/L) ρ(U)/(mg/L)
原水 1 250 856.58 17.20
化学沉淀系统 205.6 767.73 9.38
过滤系统 121.6 698.25 8.90
有机物预处理 86.13 475.93 8.45
有机物分解系统 67.20 143.54 8.30
超滤系统 15.66 110.25 3.18
), ArticleFig(id=1179340501233841044, tenantId=1146029695717560320, journalId=1146123346816638986, articleId=1147999698855649662, language=CN, label=表1, caption=

预处理各系统数据统计

, figureFileSmall=null, figureFileBig=null, tableContent=
系统 浊度/NTU COD/(mg/L) ρ(U)/(mg/L)
原水 1 250 856.58 17.20
化学沉淀系统 205.6 767.73 9.38
过滤系统 121.6 698.25 8.90
有机物预处理 86.13 475.93 8.45
有机物分解系统 67.20 143.54 8.30
超滤系统 15.66 110.25 3.18
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含铀废液预处理技术的研究和应用
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侯彦龙 , 耿龙 , 王伟 , 杨磊 , 陈静 , 彭子阳
铀矿冶 | 安全·环保 2025,44(1): 144-150
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铀矿冶 | 安全·环保 2025, 44(1): 144-150
含铀废液预处理技术的研究和应用
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侯彦龙, 耿龙, 王伟, 杨磊, 陈静, 彭子阳
作者信息
  • 中核四0四有限公司第一分公司, 甘肃 兰州 732850
  • 侯彦龙(1989—),男,陕西西安人,硕士,高级工程师,主要从事核化工研究。

Research and Application of Pretreatment Technology for Uranium Containing Waste Liquid
Yanlong HOU, Long GENG, Wei WANG, Lei YANG, Jing CHEN, Ziyang PENG
Affiliations
  • The First Filial Company of the 404 Co., Ltd., CNNC, Lanzhou 732850, China
出版时间: 2025-02-20 doi: 10.13426/j.cnki.yky.2024.04.16
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针对铀转化含铀废液处理中存在的纳滤膜堵塞和离子交换树脂中毒问题,提出了含铀废液预处理工艺路线。实验室确定工艺路线中化学沉淀和有机物分解的最佳工艺参数,在此基础上进行了工程设计与验证。结果表明:预处理后废液浊度可降低至16.25 NTU(去除率达98.74%),COD可降低至110.25 mg/L(去除率达87.13%),预处理后的废液满足纳滤与离子交换树脂的水质要求,预处理工艺有效解决了铀转化含铀废液处理中存在的问题。
含铀废液  /  铀转化  /  预处理  /  化学沉降  /  有机物分解

A pretreatment process for uranium containing waste liquid was proposed to address the issues of nanofiltration membrane blockage and ion exchange resin poisoning in the treatment of uranium containing waste liquid. On the basis of determining the optimal process parameters for chemical precipitation and organic matter decomposition in the laboratory, engineering design and verification were carried out. The results show that after pretreatment, the turbidity of the waste liquid can be reduced to 16.25 NTU (removal rate of 98.74%), and COD can be reduced to 110.25 mg/L (removal rate of 87.13%). The waste liquid after pretreatment meets the water quality requirements of nanofiltration and ion exchange resin, and the pretreatment process effectively solves the problems in the treatment of uranium containing wastewater during uranium conversion.

uranium containing waste liquid  /  uranium conversion  /  pretreatment  /  chemical sedimentation  /  organic matter decomposition
侯彦龙, 耿龙, 王伟, 杨磊, 陈静, 彭子阳. 含铀废液预处理技术的研究和应用. 铀矿冶, 2025 , 44 (1) : 144 -150 . DOI: 10.13426/j.cnki.yky.2024.04.16
Yanlong HOU, Long GENG, Wei WANG, Lei YANG, Jing CHEN, Ziyang PENG. Research and Application of Pretreatment Technology for Uranium Containing Waste Liquid[J]. Uranium Mining and Metallurgy, 2025 , 44 (1) : 144 -150 . DOI: 10.13426/j.cnki.yky.2024.04.16
天然铀纯化转化过程中产生的含铀废液,含有铀酰离子、金属离子、不溶颗粒以及微量有机物等,需处理达标后方能排放[1]。目前含铀废液的处理方法主要有蒸发浓缩法、吸附法、沉淀法、溶解萃取法、离子交换法、膜分离法等[2-4]
离子交换法是一种工业中常用的深度除铀方法。采用流化床离子交换设备处理含铀废液,可将铀质量浓度从15~36 mg/L降至0.1 mg/L[5];采用强酸性阳离子树脂处理分析检测过程产生的废液,可使溢流液中的铀质量浓度小于50 μg/L[6];采用碳酸钠对天然水体进行预处理,再利用新型硅负载阴离子交换树脂对水样中的铀进行定量回收,回收率大于95%[7]。对某大型铀矿渗透水处理系统SBA树脂上的含铀物质的化学组成、微生物群落结构等的研究发现,树脂失活的主要原因可能是树脂表面沉积物的形成,而不是官能团的饱和[8]。在工业应用中,也发现当被处理液体中的有机物或细小颗粒较多时,容易导致树脂中毒、吸附量降低。因此,需要对废液进行预处理,以降低废液的浊度和有机物含量。
膜分离法是一种高效分离技术,一般超滤或微滤工艺对水溶液中阳离子和阴离子拦截效果较差[9],而纳滤工艺对多价离子截留效果较好。纳滤能选择性地去除铀,同时允许其他微量矿物质通过[10-11],采用改性蒙脱石材质的纳滤膜可将铀去除率提高到99%以上[12]。膜分离技术对进水水质要求极高,需要较低的浊度和有机物含量。
铀转化产生的含铀废水中含有悬浮物、胶体、微生物,以及TBP、煤油、石油磺酸、润滑油等有机物,在运行过程中,这些物质会对离子交换柱和纳滤膜系统的稳定运行产生较大影响。针对这些问题,研究该废水的预处理工艺,旨在去除含铀废水中的污染物,使之满足深度除铀系统的进水要求(铀质量浓度<10 mg/L、浊度<20 NTU、COD<150 mg/L、pH=5~7),实现系统的稳定运行。
目前,国内外研发出了一系列含铀废水处理技术,主要有化学沉淀法[13]、纳米零价铁还原固化法、离子交换法、吸附法、微生物法、电沉积法、膜分离法和矿物固铀法等[14]。化学沉淀法处理含铀废水技术相对成熟,但沉淀处理后的溶液很难达到排放标准。因此,该方法常用于含铀废水的预处理。另外,废水中存在着大量难以被一般化学氧化法氧化降解的有机物,利用芬顿催化法可以有效降解此类有机物[15]
本研究通过采用化学沉淀法、芬顿催化法,以及超滤方法,来有效保障废水处理达标。原工艺没有预处理系统,本研究新增的预处理系统主要包括化学沉淀、过滤、有机物预处理、有机物分解、超滤工序,其工艺流程见图1
在水溶液中,${\mathrm{U}\mathrm{O}}_{2}^{2+}$可与含氧配位基进行配合反应;在碳酸体系下,${\mathrm{U}\mathrm{O}}_{2}^{2+}$可与$\mathrm{C}{\mathrm{O}}_{3}^{2-}$形成UO2(CO3)${_{3}^{4-}}$[16],这些反应对含铀废液的碱沉淀过程会产生不利影响。因此,采用酸化、碱化、絮凝沉降方式,加入PAM可使小颗粒絮状物凝结为大颗粒的絮状物,颗粒间在吸附架桥作用下,加速絮凝沉降,使水中微粒、大分子有机物等杂质从水相中分离出来[17]
过滤工序可去除水中的固体悬浮物或胶态杂质,能有效去除沉淀技术不能去除的微小粒子。由于石英砂具有过滤阻力小、比表面积大、耐酸碱性能强、抗污染性能好等特点[18],本系统选用石英砂作为过滤介质。
有机物预处理工序的主体设备为除油树脂塔,塔内填装的树脂是一种由亲油性的交联聚苯乙稀为母体聚合物和位于母体聚合物上的亲水性磺酸基团构成的高分子材料[19],该材料比表面积较大,能将油分子吸附至树脂内部孔道中;当油膜达到一定厚度时,在水流的曳力作用下,富集的油以大油滴形式脱落升向液面,从而实现油水分离。该树脂无需单独再生,油膜脱离后,树脂即恢复吸附性能[20]
有机物分解系工序采用芬顿催化氧化法。羟基自由基对含硝基、磺酸基、氯基等电子密度高的有机物具有独特的氧化优势[21]。芬顿催化氧化法本质上是通过催化过氧化氢所产生的羟基自由基对有机污染物进行氧化分解,使有机污染物分解为二氧化碳、水和其他物质。
超滤工序可有效拦截有机分子、胶体、细菌或不溶微粒,对后续纳滤膜起到保护作用。
铀转化生产线产生的碳酸钠淋洗液及其配套辅助设施产生的分析、清洗以及排风淋洗液,其pH在8~11之间,铀含量质量浓度为100~500 mg/L,含有${\mathrm{H}\mathrm{C}\mathrm{O}}_{3}^{-}$${\mathrm{C}\mathrm{O}}_{3}^{2-}$、Cl-、F-、Na+及微量Fe3+、Ca2+,含少量硝酸根和有机相。另外,树脂塔解析液也属于碳酸系废水,其铀质量浓度约为2 g/L。试验原液浊度为1 250 NTU,pH为8,使用该废水进行试验,以浊度去除率间接反映悬浮物及胶体的去除率。
主要药剂:10% H2SO4溶液、30% NaOH溶液、38%PFC溶液、1‰PAM溶液、30%过氧化氢溶液以及芬顿催化剂。
烧杯、磁力搅拌器等常规试验设备,检测仪器有便携式pH计、浊度测定仪、COD测定仪等。
1)酸化条件试验:取原液500 mL置于烧杯中,用H2SO4溶液将其pH分别调至2、3、4、5、6后,搅拌20 min,使之充分酸化;然后分别向各酸化废液中加入NaOH溶液,调节pH至12,在室温下搅拌20 min使之充分碱化;静置沉淀2 h,取上清液进行浊度分析,确定最佳酸化pH。
2)碱化条件试验:取原液500 mL置于烧杯中,用H2SO4溶液将其pH调至最佳酸化pH,搅拌20 min,使之充分酸化;然后分别向酸化废液中加入NaOH溶液,调节其pH至8、9、10、11、12、13,室温下搅拌20 min,使之充分碱化;静置沉淀2 h,取上清液进行浊度分析,确定最佳碱化pH;
3)PFC添加量条件试验:取原液500 mL置于烧杯中,用H2SO4溶液将其pH调至最佳酸化pH,搅拌20 min;然后用NaOH溶液将废液pH调至最佳碱化pH,再分别加入0.20、0.25、0.30、0.35、0.40 mL的38% PFC溶液及1‰ PAM溶液,搅拌20 min;静置沉淀2 h,取上清液进行浊度、COD、铀浓度分析,确定最佳PFC添加量。
1)催化氧化pH调节条件试验:取原液500 mL置于烧杯中,用H2SO4溶液将其pH分别调节为2、3、4、5后,加入催化剂,搅拌均匀;分别向其中加入1.5倍原液COD量的过氧化氢,搅拌均匀后反应3 h,每隔0.5 h取样1次分析COD,确定催化氧化pH调节最佳值。
2)过氧化氢添加量条件试验:取原液500 mL置于烧杯中,用H2SO4溶液将其pH分别调节至催化氧化pH调节最佳值,加入催化剂,搅拌均匀;分别向其中加入原液COD量的1~3倍的过氧化氢,搅拌均匀后反应3 h,每隔0.5 h取样1次分析COD,确定催化氧化过氧化氢添加量最佳值。
酸化条件试验结果见图2。可以看出,随着pH增加,浊度去除率呈先增加后减小的趋势。当pH为3时,浊度去除率达64.60%,沉淀效果最佳;当pH>3时,由于酸化过程消除了原液中${\mathrm{C}\mathrm{O}}_{3}^{2-}$对重铀酸钠形成的不利影响,同时使含铀悬浮颗粒充分溶解,提高了氢氧化钠沉淀的效率;当pH≤3时,${\mathrm{C}\mathrm{O}}_{3}^{2-}$已基本去除,但铀酰根离子在水溶液中除了与碳酸根发生配合反应外,与硫酸根和硝酸根等其他含氧配位基也可发生配合反应。因此,酸化pH以3为宜。
原液浊度为1 250 NTU,pH为8,使用该废水进行碱化条件试验,然后取上清液进行浊度分析。以浊度去除率间接反映悬浮物及胶体的去除率,结果见图3
图3可看出,随着碱化pH的增加,浊度去除率呈先增加后减小趋势,当pH=11时,浊度去除率最高。这是由于溶液中氢氧根浓度越高,铀酰根离子与氢氧根结合能力越强,越易形成重铀酸钠;当pH过大后,重铀酸钠形成过快,晶体粒径减小,形成的沉淀颗粒不易沉降,上清液浊度增加,去除率反而下降。因此,碱化pH以11为宜。
原液浊度为1 250 NTU,pH为8,使用该废水进行PFC添加量条件试验,然后取上清液进行浊度、COD、铀浓度分析。通过计算得出废液中悬浮物、胶体及有机物、铀的去除率,其结果见图4
图4可看出,当酸化pH=3、碱化pH=11时,随着PFC加入量的不断增加,废液中悬浮物及胶体、有机物与铀的去除率均不断增加,当PFC加入量超过0.35 mL时,各去除率均无明显变化。故PFC加入量以0.35 mL为宜,对应质量浓度为260 mg/L。
加入PFC后,悬浮物的去除率明显提高。这是由于PFC在碱性环境下水解产生的Fe(OH)3对重铀酸钠及其他杂质起到良好的絮凝效果,提高了沉淀效率,使悬浮微粒随絮凝物共沉淀。此外,絮凝沉淀过程对部分有机物同样具有去除效果,酸化过程中由于有机溶剂的溶解度减小,可以达到去除有机溶剂的目的;碱化过程中在Fe(OH)3和PAM的共同作用下,在絮体形成过程中会吸附有机物,达到去除有机物的效果。
对不同pH的废水进行过氧化氢催化氧化试验,原液COD为837 mg/L。使用该废水进行催化氧化过氧化氢添加量条件试验,每隔0.5 h取样1次分析其中的COD,试验结果见图5
图5可看出,随着pH的升高,废水中COD的去除率先升高后降低。当pH为4时,分解效率最高,2.5 h后COD去除率变化较小,维持在到54%,说明催化氧化分解的最佳pH为4。通过不同pH的试验发现,前2 h有机物分解较快,例如当pH=4时,前2 h的废水中COD去除率达49%;后1 h的COD去除率呈现出明显的降低趋势,仅有4%。分解率降低的原因是过氧化氢作为强氧化剂,结构不稳定,易发生氧化和分解反应,随着反应的进行,过氧化氢逐渐被消耗,导致后续反应缓慢。同时,过氧化氢催化氧化对于部分有机物的分解只限于长碳链结构,当有机物分解为更为稳定的短链结构时,过氧化氢催化氧化法就难以继续分解,分解效率随之降低。
原液COD为837 mg/L,pH为8,对该废水进行催化氧化过氧化氢添加量条件试验,每隔0.5 h取样1次分析其中的COD,试验结果见图6。可以看出,H2O2与催化剂共同使用时能够明显提高COD去除率。随着H2O2量的增加,分解活性先增强后降低。当H2O2加入倍数为2倍时,分解活性最好,在2.5 h内达到50%以上的有机物去除率;2.5 h后,分解率上升趋势逐渐减慢。
当H2O2加入量过大时,分解效果反而下降,是由于H2O2具有氧化还原性,当遇到比它氧化性更强的氧化剂时,表现出还原性,会与COD分析仪所使用的重铬酸钾发生反应,增加重铬酸钾消耗量,当H2O2添加量过大时,分析误差影响占据主导作用。因此,最终确定H2O2含量为2倍COD含量,此时催化氧化效果最佳。
本工艺确定有机物分解工艺的最佳运行参数:pH控制为4,H2O2含量为2倍COD,反应时间为2.5 h。
建立处理能力为48 m3/d的废水预处理工程平台,将生产线实际废水引入预处理工程,分别对源项废水以及各关键处理工序尾水进行取样分析(表1),验证系统的有效性。
经工程化应用验证,化学沉降系统、过滤系统、有机物预处理系统、有机物分解系统、超滤系统各工序对固体悬浮物及胶体、有机物均有一定的去除效果,整套系统可将废液中的浊度从1 250 NTU降至15.66 NTU,浊度去除率98.74%,达到预期的浊度小于20 NTU的效果;可将废液中的COD从856.58 mg/L降至110.25 mg/L,COD去除率为87.13%,达到预期的COD降至150 mg/L以下的设计要求。
研究确定了铀转化含铀废水的预处理工艺及最佳工艺参数,其中化学沉淀工序中酸化pH为3,碱化pH为11,PFC加入量在260 mg/L;有机物分解工艺中,催化氧化pH为4,H2O2含量为2倍COD含量,反应时间为2.5 h。该预处理工艺可去除废液中悬浮物、胶体及有机物等,处理后废液浊度可降低至16.25 NTU,COD可降低至110.25 mg/L。
增加预处理工艺后,保证了铀纯化转化含铀废液深度除铀工艺中纳滤膜和离子交换工序的稳定运行,解决了纳滤膜堵塞和离子交换树脂的中毒问题,提高了铀纯化转化含铀废液处理工艺系统运行的稳定性。
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doi: 10.13426/j.cnki.yky.2024.04.16
  • 接收时间:2024-04-27
  • 首发时间:2025-07-04
  • 出版时间:2025-02-20
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  • 收稿日期:2024-04-27
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    中核四0四有限公司第一分公司, 甘肃 兰州 732850
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Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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