Article(id=1319237194645090588, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319237171312177253, articleNumber=null, orderNo=null, doi=10.14062/j.issn.0454-5648.20220508, pmid=null, cstr=null, oa=null, hot=null, price=null, onlineType=0, articleFormat=0, articleType=null, articleTypeStr=null, receivedDate=1655913600000, receivedDateStr=2022-06-23, revisedDate=1659369600000, revisedDateStr=2022-08-02, acceptedDate=null, acceptedDateStr=null, onlineDate=1792460257445, onlineDateStr=2026-10-20, pubDate=1671465600000, pubDateStr=2022-12-20, doiRegisterDate=null, doiRegisterDateStr=null, onlineIssueDate=1792460257445, onlineIssueDateStr=2026-10-20, onlineJustAcceptDate=null, onlineJustAcceptDateStr=null, onlineFirstDate=null, onlineFirstDateStr=null, sourceXml=null, magXml=null, createTime=1792460257445, creator=13701087609, updateTime=1792460257445, updator=13701087609, issue=Issue{id=1319237171312177253, tenantId=1146029695717560320, journalId=1263187385517883426, year='2022', volume='50', issue='12', pageStart='3091', pageEnd='3336', issueExtLink='null', onlineDate='null', pubDate='1671465600000', pubDateStr='2022-12-20', beforeIssueId=null, nextIssueId=null, price=null, status=1, issueComplete=1, articleOrder=1, issueType=-1, specialIssue=null, createTime=1792460251882, creator='13701087609', updateTime=1792460721974, updator='13701087609', preIssue=null, nextIssue=null, articleTotal=null, ext={EN=IssueExt(id=1319239143067071226, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319237171312177253, language=EN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=), CN=IssueExt(id=1319239143067071227, tenantId=1146029695717560320, journalId=1263187385517883426, issueId=1319237171312177253, language=CN, specialIssueTitle=, coverIllustrator=null, specialIssueEditor=, specialIssueAbout=)}, issueFiles=null, downloadFileDto=null}, startPage=3185, endPage=3198, ext={EN=ArticleExt(id=1319237195253264669, articleId=1319237194645090588, tenantId=1146029695717560320, journalId=1263187385517883426, language=EN, title=Rare-Earth Element Ions Doped Upconversion Nanocrystals in Near-Infrared Photodetectors Applications, columnId=1321891438401532897, journalTitle=Journal of the Chinese Ceramic Society, columnName=Advanced Rare Earth Luminescence Materials for Sensing and Detection—Review, runingTitle=null, highlight=null, articleAbstract=

Photodetection technology is widely used, especially near-infrared (NIR) photodetector plays an essential role in military, communication and industrial automation. With the development of semiconductor laser technology, multiband photodetectors (PDs) have great application prospects in imaging technology, environmental monitoring, medical detection, optical communication, and flexible equipment. The selective PDs of the NIR Ⅰ-Ⅱ region with a low pump threshold and a high sensitivity is investigated for developing polychromatic bioimaging/sensor encrypted communication in bioanalysis. Recent work on the NIR selective PDs mainly focus on integrating infrared semiconductor materials with different band gaps and NIR response capabilities as well as increasing the complexity and stability of the device design and cost. Rare-earth ions (RE³⁺) doped upconversion nanocrystals (UCNCs) can absorb the NIR photons and convert them into UV or Vis photons, then being absorbed by semiconductors with a wide band gap. The UCNCs have a large Stokes/anti-Stokes shift, a superior photostability, and a selective absorption at NIR wavelengths, thus considering as good narrowband NIR photoactive materials with a potential strategy for developing the new generation of NIR selective PDs. In UCNCs-based PDs, coupling with perovskite, graphene, or MoS₂ enables the PDs to exhibit an excellent responsivity and achieve a wide spectral range that a single component cannot achieve. However, UCNCs-based PDs have some problems of low fluorescence efficiency and high pump threshold of UCNCs in practical application. This review summarized recent research on utilizing RE³⁺-doped UCNCs as photoactive materials for NIR PDs, and represented several primary strategies for enhancing UCL efficiency/intensity to achieve narrowband NIR PDs. Meanwhile, the advancement of combining UCNCs with perovskite, graphene, and MoS₂ for the NIR PDs was described. In addition, recent work on RE³⁺-doped UC-perovskite NIR PDs was also given.

, authors=Yanan JI, Wen XU, authorsList=Yanan JI, Wen XU, authorCompany=null, correspAuthors=Wen XU, authorNote=, correspAuthorsNote=, copyrightStatement=null, copyrightOwner=null, extLink=null, articleAbsUrl=null, sourceXml=null, magXml=null, pdfUrl=null, pdf=null, pdfFileSize=null, pdfExtLink=null, richHtmlUrl=null, mobilePdfUrl=null, reviewReport=null, pdfFirstPage=null, abstractGraph=null, abstractGraphContent=null, abstractVideo=null, citation=null, cebUrl=null, magXmlContent=null, mapNumber=null, fund=null), CN=ArticleExt(id=1319237195580420382, articleId=1319237194645090588, tenantId=1146029695717560320, journalId=1263187385517883426, language=CN, title=稀土掺杂上转换纳米材料在近红外光电探测器中的应用, columnId=1321891439131341794, journalTitle=硅酸盐学报, columnName=稀土发光传感与探测新材料专题—综合评述, runingTitle=null, highlight=null, articleAbstract=

近红外（NIR）光电检测技术的应用非常广泛，如日常生活中的生物热成像仪、生物追踪、运动手表等，以及军事国防中的无人机、导弹制导、生产自动化等领域均扮演着重要的角色，具有波长选择性的NIR PDs在红外成像、环境监测、医疗检测、光通信等领域有着广阔的应用前景，开发易于集成、高灵敏度、低泵浦阈值的NIRⅠ-Ⅱ区的多波段选择性PDs，对加密通信生物分析等领域的发展具有重要意义。目前，波长选择性光电探测技术的应用，侧重于集成多个不同带隙，且对NIR有不同的光响应能力的半导体材料，但这不仅增加了器件的制备成本和设计上的复杂性，又严重影响其稳定性。稀土离子（RE³⁺）掺杂上转换纳米晶（UCNCs）具有大Stokes/反Stokes位移以及优异的光稳定性，吸收NIR光子后将其转化为UV/Vis光子，被窄带隙半导体材料吸收。UCNCs因为具有窄带NIR波长选择性吸收特性等优点，被视为一种优异的光敏材料，为开发新一代的波长选择性PDs提供了解决方案。研究表明：UCNCs的光电检测中，UCNCs与钙钛矿、石墨烯、MoS₂的结合可以使PDs展现出更好的光响应能力，实现单个组件无法获得的更大的光谱范围。但在实际应用中，仍需面临UCNCs的荧光效率低、泵浦阈值高的问题。

本文综述了近年来利用稀土掺杂UCNCs作为光活性材料用于NIR PDs的研究进展，主要包括：提高UCNCs发光效率/发光强度以实现窄带NIR探测的几种主要策略；UCNCs与钙钛矿、石墨烯、MoS₂结合应用于NIR PDs的研究现状；稀土掺杂上转换钙钛矿基NIR PDs的最新研究进展。

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JI Yanan (1992-), female, Ph.D., Lecturer. E-mail: jiyn@dlnu.edu.cn

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JI Yanan (1992-), female, Ph.D., Lecturer. E-mail: jiyn@dlnu.edu.cn

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季亚楠（1992—），女，博士，讲师。

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季亚楠（1992—），女，博士，讲师。

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