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Article(id=1322942855114785250, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200503, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1594137600000, receivedDateStr=2020-07-08, revisedDate=1597593600000, revisedDateStr=2020-08-17, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343755748, onlineDateStr=2026-10-30, pubDate=1611072000000, pubDateStr=2021-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343755748, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343755748, creator=13701087609, updateTime=1793343755748, updator=13701087609, issue=Issue{id=1322942385474384734, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='1', pageStart='1', pageEnd='210', issueExtLink='null', onlineDate='null', pubDate='1611072000000', pubDateStr='2021-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343643777, creator='13701087609', updateTime=1793345438198, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322949911880282449, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322949911880282450, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942385474384734, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=14, endPage=19, ext={EN=ArticleExt(id=1322942855945257443, articleId=1322942855114785250, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Performance and Durability of Perovskite Anode Solid Oxide Fuel Cell Fueled by CO-CO2, columnId=1322942386086753121, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on SOFC, runingTitle=null, highlight=null, articleAbstract=

La0.4Sr0.6Co0.2Fe0.7Nb0.1O3-δ (LSCFN) anode structure, electrochemical performance and operating stability are characterized using CO-CO2 mixed as fuel. Results show that, the ABO3 perovskite structure of LSCFN is reduced to A2BO4 Ruddlesden-popper structure in CO fuel. While, the addition of CO2 can shift the structure of LSCFN back to single perovskite, and inhibit coking effectively. The maximum output power density of single cell using pure CO fuel is 0.6 W/cm2 at 850℃. And the cell operates for more than 100 hours when using CO∶CO2 mixed gas as fuel in molar ratio of 5∶1.

, authors=Xiaoyang CHEN1, Tenglong ZHU1, Qin ZHONG1, Minfang HAN2, authorsList=Xiaoyang CHEN, Tenglong ZHU, Qin ZHONG, Minfang HAN, authorCompany=null, correspAuthors=Tenglong ZHU, Minfang HAN, authorNote=

CHEN Xiaoyang (1992-), male, Doctoral candidate. E-mail:

, correspAuthorsNote=
ZHU Tenglong (1988-), male, Ph.D., Associate Professor; E-mail:
HAN Minfang (1967-), female, Ph.D., Professor.
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以原位析出纳米Co-Fe颗粒的La0.4Sr0.6Co0.2Fe0.7Nb0.1O3-δ（LSCFN）钙钛矿为阳极，考察了直接使用CO-CO2燃料时的阳极结构演变、单电池电化学性能和稳定性。结果表明：在CO燃料中，ABO3钙钛矿结构LSCFN转变为A2BO4层状钙钛矿结构；在CO中引入少量CO2后，LSCFN则以单钙钛矿结构为主，并有效抑制了碳沉积。单电池在CO燃料下的最大功率密度可达0.6 W/cm2（850℃），并在n（CO）∶n（CO2）=5∶1（摩尔比）燃料下运行超过100 h。

, authors=陈晓阳1, 朱腾龙1, 钟秦1, 韩敏芳2, authorsList=陈晓阳, 朱腾龙, 钟秦, 韩敏芳, authorCompany=null, correspAuthors=朱腾龙, 韩敏芳, authorNote=

陈晓阳（1992—），男，博士研究生。

, correspAuthorsNote=
朱腾龙（1988—），男，博士，副教授；
韩敏芳（1967—），女，博士，教授。
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CHEN Xiaoyang (1992-), male, Doctoral candidate. E-mail:

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陈晓阳（1992—），男，博士研究生。

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钙钛矿阳极固体氧化物燃料电池在CO-CO2燃料下的性能和稳定性
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陈晓阳 1 , 朱腾龙 1 , 钟秦 1 , 韩敏芳 2
硅酸盐学报 | SOFC专题 2021,49(1): 14-19
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硅酸盐学报 |SOFC专题 2021 , 49 (1) : 14 -19
钙钛矿阳极固体氧化物燃料电池在CO-CO2燃料下的性能和稳定性
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陈晓阳1 , 朱腾龙1 , 钟秦1, 韩敏芳2
作者信息
  • 1.南京理工大学化工学院，南京 210094
  • 2.清华大学能源与动力工程系，电力系统及大型发电设备安全控制与仿真国家重点实验室，北京 100084
通讯作者:
朱腾龙（1988—），男，博士，副教授；
韩敏芳（1967—），女，博士，教授。
作者简介:

陈晓阳（1992—），男，博士研究生。

Performance and Durability of Perovskite Anode Solid Oxide Fuel Cell Fueled by CO-CO2
Xiaoyang CHEN1 , Tenglong ZHU1 , Qin ZHONG1, Minfang HAN2
Affiliations
  • 1.School of Chemical Engineering, Nanjing University of Science and Technology, Nanjing 210094, China
  • 2.Department of Energy and Power Engineering, State Key Laboratory of Power Systems, Tsinghua University, Beijing 100084, China
    • Corresponding Author:
    ZHU Tenglong (1988-), male, Ph.D., Associate Professor; E-mail:
    HAN Minfang (1967-), female, Ph.D., Professor.

    CHEN Xiaoyang (1992-), male, Doctoral candidate. E-mail:

出版时间: 2021-01-20 doi: 10.14062/j.issn.0454-5648.20200503
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以原位析出纳米Co-Fe颗粒的La0.4Sr0.6Co0.2Fe0.7Nb0.1O3-δ（LSCFN）钙钛矿为阳极，考察了直接使用CO-CO2燃料时的阳极结构演变、单电池电化学性能和稳定性。结果表明：在CO燃料中，ABO3钙钛矿结构LSCFN转变为A2BO4层状钙钛矿结构；在CO中引入少量CO2后，LSCFN则以单钙钛矿结构为主，并有效抑制了碳沉积。单电池在CO燃料下的最大功率密度可达0.6 W/cm2（850℃），并在n（CO）∶n（CO2）=5∶1（摩尔比）燃料下运行超过100 h。

固体氧化物燃料电池  /  钙钛矿阳极  /  碳基燃料  /  稳定性  /  电化学性能

La0.4Sr0.6Co0.2Fe0.7Nb0.1O3-δ (LSCFN) anode structure, electrochemical performance and operating stability are characterized using CO-CO2 mixed as fuel. Results show that, the ABO3 perovskite structure of LSCFN is reduced to A2BO4 Ruddlesden-popper structure in CO fuel. While, the addition of CO2 can shift the structure of LSCFN back to single perovskite, and inhibit coking effectively. The maximum output power density of single cell using pure CO fuel is 0.6 W/cm2 at 850℃. And the cell operates for more than 100 hours when using CO∶CO2 mixed gas as fuel in molar ratio of 5∶1.

solid oxide fuel cell  /  perovskite anode  /  carbon-based fuel  /  durability  /  electrochemical performance
陈晓阳, 朱腾龙, 钟秦, 韩敏芳. 钙钛矿阳极固体氧化物燃料电池在CO-CO2燃料下的性能和稳定性. 硅酸盐学报, 2021 , 49 (1) : 14 -19 . DOI: 10.14062/j.issn.0454-5648.20200503
Xiaoyang CHEN, Tenglong ZHU, Qin ZHONG, Minfang HAN. Performance and Durability of Perovskite Anode Solid Oxide Fuel Cell Fueled by CO-CO2[J]. Journal of the Chinese Ceramic Society, 2021 , 49 (1) : 14 -19 . DOI: 10.14062/j.issn.0454-5648.20200503
基金
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  • 国家自然科学基金(51702163)
  • 江苏省重点研发计划(BE2017098)
  • 电力系统国家重点实验室开放课题(SKLD20KM23)
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2021年第49卷第1期
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doi: 10.14062/j.issn.0454-5648.20200503
  • 接收时间：2020-07-08
  • 首发时间：2026-10-30
  • 出版时间：2021-01-20
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  • 收稿日期：2020-07-08
  • 修回日期：2020-08-17
基金
国家自然科学基金(51702163)
江苏省重点研发计划(BE2017098)
电力系统国家重点实验室开放课题(SKLD20KM23)
作者信息
    1.南京理工大学化工学院，南京 210094
    2.清华大学能源与动力工程系，电力系统及大型发电设备安全控制与仿真国家重点实验室，北京 100084

通讯作者:

朱腾龙（1988—），男，博士，副教授；
韩敏芳（1967—），女，博士，教授。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20200503
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鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
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