Article(id=1319971972298166562, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319971875086783028, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230668, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1693411200000, receivedDateStr=2023-08-31, revisedDate=1695484800000, revisedDateStr=2023-09-24, acceptedDate=null, acceptedDateStr=null, onlineDate=1792635442089, onlineDateStr=2026-10-22, pubDate=1710864000000, pubDateStr=2024-03-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792635442089, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792635442089, creator=13701087609, updateTime=1792635442089, updator=13701087609, issue=Issue{id=1319971875086783028, tenantId=1146029695717560320, journalId=1263187385517883426, year='2024', volume='52', issue='3', pageStart='737', pageEnd='1170', issueExtLink='null', onlineDate='null', pubDate='1710864000000', pubDateStr='2024-03-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792635418912, creator='13701087609', updateTime=1792641878851, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319998970110264006, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319971875086783028, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319998970110264007, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319971875086783028, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=1128, endPage=1148, ext={EN=ArticleExt(id=1319971972491104547, articleId=1319971972298166562, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Development on Spectral Regulation of Ce³⁺-Doped Garnet-Based Fluorescent Materials, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

For the favorable physicochemical properties, high fluorescence conversion efficiencies, a relatively short fluorescence lifetime, and an efficient spectral congruence between excitation and ultraviolet/blue LED emission spectra, Ce³⁺-doped garnet-based fluorescent materials can be used in encompassing lighting, displays, medical imaging, etc.. For leveraging the diverse cation sites within a garnet structure, the emission wavelength of Ce³⁺ can be continuously adjusted from 460 nm to 610 nm via the incorporation of varied matrix chemical constituents. This versatile tunability broadens the horizons of their potential applications and augments the repertoire of materials available for advancing Ce³⁺ luminescence theory. However, recent work on Ce³⁺-doped garnet-based fluorescent materials has unveiled certain anomalies and even contradictions within the characteristics and the emission wavelength modulation theory, becoming one of the prominent bottlenecks hindering the development of this material. To address this issue, this review represented the relative theories of substrate chemical component substitution and the modulation of Ce³⁺ emission wavelengths. The review also summarized recent advancements in Ce³⁺-doped garnet-based fluorescent materials, and the influence of ion substitution on Ce³⁺ luminescence performance with the distortion factor of [CeO₈].

This review discussed the Ce³⁺-doped yttrium aluminum garnet structure as a prototype and comprehensively analyzed the impacts of commonly used doping ions that occupy the [AO₈], [BO₆], and [CO₄] sites on the emission wavelength, thermal quenching resistance, and the [CeO₈] distortion factor of Ce³⁺.

The ion substitution of a single lattice generally necessitates that the substituting ion and the substituted ion have the same valence state and exhibit a minimal disparity in atomic radius. In the case of [AO₈] lattice substitution, Y³⁺ can be replaced with rare-earth ions, i.e., Lu³⁺, Tb³⁺, Gd³⁺, and La³⁺. When the radius of the doped rare-earth ions is greater that that of Y³⁺, the emission wavelength of Ce³⁺ shifts towards the red end of the spectrum. Conversely, when the radius is smaller, the shift occurs in the opposite direction.

The ion substitution of octahedral lattice sites mainly involves the replacement of Al³⁺ by Ga³⁺, Sc³⁺, and In³⁺. With an escalation in the concentration of doped ions like Ga³⁺, Sc³⁺, and In³⁺, the peak wavelength of the Ce³⁺ emission spectrum has a blue shift. In addition, the incorporation of Sc³⁺ effectively enhances the thermal quenching resistance of Ce³⁺, while the inclusion of Ga³⁺ diminishes the thermal quenching resistance of Ce³⁺.

The main substitutions of dodecahedral-octahedral lattice ion pairs include Ca²⁺-Hf⁴⁺ and Ca²⁺-Zr⁴⁺ replacing Y³⁺-Al³⁺. The emission and excitation peak wavelengths of Ce³⁺ gradually blueshifts as Ca²⁺-Hf⁴⁺ and Ca²⁺-Zr⁴⁺ doping contents increase.

The substitution of dodecahedral-tetrahedral lattice ions is mainly achieved by M²⁺-Si⁴⁺ (M=Mg, Ca, Sr, Ba) replacing Y³⁺-Al³⁺, with alkaline earth metals occupying the dodecahedral lattice and Si⁴⁺ occupying the tetrahedral lattice. In the garnet system, when M²⁺-Si⁴⁺ replaces Y³⁺-Al³⁺, the emission wavelength of Ce³⁺ undergoes a blue shift with the increase of M²⁺ ion radius, resulting in improving the thermal stability.

The substitution of octahedral-tetrahedral lattice ions mainly involves Mg²⁺-Si⁴⁺/Ge⁴⁺ replacing Al³⁺-Al³⁺, where Mg²⁺ occupies the octahedral lattice and Si⁴⁺/Ge⁴⁺ occupies the tetrahedral lattice. Among them, Mg²⁺-Si⁴⁺ replacing Al³⁺-Al³⁺ is an effective method to achieve a large redshift of Ce³⁺ emission wavelength. The introduction of Mg²⁺-Ge⁴⁺ also leads to the redshift of Ce³⁺ emission wavelength, but the extent of this redshift is considerably less than that achieved by Mg²⁺-Si⁴⁺.

The chemical components in dodecahedral-octahedral-tetrahedral lattice co-substitutions are more intricate, with Ca²⁺ and Mg²⁺ occupying the dodecahedral lattice, Mg²⁺, Sc³⁺, and Hf⁴⁺ occupying the octahedral lattice, and Si⁴⁺ and Ge⁴⁺ in the tetrahedral lattice. Different lattice ions on the co-substitution affect the luminescence performance of Ce³⁺.

, authors=Yanna TIAN, Jintai FAN, Benxue JIANG, Jie CHEN, Shengming ZHOU, authorsList=Yanna TIAN, Jintai FAN, Benxue JIANG, Jie CHEN, Shengming ZHOU, authorCompany=null, correspAuthors=Shengming ZHOU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319971972734374180, articleId=1319971972298166562, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=Ce³⁺掺杂石榴石基荧光材料的光谱调控研究进展, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

Ce³⁺掺杂石榴石基荧光材料凭借其良好的物化特性、高荧光转换效率、较短的荧光寿命、激发光谱与紫外/蓝光发光二极管发射谱的高效匹配等特点，被广泛用于照明、显示、医学成像等领域。得益于石榴石结构丰富的阳离子格位，通过多种类基质化学组分取代可实现Ce³⁺发射波长从460~610 nm范围内的连续可调，不仅大大拓宽了其潜在应用场景，也为Ce³⁺发光理论的建立和完善提供了广泛的素材。然而随着近年来相关实验探索的大幅增加，种类较为庞杂的Ce³⁺掺杂石榴石基荧光材料特性与发射波长调控理论常常出现无法解释甚至矛盾之处，成为阻碍Ce³⁺掺杂石榴石基荧光材料发展的重要瓶颈之一。针对这一问题，本文简要介绍了基质化学组分取代调控Ce³⁺发射波长的几种主要理论，综述了近年来Ce³⁺掺杂石榴石基荧光材料的研究进展，并结合理论与实验，主要从［CeO₈］畸变因子角度出发，讨论了离子取代对Ce³⁺发光性能的影响。

, authors=田燕娜, 范金太, 姜本学, 陈杰, 周圣明, authorsList=田燕娜, 范金太, 姜本学, 陈杰, 周圣明, authorCompany=null, correspAuthors=周圣明, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=W0deuW2KSP1aAj9l1j253Q==, magXml=yTdUJHuQ1RA/5ONq09kquA==, pdfUrl=null, pdf=2qpGxFnrFYeSU69m+O5/Og==, pdfFileSize=4619737, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=9QpJpg+TxIZSfMRK5CYOaQ==, mapNumber=null, fund=null)}, authors=[Author(id=1322551188566946162, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319971972298166562, orderNo=0, firstName=null, middleName=null, lastName=null, nameCn=null, orcid=null, stid=null, country=null, authorPic=null, dead=0, email=tianyanna@siom.ac.cn, emailSecond=null, emailThird=null, correspondingAuthor=0, authorType=1, ext={EN=AuthorExt(id=1322551188655026548, tenantId=1146029695717560320, journalId=1263187385517883426, articleId=1319971972298166562, authorId=1322551188566946162, language=EN, stringName=Yanna TIAN, firstName=Yanna, middleName=null, lastName=TIAN, prefix=null, suffix=null, authorComment=null, nameInitials=null, affiliation=null, department=null, xref=null, address=Key Laboratory of Materials for High Power Lasers, Shanghai Institute of Optics and Fine Mechanics, Chinese Academy of Sciences, Shanghai 201800, China, bio={"content":"

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田燕娜（1994—），女，博士，博士后。

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田燕娜（1994—），女，博士，博士后。

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