Article(id=1319987073252180393, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986978137944236, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210246, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1617897600000, receivedDateStr=2021-04-09, revisedDate=1624896000000, revisedDateStr=2021-06-29, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639042436, onlineDateStr=2026-10-22, pubDate=1647705600000, pubDateStr=2022-03-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639042436, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639042436, creator=13701087609, updateTime=1792639042436, updator=13701087609, issue=Issue{id=1319986978137944236, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='3', pageStart='555', pageEnd='876', issueExtLink='null', onlineDate='null', pubDate='1647705600000', pubDateStr='2022-03-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639019760, creator='13701087609', updateTime=1792639223744, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319987833767575858, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986978137944236, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319987833767575859, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986978137944236, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=769, endPage=774, ext={EN=ArticleExt(id=1319987073449312682, articleId=1319987073252180393, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Effect of LiOH on Tantalum Doped Li₇La₃Zr₂O₁₂ Garnet Solid Electrolyte, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Tantalum (Ta) doped Li₇La₃Zr₂O₁₂ (Ta-LLZO) ceramics were prepared via conventional solid-state reaction. LiOH was used as a lithium source and a sintering additive for ceramics. The effect of LiOH on the microstructure and ionic conductivity of Ta-LLZO ceramics was investigated. The results show that LiOH as a lithium source can promote the formation of cubic Ta-LLZO, and LiOH as a sintering additive can effectively improve the densification of ceramics. The dense cubic garnet Ta-LLZO ceramics were obtained by sintering at 1 200 ℃ for 5 h. When the amount of the sintering additive is 6% (in mass fraction), the ionic conductivity of ceramics reaches 6.23×10^-4 S·cm^-1. It is indicated that Li₇La₃Zr₂O₁₂ prepared via solid-state reaction has a great potential in the application of all-solid-state lithium ion batteries.

, authors=Jian SONG, Hang ZHANG, Lihong XUE, Wuxing ZHANG, Youwei YAN, authorsList=Jian SONG, Hang ZHANG, Lihong XUE, Wuxing ZHANG, Youwei YAN, authorCompany=null, correspAuthors=Lihong XUE, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319987073822605739, articleId=1319987073252180393, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=LiOH对Ta掺杂石榴石型Li₇La₃Zr₂O₁₂固体电解质的影响, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

通过固相法制备Ta掺杂Li₇La₃Zr₂O₁₂（Ta-LLZO）陶瓷，以LiOH为锂源合成Ta-LLZO粉末，并以LiOH为助烧剂制备Ta-LLZO陶瓷，研究了LiOH对Ta-LLZO陶瓷的组织结构和离子电导率的影响。结果表明：以LiOH为锂源可促进立方相Ta-LLZO的生成。同时，以LiOH为助烧剂，可有效促进陶瓷的致密化，在1 200 ℃烧结5 h可获得致密的立方相Ta-LLZO陶瓷。当助烧剂的添加量为6%（质量分数）时，陶瓷的离子电导率可达6.23×10^-4 S·cm^-1。可见，固相法制备的Li₇La₃Zr₂O₁₂在全固态锂离子电池中具有广阔的应用前景。

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SONG Jian (1994-), male, Master. E-mail: 952922916@qq.com

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宋健（1994—），男，硕士研究生。

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