Article(id=1322942911377190950, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942849381183980, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210281, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1618502400000, receivedDateStr=2021-04-16, revisedDate=1622649600000, revisedDateStr=2021-06-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343769162, onlineDateStr=2026-10-30, pubDate=1634659200000, pubDateStr=2021-10-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343769162, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343769162, creator=13701087609, updateTime=1793343769162, updator=13701087609, issue=Issue{id=1322942849381183980, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='10', pageStart='2045', pageEnd='2312', issueExtLink='null', onlineDate='null', pubDate='1634659200000', pubDateStr='2021-10-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343754382, creator='13701087609', updateTime=1793345931656, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322951981580562527, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942849381183980, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322951981584756832, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942849381183980, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2251, endPage=2265, ext={EN=ArticleExt(id=1322942911557546023, articleId=1322942911377190950, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Research Progress on Borosilicate Glass Formulation for High-Level Liquid Waste Immobilization, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

Borosilicate glass is currently one of the most widely used matrix materials for high-level liquid waste vitrification due to its advantages of high waste loading, suitable melting temperature, strong adaptability to changes in waste components, radiation resistance and good chemical durability. This review represented recent work on the high-level waste vitrification mechanism of borosilicate glass, key product performance, process performance and economic indicators of borosilicate glass matrix of high-level liquid waste, as well as their engineering applications. This review suggested to carry out the systematic borosilicate glass formulation research in the future and establish the glass formulation design models to meet the vitrification requirements of different types of high-level waste liquids. In addition, the leaching mechanisms and long-term behaviors of borosilicate glass matrix could be also carried out to improve the evaluation criteria for waste glasses.

, authors=Min QIAN1, 2, Sijun FAN1, Tianfeng XUE1, Xin WANG1, Liyan ZHANG1, Minzhi RUAN3, Zhongdi LI3, Shubin CHEN1, Lili HU1, authorsList=Min QIAN, Sijun FAN, Tianfeng XUE, Xin WANG, Liyan ZHANG, Minzhi RUAN, Zhongdi LI, Shubin CHEN, Lili HU, authorCompany=null, correspAuthors=Lili HU, authorNote=

QIAN Min (1987-), female, Doctoral candidate. E-mail:

, correspAuthorsNote=
HU Lili (1963-), female, Ph. D., Professor. E-mail:
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硼硅酸盐玻璃具有包容率高、熔制温度合理、对废液组分变化适应性强、抗辐射、化学稳定性好等优点,是目前工业应用最广泛的高放废液固化玻璃基质。本文综述了硼硅酸盐玻璃固化高放射性元素的机理、高放废液硼硅酸盐玻璃固化体的关键产品性能、工艺性能和经济性指标的相关研究进展,以及硼硅酸盐玻璃固化体的工程化应用情况。根据国内硼硅酸盐玻璃固化体的研究现状,未来仍需开展系统的硼硅酸盐玻璃配方研究,建立配方设计模型以适应不同类型高放废液的固化需求;同时需开展玻璃固化体的腐蚀机理研究和长期化学稳定性评估,以制定并完善玻璃固化体评估标准。

, authors=钱敏1, 2, 凡思军1, 薛天锋1, 王欣1, 张丽艳1, 阮苠秩3, 李忠镝3, 陈树彬1, 胡丽丽1, authorsList=钱敏, 凡思军, 薛天锋, 王欣, 张丽艳, 阮苠秩, 李忠镝, 陈树彬, 胡丽丽, authorCompany=null, correspAuthors=胡丽丽, authorNote=

钱敏(1987—),女,博士研究生。

, correspAuthorsNote=
胡丽丽(1963—),女,博士,研究员。
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高放废液硼硅酸盐玻璃固化配方研究进展
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钱敏 1, 2 , 凡思军 1 , 薛天锋 1 , 王欣 1 , 张丽艳 1 , 阮苠秩 3 , 李忠镝 3 , 陈树彬 1 , 胡丽丽 1
硅酸盐学报 | 2021,49(10): 2251-2265
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硅酸盐学报 | 2021 , 49 (10) : 2251 -2265
高放废液硼硅酸盐玻璃固化配方研究进展
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钱敏1, 2 , 凡思军1, 薛天锋1, 王欣1, 张丽艳1, 阮苠秩3, 李忠镝3, 陈树彬1, 胡丽丽1
作者信息
  • 1.中国科学院上海光学精密机械研究所,强激光材料重点实验室,上海 201800
  • 2.中国科学院大学,北京 100049
  • 3.中国核电工程有限公司,北京 100840
通讯作者:
胡丽丽(1963—),女,博士,研究员。
作者简介:

钱敏(1987—),女,博士研究生。

Research Progress on Borosilicate Glass Formulation for High-Level Liquid Waste Immobilization
Min QIAN1, 2 , Sijun FAN1, Tianfeng XUE1, Xin WANG1, Liyan ZHANG1, Minzhi RUAN3, Zhongdi LI3, Shubin CHEN1, Lili HU1
Affiliations
  • 1.Key Laboratory of Materials for High Power Laser, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China
  • 2.University of Chinese Academy of Sciences, Beijing 100049, China
  • 3.China Nuclear Power Engineering Co., Ltd, Beijing 100840, China
  • Corresponding Author:
    HU Lili (1963-), female, Ph. D., Professor. E-mail:

    QIAN Min (1987-), female, Doctoral candidate. E-mail:

出版时间: 2021-10-20 doi: 10.14062/j.issn.0454-5648.20210281
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硼硅酸盐玻璃具有包容率高、熔制温度合理、对废液组分变化适应性强、抗辐射、化学稳定性好等优点,是目前工业应用最广泛的高放废液固化玻璃基质。本文综述了硼硅酸盐玻璃固化高放射性元素的机理、高放废液硼硅酸盐玻璃固化体的关键产品性能、工艺性能和经济性指标的相关研究进展,以及硼硅酸盐玻璃固化体的工程化应用情况。根据国内硼硅酸盐玻璃固化体的研究现状,未来仍需开展系统的硼硅酸盐玻璃配方研究,建立配方设计模型以适应不同类型高放废液的固化需求;同时需开展玻璃固化体的腐蚀机理研究和长期化学稳定性评估,以制定并完善玻璃固化体评估标准。

高放废液  /  玻璃固化  /  硼硅酸盐玻璃  /  硼硅酸盐玻璃陶瓷  /  化学稳定性  /  长期稳定性

Borosilicate glass is currently one of the most widely used matrix materials for high-level liquid waste vitrification due to its advantages of high waste loading, suitable melting temperature, strong adaptability to changes in waste components, radiation resistance and good chemical durability. This review represented recent work on the high-level waste vitrification mechanism of borosilicate glass, key product performance, process performance and economic indicators of borosilicate glass matrix of high-level liquid waste, as well as their engineering applications. This review suggested to carry out the systematic borosilicate glass formulation research in the future and establish the glass formulation design models to meet the vitrification requirements of different types of high-level waste liquids. In addition, the leaching mechanisms and long-term behaviors of borosilicate glass matrix could be also carried out to improve the evaluation criteria for waste glasses.

high-level liquid waste  /  vitrification  /  borosilicate glasses  /  borosilicate glass-ceramic  /  chemical stability  /  long-term behaviors
钱敏, 凡思军, 薛天锋, 王欣, 张丽艳, 阮苠秩, 李忠镝, 陈树彬, 胡丽丽. 高放废液硼硅酸盐玻璃固化配方研究进展. 硅酸盐学报, 2021 , 49 (10) : 2251 -2265 . DOI: 10.14062/j.issn.0454-5648.20210281
Min QIAN, Sijun FAN, Tianfeng XUE, Xin WANG, Liyan ZHANG, Minzhi RUAN, Zhongdi LI, Shubin CHEN, Lili HU. Research Progress on Borosilicate Glass Formulation for High-Level Liquid Waste Immobilization[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (10) : 2251 -2265 . DOI: 10.14062/j.issn.0454-5648.20210281
  • 国防科工局乏燃料后处理科研专项(FKY1683ZHG001SSJS-B01-001)
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2021年第49卷第10期
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doi: 10.14062/j.issn.0454-5648.20210281
  • 接收时间:2021-04-16
  • 首发时间:2026-10-30
  • 出版时间:2021-10-20
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  • 收稿日期:2021-04-16
  • 修回日期:2021-06-03
基金
国防科工局乏燃料后处理科研专项(FKY1683ZHG001SSJS-B01-001)
作者信息
    1.中国科学院上海光学精密机械研究所,强激光材料重点实验室,上海 201800
    2.中国科学院大学,北京 100049
    3.中国核电工程有限公司,北京 100840

通讯作者:

胡丽丽(1963—),女,博士,研究员。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20210281
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2种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
total species (%)
属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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