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Article(id=1319239205516071301, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236892848148894, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220366, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1651766400000, receivedDateStr=2022-05-06, revisedDate=1654617600000, revisedDateStr=2022-06-08, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460736874, onlineDateStr=2026-10-20, pubDate=1668873600000, pubDateStr=2022-11-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460736874, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460736874, creator=13701087609, updateTime=1792460736874, updator=13701087609, issue=Issue{id=1319236892848148894, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='11', pageStart='2809', pageEnd='3090', issueExtLink='null', onlineDate='null', pubDate='1668873600000', pubDateStr='2022-11-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460185491, creator='13701087609', updateTime=1792460700564, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319239053275411177, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236892848148894, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319239053275411178, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319236892848148894, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=2924, endPage=2933, ext={EN=ArticleExt(id=1319239205700620678, articleId=1319239205516071301, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Anti-Shedding and Carbon Monoxide Catalytic Removal of Flue Gas of Structural Catalyst, columnId=1263922769897599102, journalTitle=Journal of the Chinese Ceramic Society, columnName=Research Articles, runingTitle=null, highlight=null, articleAbstract=

High activity and durable structural catalysts are increasingly needed for carbon monoxide (CO) catalytic removal of industrial flue gas. A series of structural catalysts were prepared by coating polymetallic oxide catalyst on cordierite honeycomb supports. The results showed that silica sol and hot air drying could promote the powder catalyst to evenly and compactly spread on the surface of the support, and improve the anti-shedding performance and catalytic performance of the structural catalyst. The coating shedding rate of the optimized catalyst after 60 min of ultrasonic vibration was 0.97%. The catalytic efficiency of 99% CO can be achieved at 7 500 h-1 space speed, 1% CO, 8% water vapour content and 110 ℃, and remains stable within 72 h. The CO catalytic efficiency can be stabilized above 86% after 720 h in actual sintering flue gas condition.

, authors=Xuan ZHANG1, Yingshu LIU1, Huanyu HOU2, Wenbo BIAN1, Lijun JIANG1, Chuanzhao ZHANG3, Fangzhou SUN2, Xiong YANG1, Ziyi LI1, authorsList=Xuan ZHANG, Yingshu LIU, Huanyu HOU, Wenbo BIAN, Lijun JIANG, Chuanzhao ZHANG, Fangzhou SUN, Xiong YANG, Ziyi LI, authorCompany=null, correspAuthors=Ziyi LI, authorNote=

ZHANG Xuan (1997-), female, Doctoral candidate. E-mail:

, correspAuthorsNote=
LI Ziyi (1990-), male, Ph.D., Professor. E-mail:
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工业烟气一氧化碳（CO）的催化净化对高活性耐久结构型催化剂的需求日渐迫切。将多元金属氧化物催化剂涂覆到堇青石蜂窝载体上制得了一系列结构型催化剂。结果表明，硅溶胶与热风吹动干燥可促进粉末催化剂均匀致密平铺在载体表面，提高了结构型催化剂的抗脱落性能与催化性能，优选催化剂超声60 min后的涂层脱落率为0.97%；在7 500 h-1空速、1% CO、8%水蒸气含量、110 ℃可达到99% CO催化效率，并在72 h内保持稳定；在实际烧结烟气条件下，720 h后CO催化效率可稳定在86%以上。

, authors=张璇1, 刘应书1, 侯环宇2, 卞文博1, 姜理俊1, 张传钊3, 孙方舟2, 杨雄1, 李子宜1, authorsList=张璇, 刘应书, 侯环宇, 卞文博, 姜理俊, 张传钊, 孙方舟, 杨雄, 李子宜, authorCompany=null, correspAuthors=李子宜, authorNote=

张璇（1997—），女，博士研究生。

, correspAuthorsNote=
李子宜（1990—），男，博士，教授。
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ZHANG Xuan (1997-), female, Doctoral candidate. E-mail:

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ZHANG Xuan (1997-), female, Doctoral candidate. E-mail:

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张璇（1997—），女，博士研究生。

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张璇（1997—），女，博士研究生。

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结构型催化剂的抗脱落及烟气一氧化碳催化净化性能
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张璇 1 , 刘应书 1 , 侯环宇 2 , 卞文博 1 , 姜理俊 1 , 张传钊 3 , 孙方舟 2 , 杨雄 1 , 李子宜 1
硅酸盐学报 | 研究论文 2022,50(11): 2924-2933
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硅酸盐学报 |研究论文 2022 , 50 (11) : 2924 -2933
结构型催化剂的抗脱落及烟气一氧化碳催化净化性能
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张璇1 , 刘应书1, 侯环宇2, 卞文博1, 姜理俊1, 张传钊3, 孙方舟2, 杨雄1, 李子宜1
作者信息
  • 1．北京科技大学能源与环境工程学院，北京 100083
  • 2．河钢集团钢研总院，石家庄 050023
  • 3．北京联合大学生物化学工程学院，北京 100023
通讯作者:
李子宜（1990—），男，博士，教授。
作者简介:

张璇（1997—），女，博士研究生。

Anti-Shedding and Carbon Monoxide Catalytic Removal of Flue Gas of Structural Catalyst
Xuan ZHANG1 , Yingshu LIU1, Huanyu HOU2, Wenbo BIAN1, Lijun JIANG1, Chuanzhao ZHANG3, Fangzhou SUN2, Xiong YANG1, Ziyi LI1
Affiliations
  • 1.School of Energy and Environmental Engineering, University of Science and Technology Beijing, Beijing 100083, China
  • 2.Strategic Research Institute of HBIS Group, Shijiazhuang 050023, China
  • 3.College of Health and Environment, Beijing Union University, Beijing 100023, China
    • Corresponding Author:
    LI Ziyi (1990-), male, Ph.D., Professor. E-mail:

    ZHANG Xuan (1997-), female, Doctoral candidate. E-mail:

出版时间: 2022-11-20 doi: 10.14062/j.issn.0454-5648.20220366
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工业烟气一氧化碳（CO）的催化净化对高活性耐久结构型催化剂的需求日渐迫切。将多元金属氧化物催化剂涂覆到堇青石蜂窝载体上制得了一系列结构型催化剂。结果表明，硅溶胶与热风吹动干燥可促进粉末催化剂均匀致密平铺在载体表面，提高了结构型催化剂的抗脱落性能与催化性能，优选催化剂超声60 min后的涂层脱落率为0.97%；在7 500 h-1空速、1% CO、8%水蒸气含量、110 ℃可达到99% CO催化效率，并在72 h内保持稳定；在实际烧结烟气条件下，720 h后CO催化效率可稳定在86%以上。

结构型催化剂  /  涂覆制备  /  一氧化碳  /  催化净化  /  脱落率

High activity and durable structural catalysts are increasingly needed for carbon monoxide (CO) catalytic removal of industrial flue gas. A series of structural catalysts were prepared by coating polymetallic oxide catalyst on cordierite honeycomb supports. The results showed that silica sol and hot air drying could promote the powder catalyst to evenly and compactly spread on the surface of the support, and improve the anti-shedding performance and catalytic performance of the structural catalyst. The coating shedding rate of the optimized catalyst after 60 min of ultrasonic vibration was 0.97%. The catalytic efficiency of 99% CO can be achieved at 7 500 h-1 space speed, 1% CO, 8% water vapour content and 110 ℃, and remains stable within 72 h. The CO catalytic efficiency can be stabilized above 86% after 720 h in actual sintering flue gas condition.

structural catalyst  /  coating preparation  /  carbon monoxide  /  catalytic removal  /  shedding rate
张璇, 刘应书, 侯环宇, 卞文博, 姜理俊, 张传钊, 孙方舟, 杨雄, 李子宜. 结构型催化剂的抗脱落及烟气一氧化碳催化净化性能. 硅酸盐学报, 2022 , 50 (11) : 2924 -2933 . DOI: 10.14062/j.issn.0454-5648.20220366
Xuan ZHANG, Yingshu LIU, Huanyu HOU, Wenbo BIAN, Lijun JIANG, Chuanzhao ZHANG, Fangzhou SUN, Xiong YANG, Ziyi LI. Anti-Shedding and Carbon Monoxide Catalytic Removal of Flue Gas of Structural Catalyst[J]. Journal of the Chinese Ceramic Society, 2022 , 50 (11) : 2924 -2933 . DOI: 10.14062/j.issn.0454-5648.20220366
基金
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  • 国家自然科学基金项目(21808012)
  • 河钢集团有限公司重点科技项目(HG2020204-1)
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2022年第50卷第11期
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doi: 10.14062/j.issn.0454-5648.20220366
  • 接收时间：2022-05-06
  • 首发时间：2026-10-20
  • 出版时间：2022-11-20
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  • 收稿日期：2022-05-06
  • 修回日期：2022-06-08
基金
国家自然科学基金项目(21808012)
河钢集团有限公司重点科技项目(HG2020204-1)
作者信息
    1．北京科技大学能源与环境工程学院，北京 100083
    2．河钢集团钢研总院，石家庄 050023
    3．北京联合大学生物化学工程学院，北京 100023

通讯作者:

李子宜（1990—），男，博士，教授。
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https://castjournals.cast.org.cn/joweb/gsyxb/CN/10.14062/j.issn.0454-5648.20220366
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2种不同金属材料的力学参数
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Family		 属数
Number of
genus		 种数
Number of
species		 占总种数比例
Percentage of
total species (%)		 属
Genus		 种数
Number of
species		 占总种数比例
Percentage of total
species (%)
鹅膏菌科Amanitaceae 2 11 5.26 鹅膏菌属 Amanita 10 4.78
小菇科 Mycenaceae 2 12 5.74 丝盖伞属 Inocybe 5 2.39
多孔菌科 Polyporaceae 8 14 6.70 蜡蘑属 Laccaria 5 2.39
红菇科 Russulaceae 3 23 11.00 小皮伞属 Marasmius 6 2.87
小菇属 Mycena 11 5.26
光柄菇属 Pluteus 5 2.39
红菇属 Russula 17 8.13
栓菌属 Trametes 5 2.39
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