Article(id=1322942884076454416, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200428, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1592409600000, receivedDateStr=2020-06-18, revisedDate=1597507200000, revisedDateStr=2020-08-16, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343762653, onlineDateStr=2026-10-30, pubDate=1611072000000, pubDateStr=2021-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343762653, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343762653, creator=13701087609, updateTime=1793343762653, updator=13701087609, issue=Issue{id=1322942385474384734, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='1', pageStart='1', pageEnd='210', issueExtLink='null', onlineDate='null', pubDate='1611072000000', pubDateStr='2021-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343643777, creator='13701087609', updateTime=1793345438198, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322949911880282449, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322949911880282450, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=34, endPage=41, ext={EN=ArticleExt(id=1322942887016661521, articleId=1322942884076454416, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Performance and Optimization of Cobalt-free Double Perovskite Cathode SmBaFeNiO_5+δ for Intermediate-temperature Solid Oxide Fuel Cells, columnId=1322942386086753121, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on SOFC, runingTitle=null, highlight=null, articleAbstract=

A cobalt-free double-perovskite cathode SmBaFeNiO_5+δ (SBFN) was synthesized by a modified sol-gel process, and SmBaFeNiO_5+δ-Sm_0.2Ce_0.8O_1.9 (SBFN-SDC) composite cathodes were applied to reduce the thermal expansion coefficient (TEC) and improve the electrochemical performance. The average TEC of SBFN is 14.1×10^-6K^-1 in air at 30-900℃, while the SBFN-SDC15 (the mass ratio is 85∶15) composite cathode shows the lowest average TEC of 12.0×10^-6K^-1. The maximum conductivity of SBFN is 48 S/cm at 425℃. The polarization resistance (R_p) of SBFN is 0.386 Ω·cm² at 700℃ on SDC electrolyte. Introducing SDC to SBFN can increase the electrochemical catalytic activity of the cathode materials. SBFN-SDC10 (the mass ratio is 90∶10) composite cathode has the lowest R_p, which is 0.224 Ω·cm² at 700℃. The maximum power densities of Ni-SDC|SDC|SBFN and Ni-SDC|SDC|SBFN-SDC10 single cells are 367.6 mW/cm² and 507.8 mW/cm² at 800℃, respectively.

, authors=Dawei FU¹, Fangjun JIN², Tianmin HE¹, authorsList=Dawei FU, Fangjun JIN, Tianmin HE, authorCompany=null, correspAuthors=Tianmin HE, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322942890380493331, articleId=1322942884076454416, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=无Co双钙钛矿结构中温固体氧化物燃料电池阴极材料SmBaFeNiO_5+δ及其性能优化, columnId=1322942387823194979, journalTitle=硅酸盐学报, columnName=SOFC专题, runingTitle=null, highlight=null, articleAbstract=

用溶胶-凝胶法合成了无Co的双钙钛矿SmBaFeNiO_5+δ（SBFN）阴极材料，并引入Sm_0.2Ce_0.8O_1.9（SDC）电解质材料制备复合阴极，降低热膨胀系数和优化性能。研究表明：SBFN在30~900℃的平均热膨胀系数为14.1×10^-6K^-1，SBFN-SDC15（质量比为85∶15）复合阴极的平均热膨胀系数降为12.0×10^-6 K^-1。SBFN在425℃时电导率具有最大值，为48 S/cm。700℃时SBFN|SDC|SBFN对称电池的界面极化阻抗（R_p）为0.386 Ω·cm²。在SBFN中引入SDC可以改善其电化学性能，SBFN-SDC10（质量比为90∶10）复合阴极具有最低的R_p，为0.224 Ω·cm²。800℃时，以SBFN和SBFN-SDC10为阴极的单电池，最大功率密度分别为367.6 mW/cm²和507.8 mW/cm²。

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FU Dawei (1976-), male, Ph.D., Associate Professor. E-mail: fudw@jlu.edu.cn

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FU Dawei (1976-), male, Ph.D., Associate Professor. E-mail: fudw@jlu.edu.cn

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付大伟（1976—），男，博士，副教授。

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付大伟（1976—），男，博士，副教授。

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