Article(id=1319986961700475605, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20211079, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1639238400000, receivedDateStr=2021-12-12, revisedDate=1641139200000, revisedDateStr=2022-01-03, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639015841, onlineDateStr=2026-10-22, pubDate=1650384000000, pubDateStr=2022-04-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639015841, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639015841, creator=13701087609, updateTime=1792639015841, updator=13701087609, issue=Issue{id=1319986924727677753, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='4', pageStart='877', pageEnd='1200', issueExtLink='null', onlineDate='null', pubDate='1650384000000', pubDateStr='2022-04-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792639007026, creator='13701087609', updateTime=1792639269665, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319988026600702366, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319988026600702367, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986924727677753, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=879, endPage=885, ext={EN=ArticleExt(id=1319986961947939542, articleId=1319986961700475605, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Atomic-Scale Structural Origin of Reverse Relationship Between Hardness and Glass Transition Temperature of Peraluminous Aluminosilicate Glasses with Alkaline Earth Ions, columnId=1321891873954837352, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on United Nations International Year of Glass—Research Articles, runingTitle=null, highlight=null, articleAbstract=

To investigate the atomic-scale structural origin of the Vickers hardness (H_V) and glass transition temperature (T_g) of peraluminous aluminosilicate glasses with alkaline earth ions, we prepared a series of xRO·(49-x)Al₂O₃·51SiO₂ (x=0.0-16.0, in mole fraction; R=Mg, Ca, Sr, Ba) alkaline earth aluminosilicate glassy samples. H_V and T_g were characterized by Vickers micro-hardness test and differential scanning calorimetry (DSC). The results show that H_V increases, while T_g decreases with the increase of R²⁺ field strength at a fixed RO content. At a certain type of RO, H_V and T_g decrease simultaneously with the gradual substitution of Al₂O₃ by RO. 49Al₂O₃·51SiO₂ glass has the maximum H_V (i.e., 8.26 GPa) and T_g (i.e., 941 ℃). According to the structural analysis, the interactions between the competition and synergism among the packing density, average bond energy, bond energy density of glass network skeleton ions and the interstitial ions as a charge balancer are a main atomic-scale structural origin, thus leading to the reverse evolution of H_V and T_g with the increase of field strength of substituted R²⁺ and the similar change with the substitution of RO for Al₂O₃ in peraluminous aluminosilicate glasses.

, authors=Zhentao WANG, Shaoxuan GU, Zhisong DING, Haizheng TAO, authorsList=Zhentao WANG, Shaoxuan GU, Zhisong DING, Haizheng TAO, authorCompany=null, correspAuthors=Haizheng TAO, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319986962317038295, articleId=1319986961700475605, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=碱土替换铝硅酸盐玻璃硬度和玻璃转变温度反向演化的结构起源, columnId=1321891874147775337, journalTitle=硅酸盐学报, columnName=“联合国国际玻璃年”特刊—研究论文, runingTitle=null, highlight=null, articleAbstract=

为探究过铝区碱土铝硅酸盐玻璃随碱土离子替换硬度（H_V）和玻璃转变温度（T_g）的演化规律及结构起源，采用激光加热气动悬浮技术，制备了摩尔组成为xRO·（49-x）Al₂O₃·51SiO₂（x=0~16；R=Mg，Ca，Sr，Ba）的系列碱土铝硅酸盐玻璃样品。采用显微维氏硬度仪、差示扫描量热法（DSC）分别对样品的维氏硬度（H_V）和玻璃转变温度（T_g）进行了表征。结果表明：RO含量固定，随着R²⁺场强变大，玻璃的H_V升高，T_g下降；RO种类固定，随着RO对Al₂O₃替换量的增加，玻璃的H_V和T_g均下降，49Al₂O₃·51SiO₂玻璃具有最高的H_V（8.26 GPa）和最高的T_g（941 ℃）。结构解析发现：玻璃网络骨架的堆积密度、平均键能、键能密度以及作为电荷平衡体的填隙离子对玻璃H_V和T_g提升或削弱的相互竞争和协同作用，是玻璃的H_V和T_g随R²⁺的场强变化呈现反向演化、随RO对Al₂O₃替换呈现同向演化的结构根源。

, authors=王振涛, 顾少轩, 丁志松, 陶海征, authorsList=王振涛, 顾少轩, 丁志松, 陶海征, authorCompany=null, correspAuthors=陶海征, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=eob0VmakChalCRcAv+kD/g==, magXml=EFz6eZjz8mioIddKORI4kA==, pdfUrl=null, pdf=Gac6khWa7DED/6nowuGEPQ==, pdfFileSize=1128512, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=yJ1m9wFCdcAQTeuIVD2z5g==, mapNumber=null, fund=null)}, authors=[Author(id=1322507186002055448, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319986961700475605, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=18875195524@163.com, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1322507186064970010, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319986961700475605, authorId=1322507186002055448, language=EN, stringName=Zhentao WANG, firstName=Zhentao, middleName=null, lastName=WANG, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=State Key Laboratory of Silicate Materials for Architectures, Wuhan University of Technology, Wuhan 430070, China, bio={"content":"

WANG Zhentao (1997-), male, Master candidate. E-mail: 18875195524@163.com

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WANG Zhentao (1997-), male, Master candidate. E-mail: 18875195524@163.com

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王振涛（1997—），男，硕士研究生。

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王振涛（1997—），男，硕士研究生。

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