Article(id=1319986894692270246, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20210599, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1626969600000, receivedDateStr=2021-07-23, revisedDate=1632412800000, revisedDateStr=2021-09-24, acceptedDate=null, acceptedDateStr=null, onlineDate=1792638999865, onlineDateStr=2026-10-22, pubDate=1652976000000, pubDateStr=2022-05-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792638999865, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792638999865, creator=13701087609, updateTime=1792638999865, updator=13701087609, issue=Issue{id=1319986871980118160, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='5', pageStart='1201', pageEnd='1454', issueExtLink='null', onlineDate='null', pubDate='1652976000000', pubDateStr='2022-05-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=0, createTime=1792638994450, creator='13701087609', updateTime=1792639285419, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319988092451275233, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319988092451275234, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319986871980118160, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1375, endPage=1384, ext={EN=ArticleExt(id=1319986894868431015, articleId=1319986894692270246, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Ionothermal Synthesis of CHA-Type Zeolite Membrane for Desalination, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

Zeolite chabazite (CHA) membranes with a higher Si/Al mole ratio in the zeolite framework were prepared to improve their stability and separation performance. Pure zeolite CHA membranes were synthesized with imidazolium-based ionic liquids (ILs) as a structure-directing agent, which could improve the Si/Al ratio in the framework. ILs could be used repetitively at least 3 times for the synthesis of high-crystallinity zeolites. Under the optimized synthetic conditions, a continued zeolite CHA membrane obtained from an initial gel containing 1-buthyl-3-methylimidazolium bromide ([Bmim]Br) on the mullite tubular supports has a high water flux of 6.3 kg/(m²·h) with a high ion rejection (100%) for pervaporation (PV) separation of 3.5% (in mass fraction) NaCl aqueous solution at 75 ℃. The effects of temperature and feed concentration on the desalination performance of ILs-CHA membranes were also investigated. The water flux increases to 10.3 kg/(m²·h), and their salt rejections are 100% when the operating PV temperature increases at 90 ℃. Zeolite CHA membranes prepared have the superior separation performance even for desalination of 10% NaCl aqueous solution. Furthermore, the ILs-CHA zeolite membrane has a stable separation performance with a stable water flux as well as a high salt rejection in 3.5% NaCl aqueous solution at 75 ℃ for 3.5 d.

, authors=Huizhi ZHANG, Lai GAN, Ni LIU, Xinyue HUANG, Na HU, Xiangshu CHEN, authorsList=Huizhi ZHANG, Lai GAN, Ni LIU, Xinyue HUANG, Na HU, Xiangshu CHEN, authorCompany=null, correspAuthors=Na HU, Xiangshu CHEN, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319986895111700648, articleId=1319986894692270246, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=离子热法合成CHA型分子筛膜及其脱盐应用, columnId=1263922770220560512, journalTitle=硅酸盐学报, columnName=研究论文, runingTitle=null, highlight=null, articleAbstract=

通过合成较高骨架硅铝比的CHA型分子筛膜可实现提高膜层稳定性和分离性能。采用咪唑类离子液体合成出纯相的CHA型分子筛膜，离子液体不仅作为新型结构导向剂，还提高晶体骨架Si/Al比，同时离子液体回收使用3次后仍能合成出高结晶度CHA型晶体。在最佳合成条件下，通过含溴化1-丁基-3-甲基咪唑（[Bmim]Br）的合成溶胶中在莫来石管状支撑体上获得连续的CHA型分子筛膜层，该膜在75 ℃、3.5%（质量分数）氯化钠溶液中渗透水通量为6.3 kg/（m²·h），截留率高达100%。考察了操作温度和料液浓度对膜渗透汽化脱盐性能影响。当操作温度升高至90 ℃时，膜水通量急剧提高到10.3 kg/（m²·h），甚至在10%高浓度氯化钠溶液中以及在3.5%氯化钠溶液中连续测试3.5 d，膜均表现出优异的脱盐性能。

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