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Article(id=1304141625190544200, tenantId=1146029695717560320, journalId=1303687303576780880, issueId=1304141619603726817, articleNumber=null, orderNo=null, doi=10.3969/j.issn.1009-3842.2026.01.007, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1717430400000, receivedDateStr=2024-06-04, revisedDate=1768924800000, revisedDateStr=2026-01-21, acceptedDate=null, acceptedDateStr=null, onlineDate=1788861193225, onlineDateStr=2026-09-08, pubDate=1772208000000, pubDateStr=2026-02-28, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1788861193225, onlineIssueDateStr=2026-09-08, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1788861193225, creator=13701087609, updateTime=1788861193225, updator=13701087609, issue=Issue{id=1304141619603726817, tenantId=1146029695717560320, journalId=1303687303576780880, year='2026', volume='', issue='1', pageStart='1', pageEnd='154', issueExtLink='null', onlineDate='null', pubDate='1772208000000', pubDateStr='2026-02-28', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1788861191893, creator='13701087609', updateTime=1788924965522, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1304409105645465969, tenantId=1146029695717560320, journalId=1303687303576780880, issueId=1304141619603726817, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1304409105645465970, tenantId=1146029695717560320, journalId=1303687303576780880, issueId=1304141619603726817, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=76, endPage=89, ext={EN=ArticleExt(id=1304141625383482185, articleId=1304141625190544200, tenantId=1146029695717560320, journalId=1303687303576780880, language=EN, title=Progress of Application of Cu-based Materials in Electro-reduction of Nitrate for Production of Ammonia, columnId=1304141568877814747, journalTitle=Copper Engineering, columnName=Material Preparation and Process Engineering, runingTitle=null, highlight=null, articleAbstract=

Ammonia plays an important role in human activities, which is used widely in various industries with noticeable economic values. The main method currently used in ammonia synthesis is Haber-Bosch method, which requires high-temperature or high-pressure conditions, suffering low efficiency and high energy cost. In comparison, electro-reduction of nitrite for ammonia production is a NH3-selective green chemistry process with low energy consumption. Cu-based materials are chosen as common catalyst materials in electro-production of ammonia owing to the abundance of source materials and high reaction activity towards nitrite. State-of-art Cu-based materials applied in electro catalysis of nitrate for ammonia production are mainly: metallic Cu, metallic-doped Cu-based materials, alloys, Cu oxide, Cu-containing polymetallic oxide, Cu-containing metal-organic framework (MOF), etc. These catalysts improve performances of ammonia production with different mechanisms, such as surface modulation, electron structure modulation, synergy of catalytic active centers, construction of built-in electric fields, etc. This paper aims to integrate performances and mechanisms of different Cu-based catalysts for electrochemical production of ammonia, and to provide reference for future research in this field.

, authors=Jangfeng TENG1, Shikun GE1, Ziwei WANG1, Cong PENG2, 3, Wenchao ZHANG2, 3, authorsList=Jangfeng TENG, Shikun GE, Ziwei WANG, Cong PENG, Wenchao ZHANG, authorCompany=null, correspAuthors=Cong PENG, Wenchao ZHANG, authorNote=null, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1304141625744192330, articleId=1304141625190544200, tenantId=1146029695717560320, journalId=1303687303576780880, language=CN, title=铜基材料在电催化还原硝酸盐产氨技术中的应用进展, columnId=1304141569037198301, journalTitle=铜业工程, columnName=材料制备与加工工程, runingTitle=null, highlight=null, articleAbstract=

氨在人类社会活动中扮演着至关重要的角色，广泛应用于诸多工业领域，具有重要的经济价值。目前氨合成的主要方法是Haber-Bosch法，即在高温高压下完成氨的制备，该方法效率低，能耗高。相比之下，电化学还原硝酸盐产氨是一种低能耗的绿色化学过程，对氨选择性较高。铜基材料来源广泛、成本低、催化效率高，且形貌与电子结构可调控，并对硝酸盐具有良好的选择性，因而被用作电化学产氨的常用催化剂。目前应用于硝酸盐电催化产氨的铜基材料主要有金属铜、掺杂型铜材料、合金材料、铜氧化物材料、含铜多金属氧化物、含铜金属框架（MOF）等。这些催化剂提升电化学产氨的机理各不相同，主要包括晶面调控、电子结构调控、催化活性中心协同作用、内置电场的构建等。本文旨在对不同铜基催化剂的电化学产氨效果及其机理进行综合梳理分析，为该领域的研究提供参考并对未来发展趋势进行展望。

, authors=滕蒋锋1, 葛世坤1, 王子威1, 彭聪2, 3, 张文超2, 3, authorsList=滕蒋锋, 葛世坤, 王子威, 彭聪, 张文超, authorCompany=null, correspAuthors=彭聪, 张文超, authorNote=

滕蒋锋（1998—），男，湖南常德人，硕士，研究方向：环境电化学，E-mail：

葛世坤（2000—），男，云南昆明人，硕士，研究方向：固体废物处理与资源化，E-mail：

, correspAuthorsNote=
彭聪，教授，E-mail：
张文超，教授，E-mail：
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滕蒋锋（1998—），男，湖南常德人，硕士，研究方向：环境电化学，E-mail：

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滕蒋锋（1998—），男，湖南常德人，硕士，研究方向：环境电化学，E-mail：

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葛世坤（2000—），男，云南昆明人，硕士，研究方向：固体废物处理与资源化，E-mail：

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铜基材料在电催化还原硝酸盐产氨技术中的应用进展
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滕蒋锋 1 , 葛世坤 1 , 王子威 1 , 彭聪 2, 3 , 张文超 2, 3
铜业工程 | 材料制备与加工工程 2026,(1): 76-89
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铜业工程 |材料制备与加工工程 2026 , (1) : 76 -89
铜基材料在电催化还原硝酸盐产氨技术中的应用进展
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滕蒋锋（1998—），男，湖南常德人，硕士，研究方向：环境电化学，E-mail：

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滕蒋锋（1998—），男，湖南常德人，硕士，研究方向：环境电化学，E-mail：

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葛世坤（2000—），男，云南昆明人，硕士，研究方向：固体废物处理与资源化，E-mail：

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葛世坤（2000—），男，云南昆明人，硕士，研究方向：固体废物处理与资源化，E-mail：

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滕蒋锋1 , 葛世坤1 , 王子威1, 彭聪2, 3 , 张文超2, 3
作者信息
  • 1.中南林业科技大学生态环境学院，湖南 长沙 410004
  • 2.中南大学冶金与环境学院，湖南 长沙 410083
  • 3.国家重金属污染防治工程技术研究中心， 湖南 长沙 410083
通讯作者:
彭聪，教授，E-mail：
张文超，教授，E-mail：
作者简介:

滕蒋锋（1998—），男，湖南常德人，硕士，研究方向：环境电化学，E-mail：

葛世坤（2000—），男，云南昆明人，硕士，研究方向：固体废物处理与资源化，E-mail：

Progress of Application of Cu-based Materials in Electro-reduction of Nitrate for Production of Ammonia
Jangfeng TENG1 , Shikun GE1 , Ziwei WANG1, Cong PENG2, 3 , Wenchao ZHANG2, 3
Affiliations
  • 1.School of Ecology and Environment，Central South University of Forestry & Technology，Changsha 410004，China
  • 2.School of Metallurgy and Environment，Central South University，Changsha 410083，China
  • 3.Chinese National Engineering Research Center for Control & Treatment of Heavy Metal Pollution，Changsha 410083，China
出版时间: 2026-02-28 doi: 10.3969/j.issn.1009-3842.2026.01.007
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氨在人类社会活动中扮演着至关重要的角色，广泛应用于诸多工业领域，具有重要的经济价值。目前氨合成的主要方法是Haber-Bosch法，即在高温高压下完成氨的制备，该方法效率低，能耗高。相比之下，电化学还原硝酸盐产氨是一种低能耗的绿色化学过程，对氨选择性较高。铜基材料来源广泛、成本低、催化效率高，且形貌与电子结构可调控，并对硝酸盐具有良好的选择性，因而被用作电化学产氨的常用催化剂。目前应用于硝酸盐电催化产氨的铜基材料主要有金属铜、掺杂型铜材料、合金材料、铜氧化物材料、含铜多金属氧化物、含铜金属框架（MOF）等。这些催化剂提升电化学产氨的机理各不相同，主要包括晶面调控、电子结构调控、催化活性中心协同作用、内置电场的构建等。本文旨在对不同铜基催化剂的电化学产氨效果及其机理进行综合梳理分析，为该领域的研究提供参考并对未来发展趋势进行展望。

铜基材料  /  电催化  /  产氨  /  硝酸盐

Ammonia plays an important role in human activities, which is used widely in various industries with noticeable economic values. The main method currently used in ammonia synthesis is Haber-Bosch method, which requires high-temperature or high-pressure conditions, suffering low efficiency and high energy cost. In comparison, electro-reduction of nitrite for ammonia production is a NH3-selective green chemistry process with low energy consumption. Cu-based materials are chosen as common catalyst materials in electro-production of ammonia owing to the abundance of source materials and high reaction activity towards nitrite. State-of-art Cu-based materials applied in electro catalysis of nitrate for ammonia production are mainly: metallic Cu, metallic-doped Cu-based materials, alloys, Cu oxide, Cu-containing polymetallic oxide, Cu-containing metal-organic framework (MOF), etc. These catalysts improve performances of ammonia production with different mechanisms, such as surface modulation, electron structure modulation, synergy of catalytic active centers, construction of built-in electric fields, etc. This paper aims to integrate performances and mechanisms of different Cu-based catalysts for electrochemical production of ammonia, and to provide reference for future research in this field.

copper-based material  /  electrocatalysis  /  ammonia production  /  nitrate
滕蒋锋, 葛世坤, 王子威, 彭聪, 张文超. 铜基材料在电催化还原硝酸盐产氨技术中的应用进展. 铜业工程, 2026 , (1) : 76 -89 . DOI: 10.3969/j.issn.1009-3842.2026.01.007
Jangfeng TENG, Shikun GE, Ziwei WANG, Cong PENG, Wenchao ZHANG. Progress of Application of Cu-based Materials in Electro-reduction of Nitrate for Production of Ammonia[J]. Copper Engineering, 2026 , (1) : 76 -89 . DOI: 10.3969/j.issn.1009-3842.2026.01.007
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  • 国家自然科学基金项目(52104315)
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doi: 10.3969/j.issn.1009-3842.2026.01.007
  • 接收时间：2024-06-04
  • 首发时间：2026-09-08
  • 出版时间：2026-02-28
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  • 收稿日期：2024-06-04
  • 修回日期：2026-01-21
基金
国家自然科学基金项目(52104315)
作者信息
    1.中南林业科技大学生态环境学院，湖南 长沙 410004
    2.中南大学冶金与环境学院，湖南 长沙 410083
    3.国家重金属污染防治工程技术研究中心， 湖南 长沙 410083

通讯作者:

彭聪，教授，E-mail：
张文超，教授，E-mail：
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https://castjournals.cast.org.cn/joweb/tygc/CN/10.3969/j.issn.1009-3842.2026.01.007
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2种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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