Article(id=1319986926497681927, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210792, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1631203200000, receivedDateStr=2021-09-10, revisedDate=1633449600000, revisedDateStr=2021-10-06, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639007448, onlineDateStr=2026-10-22, pubDate=1652976000000, pubDateStr=2022-05-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639007448, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639007448, creator=13701087609, updateTime=1792639007448, updator=13701087609, issue=Issue{id=1319986871980118160, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='5', pageStart='1201', pageEnd='1454', issueExtLink='null', onlineDate='null', pubDate='1652976000000', pubDateStr='2022-05-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792638994450, creator='13701087609', updateTime=1792639285419, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319988092451275233, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319988092451275234, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1263, endPage=1274, ext={EN=ArticleExt(id=1319986927143604745, articleId=1319986926497681927, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Construction and Properties of All-Solid-State Z-Scheme MoS₂/RGO/Fe₂O₃ Composites, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

It is imminent to develop and utilize solar energy to solve the increasingly serious environmental crisis. In order to improve the utilization rate of sunlight and the performance of photocatalysts, this work innovatively proposed to prepare Z-Scheme MoS₂/RGO/Fe₂O₃ ternary composites by an in-situ growth method combined with a surface electrostatic adsorption method.MoS₂/RGO hetero-structured binary composites were firstly synthesized by a hydrothermal method, and then all-solid-state Z-Scheme MoS₂/RGO/Fe₂O₃ photocatalyst was constructed via adjusting the solution pH value to create the same charges of MoS₂ and Fe₂O₃ and the opposite charges of RGO and MoS₂. According to the results by scanning electron microscopy and transmission electron microscopy, MoS₂ nanosheets and Fe₂O₃ nanoparticles are uniformly distributed on the surface of two-dimension RGO, and MoS₂ nanosheets and Fe₂O₃ nanoparticles display a stable hetero-structure onto RGO nanosheets. The RGO-based all-solid-state Z-Scheme photocatalyst possesses a superior photocatalytic reduction degradation performance under the simulated solar-driven illumination. Especially, the all-solid-state Z-Scheme photocatalyst MR0.43F has the optimum photoreduction degradation efficiency within 60 min for heavy metal Cr (VI) in a solution as a degradation indicator, which is 1.5 times greater than that of binary MoS₂/RGO composites. The all-solid-state Z-Scheme photocatalyst has wide-spectrum absorption, high separation efficiency of photogenerated carriers and surface chemical reaction efficiency, thus improving the photocatalytic properties.

, authors=Yongxin JIAO¹, Shu WANG^{1, 2}, Jianan YIN¹, Yu SUN¹, Xin LI¹, Yupu LIU¹, authorsList=Yongxin JIAO, Shu WANG, Jianan YIN, Yu SUN, Xin LI, Yupu LIU, authorCompany=null, correspAuthors=Shu WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319986928632582666, articleId=1319986926497681927, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=全固态Z-Scheme光催化剂MoS₂/RGO/Fe₂O₃的构筑及性能, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

开发利用太阳能解决日益严重的环境危机迫在眉睫，为了提高对太阳光的利用率和光催化剂的性能，采用原位生长并结合表面静电吸附的方法制备三元复合材料，先利用水热合成MoS₂/RGO二元异质结复合材料，再根据材料等电点调变溶液pH值制造MoS₂与Fe₂O₃表面电荷同性、而与RGO表面电荷异性，进而构筑MoS₂/RGO/Fe₂O₃全固态Z-Scheme光催化剂。通过扫描电镜和透射电子显微镜观察发现，MoS₂纳米花球和Fe₂O₃纳米颗粒均匀分布在二维片层结构的电子介体RGO表面，MoS₂和Fe₂O₃分别与RGO形成稳定的异质结构，充分证明此种方式构建复杂三元复合材料的可行性。RGO基全固态Z-Scheme光催化剂在模拟太阳光照射下具有优异的光催化还原降解性能，以无机重金属Cr（VI）溶液作为降解指示剂，60min内全固态Z-Scheme光催化剂中活性最佳的为MR0.43F试样，其光还原降解效率是二元复合材料MoS₂/RGO的1.5倍。这种全固态Z-Scheme光催化剂兼具宽光谱吸收、高效光生载流子分离效率和表面化学反应效率，改性后的光催化性能得到显著提升，这一光催化设计路线为水环境处理及清洁能源制备提供了新方向。

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