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Article(id=1319987079942099575, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987055371858691, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210810, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1631635200000, receivedDateStr=2021-09-15, revisedDate=1636560000000, revisedDateStr=2021-11-11, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639044032, onlineDateStr=2026-10-22, pubDate=1645286400000, pubDateStr=2022-02-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639044032, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639044032, creator=13701087609, updateTime=1792639044032, updator=13701087609, issue=Issue{id=1319987055371858691, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='2', pageStart='277', pageEnd='554', issueExtLink='null', onlineDate='null', pubDate='1645286400000', pubDateStr='2022-02-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639038174, creator='13701087609', updateTime=1792639254308, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319987961958089069, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987055371858691, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319987961958089070, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319987055371858691, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=307, endPage=320, ext={EN=ArticleExt(id=1319987080160203384, articleId=1319987079942099575, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Thermal Transport Engineering of Several Emerging Thermoelectric Materials and Thermal Logic Devices, columnId=1321891632362926248, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Inerim Achievements of Key Program of National Natural Science Foundation of China—Review, runingTitle=null, highlight=null, articleAbstract=

With the developments of the electronics and energy technologies, studies on nanostructure engineering of the emerging thermoelectric materials and thermal logic devices are drawing increasing attentions. In this review, we focus on several promising thermoelectric materials, and study the mechanisms of thermal transport engineering in the atomic and nano-scale structures theoretically and experimentally, with a micro-nano scale thermal transport measurement system developed by our research group. Such research focuses include: the atomic alloying of Si1-xGex alloy films with full components, the mismatched interfaces of Bi2Ca2Co2Oy layered-structure single crystals, the ionic localized resonances of superionic conductor A0.5RhO2 (A=K, Rb, Cs) single crystals, and the loose microstructures in quasi-one-dimensional ZrTe5/HfTe5 single crystals as well as the SnSe2 intercalations in SnSe single crystals. The influences of various scale structures and interatomic forces on the thermal transport properties are summarized, offering effective engineering strategies on developing potential thermoelectric materials with low thermal conductivity and excellent thermoelectric performance. Besides, the realization of effective dynamic engineering of thermal conductivity using phase transition, along with its potential applications in thermal logic devices are introduced.

, authors=Ruonan ZHAN1, Chen DI1, Zhiming GENG1, Enrui ZHANG1, Ziyuan YUAN1, Xuejun YAN1, Yang ZHAO2, 3, Shuhua YAO1, 4, Hong LU1, 4, Minghui LU1, 4, authorsList=Ruonan ZHAN, Chen DI, Zhiming GENG, Enrui ZHANG, Ziyuan YUAN, Xuejun YAN, Yang ZHAO, Shuhua YAO, Hong LU, Minghui LU, authorCompany=null, correspAuthors=Minghui LU, authorNote=

ZHAN Ruonan (1997-), female, Master candidate. E-mail:

, correspAuthorsNote=
LU Minghui (1979-), male, Ph.D., Associate Professor. E-mail:
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随着电子和能源科技的发展，基于纳米结构调控的新型热电材料以及热逻辑器件研究正受到越来越多的关注。本工作围绕几种具有应用潜力的热电材料，利用项目团队自主开发的微纳尺度热输运测试系统，从理论和实验上研究了原子及纳米尺度结构对热输运特性的调控机制，包括：全组分Si1-xGex合金薄膜的原子合金化，Bi2Ca2Co2Oy层状结构单晶的错配界面，超离子导体A0.5RhO2（A=K，Rb，Cs）单晶的离子局域共振，准一维结构ZrTe5/HfTe5单晶中的疏松微结构，以及SnSe单晶中的SnSe2原子级插层，总结了不同尺度结构和原子间作用力对热传导性质的影响规律，为探索低热导率、高热电转换性能的新型热电材料提供有效的调控方案。最后，介绍了利用相变转换机制实现热导率高效动态调控的实验结果，及其在热逻辑器件方面的潜在应用。

, authors=詹若男1, 狄琛1, 耿志明1, 张恩瑞1, 袁紫媛1, 颜学俊1, 赵旸2, 3, 姚淑华1, 4, 芦红1, 4, 卢明辉1, 4, authorsList=詹若男, 狄琛, 耿志明, 张恩瑞, 袁紫媛, 颜学俊, 赵旸, 姚淑华, 芦红, 卢明辉, authorCompany=null, correspAuthors=卢明辉, authorNote=

詹若男（1997—），女，硕士研究生。

, correspAuthorsNote=
卢明辉（1979—），男，博士，教授。
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ZHAN Ruonan (1997-), female, Master candidate. E-mail:

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ZHAN Ruonan (1997-), female, Master candidate. E-mail:

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詹若男（1997—），女，硕士研究生。

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詹若男（1997—），女，硕士研究生。

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若干新型热电材料的热输运调控及热逻辑器件
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詹若男 1 , 狄琛 1 , 耿志明 1 , 张恩瑞 1 , 袁紫媛 1 , 颜学俊 1 , 赵旸 2, 3 , 姚淑华 1, 4 , 芦红 1, 4 , 卢明辉 1, 4
硅酸盐学报 | 国家自然科学基金重点项目中期成果专题—综合评述 2022,50(2): 307-320
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硅酸盐学报 |国家自然科学基金重点项目中期成果专题—综合评述 2022 , 50 (2) : 307 -320
若干新型热电材料的热输运调控及热逻辑器件
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詹若男1 , 狄琛1, 耿志明1, 张恩瑞1, 袁紫媛1, 颜学俊1, 赵旸2, 3, 姚淑华1, 4, 芦红1, 4, 卢明辉1, 4
作者信息
  • 1．南京大学现代工程与应用科学学院，南京 210093
  • 2．中国科学院材料力学行为与设计重点实验室，中国科学技术大学，合肥 230026
  • 3．中国科学技术大学精密机械与仪器系，合肥 230026
  • 4．南京大学人工微结构科学与技术协同创新中心，南京 210093
通讯作者:
卢明辉（1979—），男，博士，教授。
作者简介:

詹若男（1997—），女，硕士研究生。

Thermal Transport Engineering of Several Emerging Thermoelectric Materials and Thermal Logic Devices
Ruonan ZHAN1 , Chen DI1, Zhiming GENG1, Enrui ZHANG1, Ziyuan YUAN1, Xuejun YAN1, Yang ZHAO2, 3, Shuhua YAO1, 4, Hong LU1, 4, Minghui LU1, 4
Affiliations
  • 1.Department of Materials Science and Engineering, College of Engineering and Applied Sciences, Nanjing University, Nanjing 210093, China
  • 2.CAS Key Laboratory of Mechanical Behavior and Design of Materials and Department of Precision Machinery and Instrumentation, University of Science and Technology of China, Hefei 230026, China
  • 3.University of Science and Technology of China, Hefei 230026, China
  • 4.Collaborative Innovation Center of Advanced Microstructures, Nanjing University, Nanjing 210093, China
    • Corresponding Author:
    LU Minghui (1979-), male, Ph.D., Associate Professor. E-mail:

    ZHAN Ruonan (1997-), female, Master candidate. E-mail:

出版时间: 2022-02-20 doi: 10.14062/j.issn.0454-5648.20210810
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摘要
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随着电子和能源科技的发展，基于纳米结构调控的新型热电材料以及热逻辑器件研究正受到越来越多的关注。本工作围绕几种具有应用潜力的热电材料，利用项目团队自主开发的微纳尺度热输运测试系统，从理论和实验上研究了原子及纳米尺度结构对热输运特性的调控机制，包括：全组分Si1-xGex合金薄膜的原子合金化，Bi2Ca2Co2Oy层状结构单晶的错配界面，超离子导体A0.5RhO2（A=K，Rb，Cs）单晶的离子局域共振，准一维结构ZrTe5/HfTe5单晶中的疏松微结构，以及SnSe单晶中的SnSe2原子级插层，总结了不同尺度结构和原子间作用力对热传导性质的影响规律，为探索低热导率、高热电转换性能的新型热电材料提供有效的调控方案。最后，介绍了利用相变转换机制实现热导率高效动态调控的实验结果，及其在热逻辑器件方面的潜在应用。

热输运  /  热电材料  /  热逻辑器件  /  微纳结构

With the developments of the electronics and energy technologies, studies on nanostructure engineering of the emerging thermoelectric materials and thermal logic devices are drawing increasing attentions. In this review, we focus on several promising thermoelectric materials, and study the mechanisms of thermal transport engineering in the atomic and nano-scale structures theoretically and experimentally, with a micro-nano scale thermal transport measurement system developed by our research group. Such research focuses include: the atomic alloying of Si1-xGex alloy films with full components, the mismatched interfaces of Bi2Ca2Co2Oy layered-structure single crystals, the ionic localized resonances of superionic conductor A0.5RhO2 (A=K, Rb, Cs) single crystals, and the loose microstructures in quasi-one-dimensional ZrTe5/HfTe5 single crystals as well as the SnSe2 intercalations in SnSe single crystals. The influences of various scale structures and interatomic forces on the thermal transport properties are summarized, offering effective engineering strategies on developing potential thermoelectric materials with low thermal conductivity and excellent thermoelectric performance. Besides, the realization of effective dynamic engineering of thermal conductivity using phase transition, along with its potential applications in thermal logic devices are introduced.

thermal transport  /  thermoelectric materials  /  thermal logic devices  /  micro-nano structures
詹若男, 狄琛, 耿志明, 张恩瑞, 袁紫媛, 颜学俊, 赵旸, 姚淑华, 芦红, 卢明辉. 若干新型热电材料的热输运调控及热逻辑器件. 硅酸盐学报, 2022 , 50 (2) : 307 -320 . DOI: 10.14062/j.issn.0454-5648.20210810
Ruonan ZHAN, Chen DI, Zhiming GENG, Enrui ZHANG, Ziyuan YUAN, Xuejun YAN, Yang ZHAO, Shuhua YAO, Hong LU, Minghui LU. Thermal Transport Engineering of Several Emerging Thermoelectric Materials and Thermal Logic Devices[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (2) : 307 -320 . DOI: 10.14062/j.issn.0454-5648.20210810
基金
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  • 半导体量子结构的制备、热输运及热管理调控的研究(51732006)
  • 国家自然科学基金青年项目(11904162)
  • 国家重大科研仪器研制项目(52027803)
  • 国家自然科学基金重大研究计划(91963211)
  • 国家自然科学基金青年基金(11804149)
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2022年第50卷第2期
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doi: 10.14062/j.issn.0454-5648.20210810
  • 接收时间：2021-09-15
  • 首发时间：2026-10-22
  • 出版时间：2022-02-20
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  • 收稿日期：2021-09-15
  • 修回日期：2021-11-11
基金
半导体量子结构的制备、热输运及热管理调控的研究(51732006)
国家自然科学基金青年项目(11904162)
国家重大科研仪器研制项目(52027803)
国家自然科学基金重大研究计划(91963211)
国家自然科学基金青年基金(11804149)
作者信息
    1．南京大学现代工程与应用科学学院，南京 210093
    2．中国科学院材料力学行为与设计重点实验室，中国科学技术大学，合肥 230026
    3．中国科学技术大学精密机械与仪器系，合肥 230026
    4．南京大学人工微结构科学与技术协同创新中心，南京 210093

通讯作者:

卢明辉（1979—），男，博士，教授。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20210810
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2种不同金属材料的力学参数
科
Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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