Article(id=1322942559869349943, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942545734546372, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20200688, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1599667200000, receivedDateStr=2020-09-10, revisedDate=1602950400000, revisedDateStr=2020-10-18, acceptedDate=null, acceptedDateStr=null, onlineDate=1793343685357, onlineDateStr=2026-10-30, pubDate=1618848000000, pubDateStr=2021-04-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793343685357, onlineIssueDateStr=2026-10-30, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793343685357, creator=13701087609, updateTime=1793343685357, updator=13701087609, issue=Issue{id=1322942545734546372, tenantId=1146029695717560320, journalId=1263187385517883426, year='2021', volume='49', issue='4', pageStart='605', pageEnd='806', issueExtLink='null', onlineDate='null', pubDate='1618848000000', pubDateStr='2021-04-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793343681986, creator='13701087609', updateTime=1793345524324, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322950273110508350, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942545734546372, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322950273110508351, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322942545734546372, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=749, endPage=756, ext={EN=ArticleExt(id=1322942560079065145, articleId=1322942559869349943, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Cs₂NaBiCl₆:Mn²⁺- An Orange-yellow Inorganic Double Perovskite Phosphor, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

A series of Cs₂NaBiCl₆:Mn²⁺ double perovskite phosphors were prepared via liquid-phase synthesis, and their structures and luminescent properties were investigated by X-ray diffraction and fluorescence spectroscopy. The result show that with the gradual introduction of Mn²⁺, localized excitations centered on Bi³⁺ ions in the host lattice Cs₂NaBiCl₆ strongly absorb near-UV light, and the energy transfer between Bi³⁺ and Mn²⁺ promotes the electron transition between atomic d orbitals, thus leading to an intense orange-yellow photoluminescence. The photoluminescence reduces when the manganese-bismuth molar ratio is 0.7 due to the concentration quenching effect. Also, a broad emission peak centered at 590 nm is assigned to the ⁴T₁→⁶A₁ transition of octahedrally coordinated Mn²⁺. Based on the excitation spectrum, there are some peaks at 354 nm that arise from 6s²→6s¹6p¹ excitations of Bi³+ions. It is indicated that Cs₂NaBiCl₆:Mn²⁺ could be a promising fluorescent phosphor synthesized without the use of expensive reagents and toxic elements materials.

, authors=Luping WANG^{1, 2}, Guodong FAN^{1, 2}, Le WANG^{1, 2}, Fan WU^{1, 2}, authorsList=Luping WANG, Guodong FAN, Le WANG, Fan WU, authorCompany=null, correspAuthors=Guodong FAN, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1322942560771125306, articleId=1322942559869349943, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=Cs₂NaBiCl₆：Mn²⁺一种橙黄色全无机双钙钛矿荧光粉, columnId=0, journalTitle=硅酸盐学报, columnName=, runingTitle=null, highlight=null, articleAbstract=

采用液相合成法制备Cs₂NaBiCl₆：Mn²⁺荧光粉，通过利用X射线衍射、荧光光谱对其结构及发光性能进行了研究。结果表明：随着Mn²⁺的逐步引入，基质Cs₂NaBiCl₆中以Bi³⁺为中心的局域激发强烈吸收近紫外光，Bi³⁺向Mn²⁺发生能量转移促进了原子d轨道之间的电子跃迁并导致了强烈的橙黄色光致发光。当锰铋摩尔比n（Mn）/n（Bi）达到0.7以后，由于浓度猝灭效应导致光致发光明显变弱，同时在发射谱中可以看到，在590 nm附近有1个宽的发射峰，为八面配位Mn²⁺的⁴T₁→⁶A₁跃迁。激发谱包含了由Bi³⁺的6s²→6s¹6p¹激发产生的356 nm的吸收峰。Cs₂NaBiCl₆：Mn²⁺不含有毒元素，合成原料价格低廉，是一种具有潜在应用前景的新型橙黄色荧光材料。

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WANG Luping (1995-), female, Master candidate. E-mail: 1124671019@qq.com

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WANG Luping (1995-), female, Master candidate. E-mail: 1124671019@qq.com

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王露平（1995—），女，硕士研究生。

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王露平（1995—），女，硕士研究生。

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