Article(id=1319969664004899279, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319969627665445134, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20230336, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1684166400000, receivedDateStr=2023-05-16, revisedDate=1686412800000, revisedDateStr=2023-06-11, acceptedDate=null, acceptedDateStr=null, onlineDate=1792634891749, onlineDateStr=2026-10-22, pubDate=1705680000000, pubDateStr=2024-01-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792634891749, onlineIssueDateStr=2026-10-22, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792634891749, creator=13701087609, updateTime=1792634891749, updator=13701087609, issue=Issue{id=1319969627665445134, tenantId=1146029695717560320, journalId=1263187385517883426, year='2024', volume='52', issue='1', pageStart='1', pageEnd='370', issueExtLink='null', onlineDate='null', pubDate='1705680000000', pubDateStr='2024-01-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792634883085, creator='13701087609', updateTime=1792641944622, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319999245965443838, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319969627665445134, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319999245965443839, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319969627665445134, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=322, endPage=332, ext={EN=ArticleExt(id=1319969664193642960, articleId=1319969664004899279, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Modification Strategy for WO₃-Based Photocatalysts, columnId=1263922772401635899, journalTitle=Journal of the Chinese Ceramic Society, columnName=Review, runingTitle=null, highlight=null, articleAbstract=

WO₃, a typical transition metal oxide, has attracted great attentions in photocatalysis due to its abundant reserves, environmentally friendly, good physicochemical stability, visible-light response and proper band edge positions, etc.. Nevertheless, several drawbacks such as the low utilization of solar energy, high charge carrier recombination rate, weak reduction ability and limited reactive sites lead to a poor photoactivity, thus restricting the industrial application. Various modification strategies are explored and utilized to promote the photocatalytic activity. It is thus necessary to review recent development on WO₃-based photocatalysts that might provide a general guidance for designing high-efficient WO₃ catalyst systems.

Morphology control can tailor WO₃ nanomaterials to expose a highly active crystal plane, which is beneficial for reactivity. Low-dimensional nanomaterials possess the larger surface area and large quantity of unsaturated coordination sites, then accelerates the surface reaction. The charge carrier migration efficiency can be increased in a small size of catalysts due to the limited transportation distance. However, the preparation of low-dimensional WO₃ with a precise structure and a stable crystal plane is an obstacle.

Oxygen vacancy in WO₃ materials can capture the photoinduced electrons and hence suppress the recombination of electron-hole pairs. Moreover, the creation of oxygen affects the band structure that can broaden the light absorption and enhance the redox ability. Nevertheless, excessive oxygen vacancy may induce the structural instability. Thus, the precise control of oxygen vacancy in WO₃ is the key point.

Metal or non-metal doping can induce the lattice distortion and then affect the physicochemical properties of semiconductor. Doping element acts as an electron acceptor that contributes to the ultrafast charge separation. Also, the introduction of impurity energy level favors the reduction of energy band. The more comprehensive understanding of the reactive sites in doping catalysts still needs further exploitation.

Loading co-catalyst in WO₃ benefits for charge carrier separation and migration. Metal co-catalyst can increase the solar energy utilization resulting from its localized surface plasmon resonance effect. The current common co-catalysts focus on noble metal that is high cost. The pursuit of abundant reserves materials is highly desired for commercial application.

The construction of II-type, Z-type and S-type WO₃-based heterojunctions is an effective strategy for solving the problems of single materials. The charge carriers in II-type heterojunction tend to transfer from agreatability of positions to the low positions, which are beneficial for spatial separation of electron-hole pairs, but the redox ability weakens. The unique merit in Z-scheme and S-scheme heterojunction is an intense redox ability maintained in separate components, thus triggering the unique photoreaction.

, authors=Wanying LEI, Liang ZHAO, Tong ZHOU, Shixiang XUE, Pan WU, Xinxin YANG, Ziqiang TAN, authorsList=Wanying LEI, Liang ZHAO, Tong ZHOU, Shixiang XUE, Pan WU, Xinxin YANG, Ziqiang TAN, authorCompany=null, correspAuthors=null, authorNote=, correspAuthorsNote=null, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319969665649066449, articleId=1319969664004899279, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=WO₃基光催化剂的改性策略现状与展望, columnId=1263922774356181565, journalTitle=硅酸盐学报, columnName=综合评述, runingTitle=null, highlight=null, articleAbstract=

WO₃是一种典型的过渡金属氧化物，具有储量丰富、绿色环保、稳定性好、可见光响应和合适的能带结构等特性，在光催化领域有广阔的应用前景，但是较低的太阳能利用率、较高的载流子复合率、弱的还原能力和活性位点密度低等缺点导致其性能较低，从而极大限制了其实际应用。本文综述了近年来WO₃光催化材料的改性策略，包括形貌调控、氧空位调控、元素掺杂、助催化剂负载、构建异质结等。最后讨论了WO₃材料现阶段的制约点和其在未来能源转化领域的发展方向。

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LEI Wanying (1991-), female, Ph.D., Associate Professor. E-mail: leiwy@xauat.edu.cn

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LEI Wanying (1991-), female, Ph.D., Associate Professor. E-mail: leiwy@xauat.edu.cn

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雷琬莹（1991—），女，博士，副教授。

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雷琬莹（1991—），女，博士，副教授。

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