Article(id=1319986902632091971, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210743, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1630252800000, receivedDateStr=2021-08-30, revisedDate=1634400000000, revisedDateStr=2021-10-17, acceptedDate=null, acceptedDateStr=null, onlineDate=1792639001757, onlineDateStr=2026-10-22, pubDate=1652976000000, pubDateStr=2022-05-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792639001757, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792639001757, creator=13701087609, updateTime=1792639001757, updator=13701087609, issue=Issue{id=1319986871980118160, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='5', pageStart='1201', pageEnd='1454', issueExtLink='null', onlineDate='null', pubDate='1652976000000', pubDateStr='2022-05-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792638994450, creator='13701087609', updateTime=1792639285419, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319988092451275233, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319988092451275234, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1248, endPage=1256, ext={EN=ArticleExt(id=1319986902866972996, articleId=1319986902632091971, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Preparation and Properties of Bi_1-xCa_xFeO_3-δ Cathode Materials for Intermediate-Temperature Solid Oxide Fuel Cell, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Developing cathode materials with superior electrochemical activity is of great importance to the application of intermediate-temperature solid oxide fuel cell (IT-SOFC). In this paper, Bi_1-xCa_xFeO_3-δ (BCFx, x=0.1, 0.2 and 0.3) compounds were synthesized via solid-state reaction as a cathode material for IT-SOFC. The phase structure, electrical conductivity, oxygen transport performance, and the electrochemical performances of these compounds were evaluated. The as-prepared BCFx compounds show a single-phase perovskite structure. Among the BCFx materials, Bi_0.8Ca_0.2FeO_3-δ (BCF0.2) oxide has the maximum electrochemical catalytic activity. The polarization resistance of BCF0.2 cathode on symmetrical cell is 0.06 Ω·cm² at 750 ℃ in air. Meanwhile, the maximum peak power density of Ni-(Y₂O₃)_0.08(ZrO₂)_0.92(Ni-8YSZ) anode-supported single cell reaches 730 mW·cm² at 750 ℃. As is indicated by the electrical conductivity relaxation, the favorable oxygen reduction reaction catalytic activity of BCF0.2 can be ascribed to the higher oxygen bulk diffusion and surface exchange coefficient. The results of oxygen reduction kinetics reveal that the dissociation of adsorbed molecular oxygen is a limiting step for oxygen reduction reaction on BCF0.2 cathode.

, authors=Weiwei FENG, Huifen ZHAO, Muyi SHEN, Han CHEN, Lucun GUO, authorsList=Weiwei FENG, Huifen ZHAO, Muyi SHEN, Han CHEN, Lucun GUO, authorCompany=null, correspAuthors=Lucun GUO, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319986903085076805, articleId=1319986902632091971, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=中温固体氧化物燃料电池阴极材料Bi_1-xCa_xFeO_3-δ的制备及其性能, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

开发具有优异电化学活性的阴极材料对中温固体氧化物燃料电池（IT-SOFC）的应用至关重要。采用固相法制备无钴阴极材料Bi_1-xCa_xFeO_3-δ（BCFx，x=0.1、0.2和0.3），通过该体系材料的物相结构、电导率、氧传输特性以及电化学性能研究表明，950 ℃时可以合成具有单相钙钛矿结构的Bi_1-xCa_xFeO_3-δ（x=0.1、0.2和0.3）阴极粉体。BCFx阴极材料中，样品BCF0.2具有较高的电化学催化活性，750 ℃时，对称电池极化阻抗为0.06 Ω·cm²，Ni-（Y₂O₃）_0.08（ZrO₂）_0.92（Ni-8YSZ）阳极支撑单电池最大功率密度为730 mW/cm²。由电导弛豫结果得知，BCF0.2阴极良好的氧还原催化活性主要归因于其较高的氧扩散系数和表面交换系数。氧还原反应动力学研究表明，样品BCF0.2阴极氧还原反应的速率控制步骤为吸附氧的解离过程。

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FENG Weiwei (1995-), male, Master candidate. E-mail: ww_feng186@163.com

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FENG Weiwei (1995-), male, Master candidate. E-mail: ww_feng186@163.com

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冯伟伟（1995—），男，硕士研究生。

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冯伟伟（1995—），男，硕士研究生。

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