Article(id=1322612216860357147, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612191723897081, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20190367, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1559232000000, receivedDateStr=2019-05-31, revisedDate=1561910400000, revisedDateStr=2019-07-01, acceptedDate=null, acceptedDateStr=null, onlineDate=1793264925445, onlineDateStr=2026-10-29, pubDate=1584633600000, pubDateStr=2020-03-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1793264925445, onlineIssueDateStr=2026-10-29, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1793264925445, creator=13701087609, updateTime=1793264925445, updator=13701087609, issue=Issue{id=1322612191723897081, tenantId=1146029695717560320, journalId=1263187385517883426, year='2020', volume='48', issue='3', pageStart='325', pageEnd='462', issueExtLink='null', onlineDate='null', pubDate='1584633600000', pubDateStr='2020-03-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1793264919452, creator='13701087609', updateTime=1793277037156, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1322663017125368549, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612191723897081, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1322663017125368550, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1322612191723897081, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=408, endPage=415, ext={EN=ArticleExt(id=1322612218634547741, articleId=1322612216860357147, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Mechanism of Stress Release in RB-SiC Ceramic Joints Bonded by Eucryptite/glass Composite Braze, columnId=null, journalTitle=Journal of the Chinese Ceramic Society, columnName=null, runingTitle=null, highlight=null, articleAbstract=

To solve thermal mismatch problem in the bonding process of RB-SiC ceramic using borosilicate glass braze (BS), β-eucryptite/BS composite braze (BSL) was designed. The effect of β-eucryptite addition on a) the characteristic temperature, thermal expansion coefficient and wettability of composite glass braze, as well as b) the microstructure and mechanical properties of joints was investigated. The thermal expansion coefficient of BSL decreases and its rate increases with the increase of β-eucryptite amount. Also, the characteristic temperature of BSL and its rate both increase with the increase of β-eucryptite amount. The apparent contact angle of BSL increases at the same temperature, and the variation of apparent contact angle along with temperature becomes slow. The RB-SiC/composite glass solder (BSL3)/RB-SiC joint has the similar interface to the RB-SiC/BS/RB-SiC joint bonded at 850 ℃ for 10 min. However, in the glass seam, β-eucryptite turns into massive gray KAlSiO4 crystals (i.e., kaliophilite). The massive KAlSiO4 crystals with a negative expansion characteristic can reduce the thermal expansion coefficient and prevent the crack propagation, thus strengthing the joint. The shear strength of the joint after reinforcement increases from 5.2 MPa to 10.9 MPa.

, authors=Panpan LIN1, Kaikai YU1, Tiesong LIN1, Peng HE1, Shouxiang LIU2, Ligang XU2, Weimin LONG3, Li BAO3, Jia MA3, authorsList=Panpan LIN, Kaikai YU, Tiesong LIN, Peng HE, Shouxiang LIU, Ligang XU, Weimin LONG, Li BAO, Jia MA, authorCompany=null, correspAuthors=Tiesong LIN, Peng HE, authorNote=

LIN Panpan (1987-), female, Ph.D., Lecturer. E-mai:

, correspAuthorsNote=
LIN Tiesong (1978-), male, Ph.D., Professor. E-mail:
HE Peng (1972-), male, Ph.D., Professor.
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设计了β-锂霞石/BS复合玻璃钎料(BSL),探究了β-锂霞石掺入量对复合玻璃钎料特征温度、热膨胀系数、润湿性及连接微观组织和力学性能的影响机制。随β-锂霞石掺入量增加,BSL复合玻璃钎料热膨胀系数逐渐降低且下降程度逐渐增大,其特征温度则逐渐升高且升高程度呈逐渐增大趋势,在相同温度下的表观接触角增大,同时其表观接触角随温度的变化变缓。当T=850 ℃、t=10 min时,复合玻璃钎料(BSL3)连接RB-SiC陶瓷的界面与相同工艺参数下的RB-SiC/BS界面组织相似,但在玻璃焊缝中,β-锂霞石转变为块状灰色KAlSiO4(钾霞石)晶体。块状KAlSiO4负膨胀相可降低热膨胀系数、阻止裂纹扩展,连接接头因此取得了较好的强化效果,接头的压剪强度从未强化前的5.2 MPa提高到10.9 MPa。

, authors=林盼盼1, 于凯凯1, 林铁松1, 何鹏1, 刘守相2, 徐李刚2, 龙伟民3, 鲍丽3, 马佳3, authorsList=林盼盼, 于凯凯, 林铁松, 何鹏, 刘守相, 徐李刚, 龙伟民, 鲍丽, 马佳, authorCompany=null, correspAuthors=林铁松, 何鹏, authorNote=

林盼盼(1987—),女,博士,讲师。

, correspAuthorsNote=
林铁松(1978—),男,博士,教授。
何鹏(1972—),男,博士,教授。
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锂霞石复合玻璃钎料连接碳化硅陶瓷接头的应力缓释机理
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林盼盼 1 , 于凯凯 1 , 林铁松 1 , 何鹏 1 , 刘守相 2 , 徐李刚 2 , 龙伟民 3 , 鲍丽 3 , 马佳 3
硅酸盐学报 | 2020,48(3): 408-415
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硅酸盐学报 | 2020 , 48 (3) : 408 -415
锂霞石复合玻璃钎料连接碳化硅陶瓷接头的应力缓释机理
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林盼盼1 , 于凯凯1, 林铁松1 , 何鹏1 , 刘守相2, 徐李刚2, 龙伟民3, 鲍丽3, 马佳3
作者信息
  • 1.哈尔滨工业大学,先进焊接与连接国家重点实验室,哈尔滨 150001
  • 2.北京无线电测量研究所,北京 100854
  • 3.郑州机械研究所,新型钎焊材料与技术国家重点实验室,郑州 450001
通讯作者:
林铁松(1978—),男,博士,教授。
何鹏(1972—),男,博士,教授。
作者简介:

林盼盼(1987—),女,博士,讲师。

Mechanism of Stress Release in RB-SiC Ceramic Joints Bonded by Eucryptite/glass Composite Braze
Panpan LIN1 , Kaikai YU1, Tiesong LIN1 , Peng HE1 , Shouxiang LIU2, Ligang XU2, Weimin LONG3, Li BAO3, Jia MA3
Affiliations
  • 1.State Key Laboratory of Advanced Welding and Joining, Harbin Institute of Technology, Harbin 150001, China
  • 2.Beijing Institute of Radio Measurement, Beijing 100845, China
  • 3.State Key Laboratory of Advanced Brazing Filler Metals and Technology, Zhengzhou Research Institute of Mechanical Engineering, Zhengzhou 450001, China
  • Corresponding Author:
    LIN Tiesong (1978-), male, Ph.D., Professor. E-mail:
    HE Peng (1972-), male, Ph.D., Professor.

    LIN Panpan (1987-), female, Ph.D., Lecturer. E-mai:

出版时间: 2020-03-20 doi: 10.14062/j.issn.0454-5648.20190367
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设计了β-锂霞石/BS复合玻璃钎料(BSL),探究了β-锂霞石掺入量对复合玻璃钎料特征温度、热膨胀系数、润湿性及连接微观组织和力学性能的影响机制。随β-锂霞石掺入量增加,BSL复合玻璃钎料热膨胀系数逐渐降低且下降程度逐渐增大,其特征温度则逐渐升高且升高程度呈逐渐增大趋势,在相同温度下的表观接触角增大,同时其表观接触角随温度的变化变缓。当T=850 ℃、t=10 min时,复合玻璃钎料(BSL3)连接RB-SiC陶瓷的界面与相同工艺参数下的RB-SiC/BS界面组织相似,但在玻璃焊缝中,β-锂霞石转变为块状灰色KAlSiO4(钾霞石)晶体。块状KAlSiO4负膨胀相可降低热膨胀系数、阻止裂纹扩展,连接接头因此取得了较好的强化效果,接头的压剪强度从未强化前的5.2 MPa提高到10.9 MPa。

反应烧结碳化硅陶瓷  /  复合玻璃钎料  /  微观组织  /  剪切强度

To solve thermal mismatch problem in the bonding process of RB-SiC ceramic using borosilicate glass braze (BS), β-eucryptite/BS composite braze (BSL) was designed. The effect of β-eucryptite addition on a) the characteristic temperature, thermal expansion coefficient and wettability of composite glass braze, as well as b) the microstructure and mechanical properties of joints was investigated. The thermal expansion coefficient of BSL decreases and its rate increases with the increase of β-eucryptite amount. Also, the characteristic temperature of BSL and its rate both increase with the increase of β-eucryptite amount. The apparent contact angle of BSL increases at the same temperature, and the variation of apparent contact angle along with temperature becomes slow. The RB-SiC/composite glass solder (BSL3)/RB-SiC joint has the similar interface to the RB-SiC/BS/RB-SiC joint bonded at 850 ℃ for 10 min. However, in the glass seam, β-eucryptite turns into massive gray KAlSiO4 crystals (i.e., kaliophilite). The massive KAlSiO4 crystals with a negative expansion characteristic can reduce the thermal expansion coefficient and prevent the crack propagation, thus strengthing the joint. The shear strength of the joint after reinforcement increases from 5.2 MPa to 10.9 MPa.

reaction sintering silicon carbide ceramic  /  composite glass braze  /  microstructure  /  shear strength
林盼盼, 于凯凯, 林铁松, 何鹏, 刘守相, 徐李刚, 龙伟民, 鲍丽, 马佳. 锂霞石复合玻璃钎料连接碳化硅陶瓷接头的应力缓释机理. 硅酸盐学报, 2020 , 48 (3) : 408 -415 . DOI: 10.14062/j.issn.0454-5648.20190367
Panpan LIN, Kaikai YU, Tiesong LIN, Peng HE, Shouxiang LIU, Ligang XU, Weimin LONG, Li BAO, Jia MA. Mechanism of Stress Release in RB-SiC Ceramic Joints Bonded by Eucryptite/glass Composite Braze[J]. Journal of the Chinese Ceramic Society, 2020 , 48 (3) : 408 -415 . DOI: 10.14062/j.issn.0454-5648.20190367
  • “战略性国际科技创新合作重点专项(2016YFE0201300)
  • 国家自然科学基金青年科学基金项目(51805112)
  • 哈尔滨工业大学科研创新基金项目(HIT.NSRIF.2020004)
  • 装备预研领域基金项目(61409230512)
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2020年第48卷第3期
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doi: 10.14062/j.issn.0454-5648.20190367
  • 接收时间:2019-05-31
  • 首发时间:2026-10-29
  • 出版时间:2020-03-20
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出版历史
  • 收稿日期:2019-05-31
  • 修回日期:2019-07-01
基金
“战略性国际科技创新合作重点专项(2016YFE0201300)
国家自然科学基金青年科学基金项目(51805112)
哈尔滨工业大学科研创新基金项目(HIT.NSRIF.2020004)
装备预研领域基金项目(61409230512)
作者信息
    1.哈尔滨工业大学,先进焊接与连接国家重点实验室,哈尔滨 150001
    2.北京无线电测量研究所,北京 100854
    3.郑州机械研究所,新型钎焊材料与技术国家重点实验室,郑州 450001

通讯作者:

林铁松(1978—),男,博士,教授。
何鹏(1972—),男,博士,教授。
参考文献
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20190367
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2种不同金属材料的力学参数
科
Family
属数
Number of
genus
种数
Number of
species
占总种数比例
Percentage of
total species (%)
属
Genus
种数
Number of
species
占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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