Article(id=1319973056223760458, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319973019079000285, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230686, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1693756800000, receivedDateStr=2023-09-04, revisedDate=1699459200000, revisedDateStr=2023-11-09, acceptedDate=null, acceptedDateStr=null, onlineDate=1792635700517, onlineDateStr=2026-10-22, pubDate=1713542400000, pubDateStr=2024-04-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792635700517, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792635700517, creator=13701087609, updateTime=1792635700517, updator=13701087609, issue=Issue{id=1319973019079000285, tenantId=1146029695717560320, journalId=1263187385517883426, year='2024', volume='52', issue='4', pageStart='1171', pageEnd='1476', issueExtLink='null', onlineDate='null', pubDate='1713542400000', pubDateStr='2024-04-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792635691661, creator='13701087609', updateTime=1792641833008, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319998777822396474, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319973019079000285, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319998777822396475, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319973019079000285, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1413, endPage=1437, ext={EN=ArticleExt(id=1319973056433475659, articleId=1319973056223760458, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Research Progress and Modification Methods of Dielectric Energy Storage Ceramic Thin Films, columnId=1321894930528719547, journalTitle=Journal of the Chinese Ceramic Society, columnName=Special Issue on Dielectric Energy Storage Materials—Review, runingTitle=null, highlight=null, articleAbstract=

In recent years, with a rapid societal development, the utilization of clean energy becomes a necessity. This demand emphasizes on energy storage equipment, prompts some research on efficient energy storage, energy loss reduction, and environmental impact mitigation. The existing prevalent energy storage devices encompass batteries, supercapacitors, and dielectric capacitors. Batteries boast a maximum energy storage density, but exhibit a comparatively lower power density. Supercapacitors strike a balance with a moderate energy storage and a power density. Dielectric capacitors, characterized by their unparalleled power density and rapid charge/discharge rate, have extensive applications in various domains such as pulsed laser weaponry, cardiac pacemakers, and energy vehicles.

Thin film materials emerge as a favorable option for addressing device miniaturization and enhancing energy density due to their smaller volume and higher energy storage density compared to polymers and block ceramics. The energy storage ceramic thin film materials can be classified based on intrinsic polarization states, i.e., encompassing linear dielectric (LD), paraelectric (PE), ferroelectric (FE), relaxation ferroelectric (RFE), superparaelectric (SPE), and antiferroelectric (AFE) materials.

LD exhibits notable breakdown strength (E_b) and energy storage efficiency (η). However, their low dielectric constant (ε_r) and polarization (P) result in a diminished energy storage density (U_rec). Elevating ε_r stands as a pivotal for enhancing the U_rec of LD. PE demonstrates non-linear changes in P and ε_r with applied electric fields (E). For the removal of E, PE maintains a non-polar state without spontaneous polarization, featuring a medium P and a substantial E_b. FE exhibits a spontaneous polarization with large P and ε_r. Nevertheless, their prominent residual polarization (P_r), dielectric loss (tanδ), and increased defect density contribute to a lowered E_b, constraining the application of FE in energy storage. Recent research in FE focuses on mitigating P_r and augmenting E_b. In contrast to FE, RFE typically exhibits nanodomains or polar nanodomains in their domain structure. The coupling among these domains is relatively weak, rendering them highly responsive to electric fields. RFE often displays a substantial P, a minimal P_r, and a slender P-E hysteresis loop. This characteristic facilitates the attainment of elevated U_rec and η. SPE maintains a local polar order, manifesting as polarity clusters spanning only a few nanometers or cells. This arrangement further diminishes mutual coupling between domains, reducing a polarity-switching energy barrier. Losses are minimized, significantly enhancing both U_rec and η. AFE features a distinctive double hysteresis loop, stemming from the parallel and opposite alignment of spontaneous polarization on adjacent lattices. This configuration results in near-zero P_r, undergoing a reversible AFE-FE phase transition under specific E, and yielding a high ε_r and substantial P. This property enables the achievement of a heightened U_rec, presenting promising applications in energy storage.

In the realm of energy storage ceramic thin film materials, enhancing P_max, E_b, and minimizing P_r are pivotal for improving energy storage performance. To achieve these objectives, diverse modification methods are used to encompass the preparation technology, component design, and interface engineering.

For the effective preparation, optimization of preparation methods, alteration of annealing processes, substitution of electrode materials, aging, and the fabrication of multi-layer film capacitors (MLFC) are employed. These interventions regulate the orientation growth and oxygen vacancy content of the material, thereby enhancing the energy storage performance of the ceramic thin film capacitor. Note that the preparation of MLFC demonstrates a substantial U_rec (i.e., 78.3 J/cm³) and η (i.e., 90.2%) and offers valuable insights for the commercialization of ceramic film capacitors.

The composition design encompasses elements such as doping, two-phase or multiphase solid solutions, entropy control, and incorporation of nanoparticles. Specifically, element doping and the creation of two-phase or multiphase solid solutions can achieve a slender P-E hysteresis loop via transforming FE to RFE. Using Mn²⁺ to form defect complexes with oxygen vacancies is investigated. This reduces the oxygen vacancy content and curbs leakage current density, thereby enhancing the energy storage performance for various energy storage ceramic thin film materials. This method offers a universal approach to mitigating leakage current issues. Entropy control strategies introduce multiple elements into the system, utilizing chemical disorder caused by atomic size mismatch to reduce P_r and delay saturation polarization, thereby improving energy storage performance. Nanoparticle composite can be prepared via adding the nanoparticles into matrix material evenly, with the base materials to improve the energy storage of materials performance as a whole.

Interface engineering primarily enhances E_b via manipulating material structures, incorporating effects (i.e., 'dead-layer' effect, electric field amplification effect, space charge effect, heterojunction effect, interface barrier effect, and interlayer coupling effect). This optimization aims to achieve a superior energy storage performance. Multilayer films in interface engineering typically involve the use of two or more component materials, allowing the strategic utilization of diverse material characteristics to maximize effectiveness. For instance, 'dead-layer' engineering involves the incorporation of high resistivity and low ε_r Al₂O₃ layer as the top layer, enhancing the E_b of the multilayer film. In multilayer films, the interplay of various effects collectively affects their electrical properties and energy storage performance. The comprehensive consideration of these effects is crucial in the design and research of multilayer films. The energy storage performance of multilayer films can be improved, further aligning dielectric energy storage films with the practical applications.

, authors=Wenfeng YUE¹, Tingnan YAN², Dawei WANG¹, authorsList=Wenfeng YUE, Tingnan YAN, Dawei WANG, authorCompany=null, correspAuthors=Dawei WANG, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319973056756437068, articleId=1319973056223760458, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=电介质储能陶瓷薄膜研究进展及改性方法, columnId=1321894930713268924, journalTitle=硅酸盐学报, columnName=电介质储能材料专刊—综合评述, runingTitle=null, highlight=null, articleAbstract=

电介质陶瓷薄膜材料制备的储能电容器，具有充放电速率快、功率密度大以及良好的温度稳定性和循环稳定性等优势，在脉冲激光武器、心脏起搏器等军事、民用领域具有广阔的应用前景。然而，电介质电容器的储能密度相对较低，限制了其应用范围，因此如何提高其储能密度成为当前研究的重点之一。此外，电介质储能陶瓷薄膜材料种类繁多、制备工艺复杂，因此选择合适的材料体系和制备工艺至关重要。本文总结了电介质储能陶瓷薄膜材料的研究进展，重点讨论了6种类型的材料，包括线性电介质、顺电材料、铁电材料、弛豫铁电材料、超顺电材料和反铁电材料。此外，进一步总结了目前常用的提升电介质储能陶瓷薄膜材料储能性能的方法。期望本文的研究成果能够对开发新一代高性能电介质储能陶瓷薄膜提供有价值的参考。

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