Article(id=1319986974258217609, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20211030, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1638201600000, receivedDateStr=2021-11-30, revisedDate=1639929600000, revisedDateStr=2021-12-20, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639018835, onlineDateStr=2026-10-22, pubDate=1650384000000, pubDateStr=2022-04-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639018835, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639018835, creator=13701087609, updateTime=1792639018835, updator=13701087609, issue=Issue{id=1319986924727677753, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='4', pageStart='877', pageEnd='1200', issueExtLink='null', onlineDate='null', pubDate='1650384000000', pubDateStr='2022-04-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639007026, creator='13701087609', updateTime=1792639269665, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319988026600702366, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319988026600702367, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=966, endPage=974, ext={EN=ArticleExt(id=1319986974451155594, articleId=1319986974258217609, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Optical Thermometry Based on Fluorescence Intensity Ratio in Dual-Phases Glass Ceramics Containing LiYF₄∶Ln³⁺(Ln=Tb, Dy) and ZnAl₂O₄∶Cr³⁺ Nanocrystals, columnId=1321891873954837352, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on United Nations International Year of Glass—Research Articles, runingTitle=null, highlight=null, articleAbstract=

Dual-phases glass ceramics (GCs) containing LiYF₄∶Ln³⁺(Ln=Eu, Tb, Dy) and ZnAl₂O₄∶Cr³⁺ nanocrystals (NCs) were fabricated by a conventional melt-quenching method. The structural and spectrographic characterizations indicate that Ln³⁺ can be doped into LiYF₄ lattice and Cr³⁺ can be introduced into ZnAl₂O₄ lattice, respectively. In this regard, the luminescent centers are physically separated through a spatial isolation strategy, getting rid of adverse energy transfer processes. The dual-modal luminescence of Ln³⁺ and Cr³⁺ can be thus attained simultaneously. Also, optical thermometry based on the fluorescence intensity ratio (FIR) of Ln³⁺/Cr³⁺ is performed. Under irradiation upon 377 nm, the FIR value for Tb³⁺∶⁵D₄→⁷F₅ and Cr³⁺∶²E→⁴A₂ transitions varies acutely, with a maximal relative sensitivity of 0.80%·K^-1 at 570 K. The FIR-based optical thermometry for Dy³⁺∶⁴F_9/2→⁶H_13/2 and Cr³⁺∶²E→⁴A₂ transitions is carried out, with a maximal relative sensitivity of 0.86%·K^-1 at 573 K. As a consequence, the dual-phases GCs can be an ideal medium for the spatial isolation of luminescent centers, suppressing an adverse energy transfer process and realizing an efficient dual-mode luminescence. This is beneficial to the application of FIR-based optical thermometry for GC materials.

, authors=Xinyue LI¹, Yuzheng TONG¹, Jidong LIN², Shaoxiong WANG², Shichen LI³, Daqin CHEN¹, authorsList=Xinyue LI, Yuzheng TONG, Jidong LIN, Shaoxiong WANG, Shichen LI, Daqin CHEN, authorCompany=null, correspAuthors=Shichen LI, Daqin CHEN, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319986974669259403, articleId=1319986974258217609, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=基于LiYF₄∶Ln³⁺(Ln=Tb, Dy)和ZnAl₂O₄∶Cr³⁺双晶相玻璃陶瓷的荧光强度比温度传感特性, columnId=1321891874147775337, journalTitle=硅酸盐学报, columnName=“联合国国际玻璃年”特刊—研究论文, runingTitle=null, highlight=null, articleAbstract=

采用熔融急冷法在母体玻璃中原位析出四方LiYF₄和立方ZnAl₂O₄两种纳米晶。结构和光谱表征表明Ln³⁺（Ln=Eu, Tb, Dy）随玻璃原位晶化进入LiYF₄晶相，而Cr³⁺进入ZnAl₂O₄晶相中，因此发光中心Ln³⁺和Cr³⁺实现空间隔离，有效抑制其能量传递，从而同时得到Ln³⁺和Cr³⁺的高效发光。此外，利用Ln³⁺和Cr³⁺发光对温度的不同响应，实现Ln³⁺/Cr³⁺的荧光强度比温度传感。在377 nm波长激发下，Tb³⁺和Cr³⁺同时被有效激发，并且Tb³⁺∶⁵D₄→⁷F₅和Cr³⁺∶²E→⁴A₂能级跃迁强度比呈现出强烈的温度依赖特性，测温相对灵敏度在570 K时达到最大值0.80%·K^-1；在364 nm波长激发下，Dy³⁺的⁴F_9/2→⁶H_13/2和Cr³⁺离子的²E→⁴A₂能级跃迁强度比随温度变化而剧烈变化，测温相对灵敏度在573 K时达到最大值0.86%·K^-1。因此，双晶相玻璃陶瓷可有效隔离Ln³⁺和Cr³⁺等不同发光中心，同时实现高效发光，有利于荧光强度比光学测温，同时也拓展了玻璃陶瓷材料的应用。

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LI Xinyue (1990-), female, Ph. D., associate Professor. E-mail: lixy@hdu.edu.cn

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